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1.
2.
Langford NK Dalton RB Harvey MD O'Brien JL Pryde GJ Gilchrist A Bartlett SD White AG 《Physical review letters》2004,93(5):053601
We produce and holographically measure entangled qudits encoded in transverse spatial modes of single photons. With the novel use of a quantum state tomography method that only requires two-state superpositions, we achieve the most complete characterization of entangled qutrits to date. Ideally, entangled qutrits provide better security than qubits in quantum bit commitment: we model the sensitivity of this to mixture and show experimentally and theoretically that qutrits with even a small amount of decoherence cannot offer increased security over qubits. 相似文献
3.
Gilchrist ML Monde K Tomita Y Iwashita T Nakanishi K McDermott AE 《Journal of magnetic resonance (San Diego, Calif. : 1997)》2001,152(1):1-6
(19)F homonuclear dipolar recoupling methods were used to measure internuclear distances ranging from 5 to 12 A in fluorinated organic compounds in the solid state. Magic-angle-spinning-based high-resolution techniques were utilized. Trifluoromethyl and aromatic fluorine groups were separated by rigid aromatic spacers; these compounds were diluted into nonfluorinated host molecule matrices to give isolated homonuclear spin pairs with known internuclear distances. Radiofrequency-driven recoupling (RFDR) was used to elicit magnetization exchange between the spin pairs in 1D and 2D experiments. Simulation of the exchange was accomplished using a Monte Carlo-type algorithm to search the parameter space. These methods allow the determination of distances with an accuracy of 1 A at shorter distances and 2 A at longer distances, with the assumption of no prior knowledge of T(2)(ZQ). 相似文献
4.
Horizontal turbulent water vapour (steam) jets were discharged into ambient air from a circular convergent nozzle under unchoked/choked
and saturated/superheated nozzle exit conditions, resulting in two-phase (liquid and vapour), two-fluid (air and water) condensing
free jets. Flow properties and mixing characteristics have been measured with the aid of an isokinetic sampling probe arrangement.
Radial and axial profiles of air and steam mass flow rates and mass fractions were measured from which entrainment, centreline
decay and half-width spreading rates were calculated and compared with data from the literature. Overall, the mixing characteristics
of the condensing jets are very similar to those of non-condensing jets extensively reported in the literature.
Received: 30 September 1996 / Accepted: 19 May 1997 相似文献
5.
Jelver A. Sierra Katherine Gilchrist Jorge H. Tabares-Guevara Liliana Betancur-Galvis Jose R. Ramirez-Pineda Miguel A. Gonzlez-Cardenete 《Molecules (Basel, Switzerland)》2022,27(19)
Abietic acid (AA), dehydroabietic acid (DHA) and triptoquinones (TQs) are bioactive abietane-type diterpenoids, which are present in many edible vegetables and medicinal herbs with health-promoting properties. Evidence suggests that beneficial effects of diterpenes operate, at least in part, through effects on cells in the immune system. Dendritic cells (DCs) are a key type of leukocyte involved in the initiation and regulation of the immune/inflammatory response and natural or synthetic compounds that modulate DC functions could be potential anti-inflammatory/immunomodulatory agents. Herein, we report the screening of 23 known semisynthetic AA and DHA derivatives, and TQs, synthesized previously by us, in a multi-analyte DC-based assay that detects inhibition of pro-inflammatory cytokine production. Based on the magnitude of the inhibitory effect observed and the number of cytokines inhibited, a variety of activities among compounds were observed, ranging from inactive/weak to very potent inhibitors. Structurally, either alcohol or methyl ester substituents on ring A along with the introduction of aromaticity and oxidation in ring C in the abietane skeleton were found in compounds with higher inhibitory properties. Two DHA derivatives and two TQs exhibited a significant inhibition in all pro-inflammatory cytokines tested and were further investigated. The results confirmed their ability to inhibit, dose dependently, LPS-stimulated expression of the co-stimulatory molecules CD40 and/or CD86 and the production of the pro-inflammatory cytokines IL-1β, IL-6, IL-12 and TNFα. Our results demonstrate that DC maturation process can be targeted by semisynthetic DHA derivatives and TQ epimers and indicate the potential of these compounds as optimizable anti-inflammatory/immunomodulatory agents. 相似文献
6.
G. P. Baxter W. M. MacNevin O. Hönigschmid R. Sachtleben V. Chlopin Frau Pasvik-Chlopin C. R. Johnson W. E. Shaefer M. J. Dorcas E. W. Scripture Jr L. D. Fritzell W. Kapfenberger C. M. Alter K. Wintersberger H. Baudrexler J. S. Thomas R. Gilchrist R. Schlee A. v. Grosse M. Woodhead R. Whytlaw-Gray E. Moles M. T. Salazar A. H. Hale F. G. Nuñez R. Lautié und O. Hahn 《Fresenius' Journal of Analytical Chemistry》1936,105(5-6):205-212
Ohne Zusammenfassung 相似文献
7.
R. Gilchrist und E. Wichers 《Fresenius' Journal of Analytical Chemistry》1937,109(3-4):123-126
Ohne Zusammenfassung 相似文献
8.
R. Gilchrist H. St. C. Deville und J. S. Stas 《Fresenius' Journal of Analytical Chemistry》1930,82(8-9):321-322
Ohne Zusammenfassung 相似文献
9.
The azoalkenes (1) have been prepared from the corresponding hydrazones of dichloroacetalhyde; they react with 1,3-dicarbonyl compounds to give first the addition-elimination products (4) and then pyrroles (6). 相似文献
10.
An infra-red reflectance microscope accessory and several of its analytical applications including Chromatographic fractions and in-situ thin films are described. 相似文献