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1.
Philip B. Lukins 《Chemical physics letters》1991,180(6):551-555
Measurements of the magneto-optical Cotton—Mouton effect at 632.8 nm of O2(3Σ) over a range of temperature (≈299–464 K) and pressure (up to 613 kPa) are reported and analysed. The study enables a useful comparison to be made of data obtained under different conditions by the two groups that have undertaken systematic measurements of this effect. Agreement between the experimental results and also the derived molecular properties is found to be satisfactory. 相似文献
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Philip A. Wheeler Michael Brungs Graham R. Atkins 《Journal of Sol-Gel Science and Technology》2003,27(3):321-326
Organically modified silicates (ormosils) have been viewed as possible materials for optical signal processing devices for communications networks. One significant problem obstructing their use in this application is the absorption of infrared light by hydroxy species (present for example in silanol groups (SiOH) and water) around the communications wavelengths (1310 and 1550 nm). We have investigated several ormosil compositions, synthesised via an aqueous sol-gel method, to determine if residual hydroxy groups can be removed more effectively via reducing the connectivity of the material by increasing the number of organic groups (such as Si—CH3). Furthermore, we have investigated the effect of different inert atmospheres on the drying process. It was found that reducing the connectivity does promote the removal of hydroxy absorption, mainly via the condensation of residual silanol groups, but also by removal of residual water, depending on the other precursors in the system. It was also found that the drying atmosphere used (nitrogen or helium) had no effect on the drying process. 相似文献
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A series of optically active main chain polyesters were synthesized by high temperature polycondensation from biphenolic azo chromophores with azobenzene-4,4'-dicarbonylchloride and 1,4:3,6-dianhydro-D-sorbitol ([!]D25=+42.5°). The second harmonic generation of the polyesters is studied in thin films. The polar order in films is determined from the UV-visible absorption spectra. The variation in SHG intensity with chiral monomer concentration is explained as a function of polar order. The polymers with chiral units showed good second harmonic efficiency. The intensity of second harmonic light (532 nm) increased with angle of incidence and indicated the polar order in the plane of the film. The SH signal also showed good temporal stability. 相似文献
7.
Philip Sternberg 《Journal of Combinatorial Theory, Series A》2007,114(5):809-824
Let g be a Lie algebra all of whose regular subalgebras of rank 2 are type A1×A1, A2, or C2, and let B be a crystal graph corresponding to a representation of g. We explicitly describe the local structure of B, confirming a conjecture of Stembridge. 相似文献
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A new consistency measure, the harmonic consistency index, is obtained for any positive reciprocal matrix in the analytic hierarchy process. We show how this index varies with changes in any matrix element. A tight upper bound is provided for this new consistency measure when the entries of matrix are at most 9, as is often recommended. Using simulation, the harmonic consistency index is shown to give numerical values similar to the standard consistency index but it is easier to compute and interpret. In addition, new properties of the column sums of reciprocal matrices are obtained. 相似文献
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Consider a semigroup generated by matrices associated with an edge-coloring of a strongly connected, aperiodic digraph. We
call the semigroup Lie-solvable if the Lie algebra generated by its elements is solvable. We show that if the semigroup is
Lie-solvable then its kernel is a right group. Next, we study the Lie algebra generated by the kernel. Lie algebras generated
by two idempotents are analyzed in detail. We find that these have homomorphic images that are generalized quaternion algebras.
We show that if the kernel is not a direct product, then the Lie algebra generated by the kernel is not solvable by describing
the structure of these algebras. Finally, we discuss an infinite class of examples that are shown to always produce strongly
connected aperiodic digraphs having kernels that are not right groups. 相似文献