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The crystal growth,x-ray diffraction pattern,absorption spectrum,emission spectrum,and fluorescence lifetime of a Tb:Lu_2O_3 single crystal were studied.Excited at 483 nm,the peak absorption cross-section was calculated to be 3.5×10~(-22)cm~2,and the full width at half maximum was found to be 2.85 nm.The Judd-Ofelt(J-O)intensity parameters ?_2,?_4,and ?_6 were computed to be 3.79×10~(-20)cm~2,1.30×10~(-20)cm~2,and 1.08×10~(-20)cm~2,with a spectroscopic quality factor ?_4/?_6 being 1.20.The emission cross-sections of green emission around 543 nm and yellow emission around 584 nm were calculated to be 9.43×10~(-22)cm~2 and 1.32×10~(-22)cm~2,respectively.The fluorescence lifetimeτexp of ~5D_4 was fitted to be 1.13 ms.The data suggest that the Tb:Lu_2O_3 crystal could be a potential candidate for green and yellow laser operation. 相似文献
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用提拉法技术生长出了掺Bi的α-BaB2O4单晶并经过γ射线辐照.测定了样品在室温下的吸收光谱、发射光谱及荧光衰减曲线.在808 nm波长光的激发下,经γ射线辐照后的α-BaB2O4单晶中发现了中心波长为1139 nm、半高宽为113 nm的近红外宽带发光现象.讨论了辐照条件和退火处理对Bi离子发光的影响.对于其发光机理进行了初步的探讨.
关键词:
近红外宽带发光
2O4单晶')" href="#">α-BaB2O4单晶
辐照
退火处理 相似文献
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Intensities and spectral features of the ~4I_(13/2)-~4I_(15/2) potential laser transition of Er~(3+) centers in CaF_2-CeF_3 disordered crystal 下载免费PDF全文
A CaF_2-CeF_3 disordered crystal containing 1.06% of Er~(3+) ions was grown by the temperature gradient technique.Optical absorption and emission spectra recorded at room temperature and at 10 K, luminescence decay curve recorded at room temperature, and extended x-ray-absorption fine structure spectra were analyzed with an intention to assess the laser potential related to the ~4I_(13/2)→~4I_(15/2) transition of Er~(3+). In addition, the thermal diffusivity of the crystal was measured at room temperature. The analysis of room-temperature spectra revealed that the ~4I_(13/2) emission is long-lived with a radiative lifetime value of 5.5 ms, peak emission cross section of 0.73 × 10~(-20) cm~2, and large spectral width pointing at the tunability of the emission wavelength in the region stretching from approximately 1480 nm to 1630 nm. The energies of the crystal field components for the ground and excited multiplets determined from low-temperature absorption and emission spectra made it possible to predict successfully the spectral position and shape of the room-temperature ~4I_(13/2)→~4I_(15/2) emission band. Based on the correlation of the optical spectra and dynamics of the luminescence decay, it was concluded that in contrast to Yb~(3+) ions in heavily doped CaF_2 erbium ions in the CaF_2-CeF_3 crystal reside in numerous sites with dissimilar relaxation rates. 相似文献
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用提拉法技术生长出了Bi:α-BaB2O4单晶,并进行电子束辐照.测定了电子束辐照前后的吸收谱和荧光发射谱.在808 nm波长激光二极管的激发下,电子束辐照后的Bi:α-BaB2O4单晶中观测到了中心波长在1135 nm附近、半高宽为52 nm左右的近红外宽带发光现象.近红外宽带发光的发光中心是Bi+离子.电子束射线起到了将Bi3+和Bi2+还原至一价态
关键词:
近红外宽带发光
2O4单晶')" href="#">α-BaB2O4单晶
电子束辐照 相似文献
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Crystal growth,spectroscopic characteristics,and Judd–Ofelt analysis of Dy:Lu_2O_3 for yellow laser 下载免费PDF全文
Dy:Lu_2O_3 was grown by the float-zone(Fz) method. According to the absorption spectrum, the Judd–Ofelt(JO) parameters ?_2, ?_4, and ?_6 were calculated to be 4.86 × 10~(-20) cm~2, 2.02 × 10~(-20) cm~2, and 1.76 × 10~(-20) cm~2, respectively.The emission cross-section at 574 nm corresponding to the ~4F6_(9/2)→~6H_(13/2) transition was calculated to be 0.53 × 10~(-20) cm~2.The yellow(~4F_(9/2)→~6H_(13/2) transition) to blue(~4F_(9/2)→~6H_(15/2) transition) intensity ratio ranges up to 12.9. The fluorescence lifetime of the ~4F_(9/2) energy level was measured to be 112.1 μs. These results reveal that Dy:Lu_2O_3 is a promising material for use in yellow lasers. 相似文献
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The 4-at.% Tm:Sc_2SiO_5 (Tm:SSO) crystal is successfully obtained by the Czochralski method. The optical properties and thermal conductivity of the crystal are investigated. The broad continuous wave(CW) laser output of(100)-cut Tm:SSO with the dimensions of 3 mm×3 mm×3 mm under laser diode(LD)-pumping is realized. The full width at half maximum(FWHM) of the laser emitting reaches up to 21 nm. The laser threshold of Tm:SSO is measured to be 0.43 W. Efficient diode-pumped CW laser performance of Tm:SSO is demonstrated with a slope efficiency of 25.9% and maximum output power of 934 mW. 相似文献
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