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1.
We investigate the dynamics of the Λ system driven by two resonant laser fields in presence of dissipation for coupling strengths where the rotating‐wave approximation starts to break down. This regime is characterised by Rabi frequencies being approximately equal or smaller than the field frequencies. A systematic procedure to obtain an expansion for the solution of the Bloch evolution equations of the system is presented. The lowest contribution results to be the well‐known rotating‐wave approximation. The method is based on a semi‐classical treatment of the problem, and its predictions are interpreted fully quantum mechanically. The theory is illustrated by a detailed study of the disappearance of coherent population trapping as the intensities of the fields increase.  相似文献   
2.
It is shown that the dephasing which suppresses the weak localization correction to the conductivity has the same physical origin than pair-breaking in superconductors and thus-following de Gennes-may be expressed in terms of the correlation function of the operator for time reversal.  相似文献   
3.
For bounded normal operators in Krein spaces we give a necessary and sufficient condition for strong stability. The same result for unitary operators was obtained by M.G.Krein [1] (see also [2]). For selfadjoint operators we refer to the papers of P.Jonas, H.Langer [3] and H.Langer [4].  相似文献   
4.
Novel organylthio(alkoxy)silanes (I, II, III and XII) and organylthio(diethylamino)silanes (IV, V) are described. They were prepared by treating lithium or lead thiolates with the corresponding chlorosilanes or by cleavage of dimethylbis(diethylamino)silane with thiols. Phenylthiosilanes (Me3SiSPh, III and XIII) furthermore can be obtained by reaction of chlorosilanes with benzenethiol in the presence of tertiary amines. The SiS bond of Me3SiSPh is cleaved by chlorosilanes like Me2Si(NEt2)Cl or Me2Si(OPr)Cl. This reaction is a convenient route to prepare compounds I and IV. The physical and chemical properties of the novel compounds were investigated.  相似文献   
5.
6.
Carbon K‐edge X‐ray spectroscopy has been applied to the study of a wide range of organic samples, from polymers and coals to interstellar dust particles. Identification of carbonaceous materials within these samples is accomplished by the pattern of resonances in the 280–320 eV energy region. Carbonate minerals are often encountered in the study of natural samples, and have been identified by a distinctive resonance at 290.3 eV. Here C K‐edge and Ca L‐edge spectra from a range of carbonate minerals are presented. Although all carbonates exhibit a sharp 290 eV resonance, both the precise position of this resonance and the positions of other resonances vary among minerals. The relative strengths of the different carbonate resonances also vary with crystal orientation to the linearly polarized X‐ray beam. Intriguingly, several carbonate minerals also exhibit a strong 288.6 eV resonance, consistent with the position of a carbonyl resonance rather than carbonate. Calcite and aragonite, although indistinguishable spectrally at the C K‐edge, exhibited significantly different spectra at the Ca L‐edge. The distinctive spectral fingerprints of carbonates provide an identification tool, allowing for the examination of such processes as carbon sequestration in minerals, Mn substitution in marine calcium carbonates (dolomitization) and serpentinization of basalts.  相似文献   
7.
Seemingly heartbreaking for a stereochemist, the one-step selective construction of a stereopentad and its prompt destruction by aromatization has been proven to be an efficient strategy for the synthesis of fivefold substituted, pharmacologically highly active arenes (see scheme).  相似文献   
8.
We propose a new transport mechanism through tunnel-coupled quantum dots based on the coherent population trapping effect. Coupling to an excited level by the coherent radiation of two microwaves can lead to an extremely narrow current antiresonance. The effect can be used to determine interdot dephasing rates and is a mechanism for a very sensitive, optically controlled current switch.  相似文献   
9.
We present a clustering method for collections of graphs based on the assumptions that graphs in the same cluster have a similar role structure and that the respective roles can be founded on implicit vertex types. Given a network ensemble (a collection of attributed graphs with some substantive commonality), we start by partitioning the set of all vertices based on attribute similarity. Projection of each graph onto the resulting vertex types yields feature vectors of equal dimensionality, irrespective of the original graph sizes. These feature vectors are then subjected to standard clustering methods. This approach is motivated by social network concepts, and we demonstrate its utility on an ensemble of personal networks of migrants, where we extract structurally similar groups and show their resemblance to predicted acculturation strategies.  相似文献   
10.
PDE-constrained optimization problems under the influence of perturbation parameters are considered. A quantitative stability analysis for local optimal solutions is performed. The perturbation directions of greatest impact on an observed quantity are characterized using the singular value decomposition of a certain linear operator. An efficient numerical method is proposed to compute a partial singular value decomposition for discretized problems, with an emphasis on infinite-dimensional parameter and observation spaces. Numerical examples are provided.  相似文献   
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