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1.
Novel mixed valence states have been obtained by the treatment of cobaltous ferrocyanides (Co+2FeII) and ferricyanides (Co+2FeIII) in an ozone flow. The CN stretching bands occur at 2085 cm–1 for Co+2FeII and at 2160 cm–1 for Co+2FeIII. After the ozonization process of Co+2FeII, an intense band approximately at 2125 cm–1 is detected. This intermediate band must correspond to a mixed valence state of the type: FeII–CN–Co2+–NC–FeIII Mössbauer spectra recorded in situ during the ozonization of Co+2FeII show the presence of two components: a doublet with isomer shift and quadrupole splitting values close to the cobalti ferricyanide and a very broad line for the mixed valence state. From the Mössbauer and infrared spectra of the aged samples of the Co+2FeII after ozonization, a relaxation process to the initial state of the samples is observed but the mixed valence state is stable. 相似文献
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Hearing talkers produce shorter vowel and word durations in multisyllabic contexts than in monosyllabic contexts. This investigation determined whether a similar effect occurs for deaf talkers, a population often characterized as lacking coarticulation in their speech. Four prelingually deafened adults and two hearing controls produced three sets of word sequences. Each set included a kernel word and six derived forms (e.g., "speed," "speedy," "speeding," etc.). The derived forms were created by adding unstressed and stressed syllables to the kernel form. A spectrographic analysis indicated that the deaf subjects did not always decrease word and vowel durations for the derivatives. Unlike hearing speakers, they often did not reduce vowel segments more than consonant segments. Three explanations are forwarded for the shortening effects. One relates to the implementation of temporal rules, the second concerns the organization imposed upon the articulators to produce speech, and the third suggests a language-independent vocal tract characteristic. The role of auditory information in developing the shortening effects is also considered. 相似文献
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van den Brand JF Ent R Anthony PL Arnold RG Arrington J Beise EJ Belz JE Bosted PE Bulten H Chapman MS Coulter KP Dietrich FS Epstein M Filippone BW Gao H Gearhart RA Geesaman DF Hansen J Holt RJ Jackson HE Jones CE Keppel CE Kinney ER Kuhn S Lee K Lorenzon W Lung A Makins NC Margaziotis DJ McKeown RD Milner RG Mueller B Napolitano J Nelson J O'Neill TG Papavassiliou V Petratos GG Potterveld DH Rock SE Spengos M Szalata ZM Tao LH van Bibber K Wasson DA White JL Zeidman B 《Physical review D: Particles and fields》1995,52(9):4868-4871
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Makins NC Ent R Chapman MS Hansen J Lee K Milner RG Nelson J Arnold RG Bosted PE Keppel CE Lung A Rock SE Spengos M Szalata ZM Tao LH White JL Coulter KP Geesaman DF Holt RJ Jackson HE Papavassiliou V Potterveld DH Zeidman B Arrington J Beise EJ Belz E Filippone BW Gao H Lorenzon W Mueller B McKeown RD O'Neill TG Epstein M Margaziotis DJ Napolitano J Kinney E Anthony PL van Bibber K Dietrich FS Gearhart RA Patratos GG Kuhn SE van den Brand JF Bulten H Jones CE 《Physical review letters》1994,72(13):1986-1989
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Tkaczyk S Tollefson K Tollestrup A Toyoda H Trischuk W de Troconiz JF Tseng J Turini N Ukegawa F Valls J Vejcik S Velev G Vidal R Vilar R Vologouev I Vucinic D Wagner RG Wagner RL Wahl J Wallace NB Walsh AM Wang C Wang CH Wang MJ Watanabe T Waters D 《Physical review letters》2000,84(6):1110-1115
We search for color singlet technirho and technipion production in p&pmacr; collisions at sqrt[s] = 1.8 TeV recorded with the Collider Detector at Fermilab. These exotic technimesons are present in a model of walking technicolor. The signatures studied are lepton plus two jets plus E(T) and multijet final states. No excess of events is seen in either final state. We set an upper limit on the technirho production cross section and exclude a region in the technipion mass versus technirho mass plane. 相似文献
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Toyoda H Trischuk W de Troconiz JF Tseng J Turini N Ukegawa F Vaiciulis T Valls J Vejcik S Velev G Vidal R Vilar R Volobouev I Vucinic D Wagner RG Wagner RL Wahl J Wallace NB Walsh AM Wang C Wang CH Wang MJ Watanabe T Waters D Watts T Webb R 《Physical review letters》2000,84(22):5043-5048
We report results from a study of events with a leading antiproton of beam momentum fraction 0.9057 GeV. Using the dijet events, we evaluate the diffractive structure function of the antiproton and compare it with expectations based on results obtained in diffractive deep inelastic scattering experiments at the DESY ep collider HERA. 相似文献
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Here we show that the surface of human cervical epithelial cells demonstrates substantially different fractal behavior when the cell becomes cancerous. Analyzing the adhesion maps of individual cervical cells, which were obtained using the atomic force microscopy operating in the HarmoniX mode, we found that cancerous cells demonstrate simple fractal behavior, whereas normal cells can only be approximated at best as multifractal. Tested on ~300 cells collected from 12 humans, the fractal dimensionality of cancerous cells is found to be unambiguously higher than that for normal cells. 相似文献