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Sinars DB Slutz SA Herrmann MC McBride RD Cuneo ME Peterson KJ Vesey RA Nakhleh C Blue BE Killebrew K Schroen D Tomlinson K Edens AD Lopez MR Smith IC Shores J Bigman V Bennett GR Atherton BW Savage M Stygar WA Leifeste GT Porter JL 《Physical review letters》2010,105(18):185001
The first controlled experiments measuring the growth of the magneto-Rayleigh-Taylor instability in fast (~100 ns) Z-pinch plasmas are reported. Sinusoidal perturbations on the surface of an initially solid Al tube (liner) with wavelengths of 25-400 μm were used to seed the instability. Radiographs with 15 μm resolution captured the evolution of the outer liner surface. Comparisons with numerical radiation magnetohydrodynamic simulations show remarkably good agreement down to 50 μm wavelengths. 相似文献
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Moses AW Raab C Nelson RC Leifeste HD Ramsahye NA Chattopadhyay S Eckert J Chmelka BF Scott SL 《Journal of the American Chemical Society》2007,129(28):8912-8920
Deposition of CH3ReO3 onto the surface of dehydrated, amorphous silica-alumina generates a highly active, supported catalyst for the metathesis of olefins. However, silica-alumina with a high (10 wt %) Re loading is no more active than silica-alumina with low (1 wt %) loading, while CH3ReO3 on silica is completely inactive. Catalysts prepared by grafting CH3ReO3 on silica-alumina contain two types of spectroscopically distinct sites. The more strongly bound sites are responsible for olefin metathesis activity and are formed preferentially at low Re loadings (< or =1 wt %). They are created by two Lewis acid/base interactions: (1) the coordination of an oxo ligand to an Al center of the support and (2) interaction of one of the adjacent bridging oxygens (AlOSi) with the Re center. At higher Re loadings (1-10 wt %), CH3ReO3 also interacts with surface silanols by H-bonding. This gives rise to highly mobile sites, most of which can be observed by 13C solid-state NMR even without magic-angle spinning. Their formation can be prevented by capping the surface hydroxyl groups with hexamethyldisilazane prior to grafting CH3ReO3, resulting in a metathesis catalyst that is more selective, more robust, and more efficient in terms of Re use. 相似文献
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We present evidence for a nonsingular origin of the Universe with intial conditions determined by quantum physics and relativistic
gravity. In particular, we establish that the present temperature of the microwave background and the present density of the
Universe agree well with our predictions from these intial conditions, after evolution to the present age using the Einstein-Friedmann
equation. Remarkably, the quantum origin for the Universe naturally allows its evolution at exactly the critical density.
We also discuss the consequences of these results to some fundamental aspects of quantum physics in the early Universe. 相似文献
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