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研发能够精确、实时、原位获取热液甲烷数据的深海甲烷传感器对深海研究具有非常重要的意义。前期研制的两款深海甲烷光学成像干涉系统,均利用甲烷辐射光谱开展甲烷状态参数探测和反演。首先,以分子光谱辐射理论为基础,建立了分子辐射光谱与浓度、温度、压强的理论关系式,结合深海高压环境特点,建立了基于Lorentz线型的深海分子辐射模型,该模型为利用光谱法定量反演分子浓度、温度、压强等状态参数提供理论依据,同时为深海分子光谱仿真提供有力工具。接着,借助HITRAN分子光谱数据库提供的分子基本谱线参数,挑选出甲烷成像干涉系统的光源谱线。对比CH4分子与CO2, H2S, H2O等分子的特征吸收谱线,在5 990~6 150 cm-1波段范围内,CH4谱线强度比CO2, H2S, H2O等三种干扰分子的谱线强度约高2~3个数量级,且此波段内甲烷六条有效谱线分布均匀,谱线间距皆约为2~3 nm,非常适合采用光谱法进行分子状态参数探测,因此选择谱线干扰较弱、谱线分布均匀、谱线间距适中的甲烷六条谱线(1 640.37, 1 642.91, 1 645.56, 1 648.23, 1 650.96和1 653.72 nm)作为甲烷成像干涉探测系统的目标光源谱线。最后,基于深海分子辐射模型和HITRAN数据库的甲烷分子基本谱线参数,人工合成了甲烷任意浓度,任意温度和任意压强的辐射光谱数据,并分析了甲烷辐射光谱随浓度、温度和压强的变化特征。对于单一中心谱线,甲烷分子辐亮度随着浓度的升高而线性增大,随着温度的升高而非线性增大,随着压强的升高而非线性减小。对于全波段谱线,甲烷辐射光谱的全线宽随着浓度、温度的升高而变宽,随着压强的升高而变窄。建立的深海甲烷辐射光谱理论和仿真分析结果,可以为基于光谱法的海洋原位甲烷传感器的研制和数据反演提供数据支撑和理论依据。 相似文献
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Spin-Polarized Transport through the T-Shaped Double Quantum Dots with Fano-Kondo Interaction 下载免费PDF全文
We theoretically investigate the spin-polarized transport properties of the T-shaped double quantum dots coupled to two ferromagnetic leads by the Anderson Hamiltonian. The Hamiltonian is solved by means of the slave-boson mean-field theory. We calculate the density of states and the liner conductance in this system with both parallel and antiparallel lead-polarization alignments, and our results show that the transport properties of this system depend on both the tunnelling strength between the two dots and the spin-polarized strength p. This system is a possible candidate for spin valve transistors in the spintronics. 相似文献
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Using the Keldysh nonequilibrium Green function and equation-of-motion technique, this paper investigates the spin-polarized transport properties of the T-shaped double quantum dots (DQD) coupled to two ferromagnetic leads. There are both Fano effect and Kondo effect in the system, and due to their mutual interaction, the density of states, the current, and the differential conductance of the system depend sensitively on the spin-polarized strength. Thus the obtained results show that this system is provided with excellent spin filtering property, which indicates that this system may be a candidate for spin valve transistors in the spintronics. 相似文献
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Using an equation-of-motion technique, we theoretically study the
Fano--Kondo effect in the T-shaped double quantum dots coupled to
two ferromagnetic leads by the Anderson Hamiltonian. We calculate
the density of states in this system with both parallel and
antiparallel lead-polarization alignments, and our results reveal
that the interdot coupling, the spin-polarized strength and the
energy level of the side coupled quantum dot greatly influence the
density of states of the central quantum dot. This system is a
possible candidate for spin valve transistors and may have potential
applications in the spintronics. 相似文献
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Hybridization Induced Competitive Scanning Tunneling Interference Process into a Heavy Fermion System 下载免费PDF全文
We theoretically present the results for a scanning interference tunneling process between a metallic tip and a heavy fermion system. The density of states(DOS) and the differential conductance at zero temperature under different c-f band hybridizations, as well as the interference Fano ratio strength in the heavy fermion system,are calculated. It is found that the hybridization strength gives rise to the splitting effect in the DOS around the Fermi energy. Also the interference Fano ratio strength makes the differential conductance characteristics strongly asymmetric. 相似文献
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We consider a single-level quantum dot(QD)and a topological superconducting wire hosting Majorana bound states at its ends.By the equation of motion method,we give the analytical Green’s function of the QD in the noninteracting and the infinite interacting case.We study the effects of QD energy level and the spin polarization on the density of states(DOS)and linear conductance of the system.In the noninteracting case,the DOS resonance shifts with the change of energy level and it shows bimodal structure at large spin polarization strength.In the infinite interacting case,the up-spin linear conductance first increases and then decreases with the increase of spin polarization strength,but the down-spin is stable.However,the DOS shows a splitting phenomenon in the large energy level with the increase of spin polarization strength.This provides an interesting way to explore the physical properties of such spin dependent effect in the hybrid Majorana QD systems. 相似文献
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采用密度泛函理论和非平衡格林函数相结合的方法对Au(100)-Si-Au(100) 系统左侧对顶位、右侧对空位的纳米结点的电子输运性质进行了理论模拟计算, 结果得到纳米结点的电导随电极距离(dz)增大而减小. 在dz =9.72 Å时, 结点的结合能最低, 结构最稳定, 此时电导为1.227G0 (G0=2e2/h), 其电子输运通道主要是Si原子的px, py和 pz轨道电子形成的最高占居轨道共振峰; 在外偏压下, 电流-电压曲线表现出线性特征; 随着外加正负电压的增大, 电导略有减小, 且表现出不对称性的变化.
关键词:
硅原子
电子输运
密度泛函理论
非平衡格林函数 相似文献
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