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Influence of Sulfation on the Catalytic Activity of Ni-ZrO2 for NO Reduction with Propane in Excess Oxygen 下载免费PDF全文
Selective catalytic reduction (SCR) of nitric oxide with propane in excess oxygen was investigated on Ni-ZrO2 (NZ) and sulfated Ni-ZrO2 (SNZ), prepared by coprecipitation from a mixture of nickel nitrate-zirconium oxychloride followed by modifying with (NH4)2SO4. It was found that sulfated Ni-ZrO2 catalyst showed higher activity for the SCR of NO with propane than that of Ni-ZrO2. The structural and surface properties of catalysts were studied by XRD, BET, SEM and FT-IR of pyridine adsorption. The experimental results indicated that the modification of (NH4)2SO4 resulted in the generation of strong BrOnsted and Lewis acid sites and promoted the dispersion of the Ni species, which could lead to higher NO conversion and propane efficiency in NO reduction. 相似文献
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微纳光纤环形腔作为传感器件,具有灵敏度高、响应快的优点,因而越来越广泛地应用在传感领域。环形腔的谐振光谱直接反映外界环境的变化,因此谐振光谱分析对探测环境参数至关重要。从理论和实验研究了微纳光纤环形腔谐振光谱与海水温度的关系。首先,数值计算了基模(HE11)两个垂直偏振态的传播常数随光纤直径和探测波长的变化关系,计算结果表明传播常数随光纤直径增大而增大,随波长增大而减小,同时计算了传播常数随海水温度的变化,海水温度越高,传播常数越大,表明海水温度的变化会影响到模式的传播常数,因而可以通过测量谐振光谱的变化得知海水温度的变化。其次,搭建了海水温度传感实验系统,获得了微纳光纤环形腔海水温度的谐振光谱,实验发现同时存在两套谐振峰,分别对应基模的TE模和TM模,两个偏振模式的传感灵敏度分别为5.54和5.24 pm·℃-1。最后,探讨了基模两个偏振态谐振光谱的产生原因,由于结型耦合区的扭曲耦合使得两个偏振态分离,并对两个偏振模式的谐振强度进行了分析。两个模式的谐振强度不同,而且随着波长的增加,一个模的谐振强度不断增强,另一个模的谐振强度逐渐减弱。这是由于不同耦合态的耦合系数和衰减决定的,而且他们随着波长而改变。实验结果与理论计算相吻合。 相似文献
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Measurement of integral diffraction coefficients of crystals on beamline 4B7 of Beijing Synchrotron Radiation Facility 下载免费PDF全文
Integral diffraction coefficients of the crystal are the essential data of a crystal spectrometer which is extensively used to measure quantitative x-ray spectra of high temperature plasmas in kilo-electron-volt region. An experimental method has been developed to measure the integral diffraction coefficients of crystals on beamline 4B7 of Beijing Synchrotron Radiation Facility. The integral diffraction coefficients of several crystals including polyethylene terephthalate (PET), thallium acid phthalate (TlAP) and rubidium acid phthalate (RAP) crystals have been measured in the x-ray energy range 2100--5600 eV and compared with the calculations of the 'Darwin Prins' and the 'Mosaic' models. It is shown that the integral diffraction coefficients of these crystals are between the calculations of the 'Darwin Prins' and the 'Mosaic' models, but more close to the `Darwin Prins' model calculations. 相似文献
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金融交易指标是分析股票等金融产品买入和卖出策略的普遍选择,但由于指标描述交易策略的模糊性,使得非专业人士很难掌握交易的时间和数量。针对上述问题,本文首先分析随机指标的交易策略。其次根据交易策略和模糊集理论建立模糊推理系统模型,此模型可以给出具体的股票交易策略,包括买入以及卖出的时间和数量等,并通过给定时间段内的获利情况来判断模型的有效性。最后以沪深A股市场的15只股票价格作为实验数据,对模型的有效性进行检验。实验表明,在没有人为因素参与的情况下,大多数股票由系统进行模拟交易都可以在一段时间内获取更大的利润。 相似文献
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