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1.
M. L. Bonardi C. Birattari F. Groppi L. Gini H. S. C. Mainardi 《Journal of Radioanalytical and Nuclear Chemistry》2004,259(3):415-419
Radionuclides of very high specific activity A
S(t) have great relevance for applications in the life sciences. Updated definitions of A
S are given. The real A
S(t) must be measured by analytical and radioanalytical techniques. No-carrier-added (NCA) radionuclides have A
S(NCA) sometimes close to the carrier-free (CF) value A
S(CF). The accurate knowledge of excitation functions of nuclear reactions vs. ion beam energy is mandatory to maximize A
S(NCA); the minimization of isotopic dilution factor IDF(t) has been achieved too. A range of accelerator production and radioanalytical QC methods for A
S(NCA) optimization and determination is presented.
This revised version was published online in August 2006 with corrections to the Cover Date. 相似文献
2.
Bonardi M Birattari C Groppi F Gini L Ghioni A Mainardi HS Arginelli D Gallorini M Rizzio E Sabbioni E 《Annali di chimica》2003,93(4):363-372
In this paper are presented the production methods for very "high specific activity" radionuclides (HSA-RN) of vanadium, manganese and thallium which have been developed in our laboratories for labelling different chemical forms of these elements present in the echo-systems in ultra-trace amounts, for metallo-toxicological and bio-kinetic studies. Use was made of both cyclotron and thermal nuclear reactor. If the nuclear reaction product has atomic number different from irradiated target, it is possible separating the radioactive nuclide from irradiated target, without addition of isotopic carrier. This kind of radionuclide is named No Carrier Added, NCA, and his specific activity, As is very high and can reach values close to the theoretical Carrier Free one, CF. The experimental determination of specific activity, chemical and radiochemical purities is mandatory for all these kinds of applications. 相似文献
3.
Summary In the present paper we develop a systematic analysis of the dispersion and dissipation effects on internal gravity waves
in fluids of geophysical interest. Dissipation induces a cut-off in the short wavelengths, leading to an admissible range
of waves. Defining a suitable criterion for detection of waves, an observable wave range results, in which the frequency dispersion
is nearly the same as for the inviscid case, whereas the amplitude is damped. The peculiar behaviour displayed by the dispersion
relationship for Prandtl number equal to one is discussed. 相似文献
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7.
The fundamental solution of the fractional diffusion equation of distributed order in time (usually adopted for modelling sub-diffusion processes) is obtained based on its Mellin–Barnes integral representation. Such solution is proved to be related via a Laplace-type integral to the Fox–Wright functions. A series expansion is also provided in order to point out the distribution of time-scales related to the distribution of the fractional orders. The results of the time fractional diffusion equation of a single order are also recalled and then re-obtained from the general theory. 相似文献
8.
A method based on rational approximations is presented to interpolate the data from sinusoidal experiments in linear viscoelasticity. Bounds to the corresponding dynamical function and a discrete approximation to the spectrum are established. From this approximation the related viscoelastic functions can be computed. The method is checked by considering two theoretical models of physical interest and a satisfactory accuracy is achieved. 相似文献
9.
In this paper we investigate a general class of linear viscoelastic models whose creep and relaxation memory functions are expressed in Laplace domain by suitable ratios of modified Bessel functions of contiguous order. In time domain these functions are shown to be expressed by Dirichlet series (that is infinite Prony series). It follows that the corresponding creep compliance and relaxation modulus turn out to be characterized by infinite discrete spectra of retardation and relaxation time respectively. As a matter of fact, we get a class of viscoelastic models depending on a real parameter \(\nu > -1\). Such models exhibit rheological properties akin to those of a fractional Maxwell model (of order 1/2) for short times and of a standard Maxwell model for long times. 相似文献
10.
M. L. Bonardi F. Groppi C. Birattari L. Gini C. Mainardi A. Ghioni E. Menapace K. Abbas U. Holzwarth M. F. Stroosnijder 《Journal of Radioanalytical and Nuclear Chemistry》2003,257(1):229-241
Copper-64 is a radionuclide suitable for labeling of a wide range of radiopharmaceuticals for PET imaging, as well as systemic or local radioimmunotherapy of tumors. Among the possible methods for cyclotron production of No Carrier Added (NCA) 64Cu (61Cu), we investigated the deuteron irradiation on natural Zn target, via (d,axn) and (d,2pxn) nuclear reactions. This paper reports the preliminary results about the experimental determination and theoretical calculation of thin-target excitation functions in the energy range up to 19 MeV for 61Cu, 64Cu, 66Ga, 67Ga, 65Zn and 69mZn. A fast selective radiochemical separation of NCA 64Cu from Zn target and Ga radionuclides, with quality control tests is described too. 相似文献