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X. M. Wen L. V. Dao P. Hannaford S. Mokkapati H. H. Tan C. Jagadish 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,62(1):65-70
We investigate the electron dynamics of p-type modulation doped and undoped
InGaAs/GaAs quantum dots using up-conversion photoluminescence at low
temperature and room temperature. The rise time of the p-doped sample is
significantly shorter than that of the undoped at low temperature. With
increasing to room temperature the undoped sample exhibits a decreased rise
time whilst that of the doped sample does not change. A relaxation mechanism
of electron-hole scattering is proposed in which the doped quantum dots
exhibit an enhanced and temperature independent relaxation due to excess
built-in holes in the valence band of the quantum dots. In contrast, the
rise time of the undoped quantum dots decreases significantly at room
temperature due to the large availability of holes in the ground state of
the valence band. Furthermore, modulation p-doping results in a shorter
lifetime due to the presence of excess defects. 相似文献
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Polymer encapsulation of yttrium oxysulfide phosphorescent particles via miniemulsion polymerization
Hyungsoo Kim Eric S. Daniels Shang Li Vijaya K. Mokkapati Keith Kardos 《Journal of polymer science. Part A, Polymer chemistry》2007,45(6):1038-1054
Yttrium oxysulfide upconverting phosphor particles can absorb infrared light and emit dopant‐dependent visible phosphorescence. This unique optical property has been used for particle‐based immunoassay applications. In this study, upconverting phosphor particles were encapsulated with a functionalized polymer (carboxylated polystyrene) shell layer via several approaches, which included the following: (1) the physical adsorption of the carboxylated polystyrene polymer onto the phosphor surfaces, (2) the miniemulsification of the preformed carboxylated polystyrene in a solvent in the presence of the phosphor particles and the subsequent stripping off of the solvent, and (3) the miniemulsification and miniemulsion copolymerization of styrene and methacrylic acid in the presence of the phosphor particles with hexadecane as a costabilizer in combination with a surfactant (sodium dodecyl sulfate, sodium dodecylbenzene sulfonate, or sodium dihexyl sulfosuccinate). Miniemulsion technology proved to be the most effective method for forming a functionalized polymeric nanoshell surrounding the phosphor particles. The morphology of the encapsulated phosphor particles was found to vary from symmetric core–shell (i.e., a uniform nanoshell layer with varying shell thicknesses), asymmetric core–shell, dumbbell‐like, or raspberry‐like partial encapsulation to multiparticle encapsulation. The amount of multiparticle encapsulation could be reduced by the postaddition of a surfactant, but it could not be eliminated completely. © 2006 Wiley Periodicals, Inc. J Polym Sci Part A: Polym Chem 45: 1038–1054, 2007 相似文献
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Some polishing experiments have been carried out on copper anodes in a hyperbolic cell designed by Gilmont and Walton, using orthophosphoric acid as the electrolyte. The results obtained have been compared to those obtained in similar experiments in a Hull cell. It has been found that very similar bands of different reflectivity and polishes are found to form in both the cells. These bands shift with time and a study of such displacements has been made. The results are briefly discussed. 相似文献
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In this paper, we report for the first time finite size effects on Néel temperature (T
N) of magnetoelectric BiFeO3 system. Novel wet chemical route has been developed to produce fine particles of BiFeO3 with controlled size and size distribution. Unlike other oxide systems, lattice volume contraction has been observed with
decrease in particle size. The decrease in T
N is co-related to unit cell volume contraction occurring with reduction in particle size. 相似文献
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Mokkapati VR Di Virgilio V Shen C Mollinger J Bastemeijer J Bossche A 《Lab on a chip》2011,11(16):2711-2719
Fabrication of nanochannels is drawing considerable interest due to its broad applications in nanobiotechnology (e.g. biomolecular sensing and single DNA manipulation). Nanochannels offer distinct advantages in allowing a slower translocation and multiple sensing spots along the channel, both of which improve the read-out resolution. However, implementing electrodes inside the nanochannel has rarely been demonstrated to our knowledge. The device described in this work is a Si-Glass anodically bonded Lab-on-a-Chip (LOC) device of a few millimetres in size capable of performing DNA manipulation. The LOC device structure is based on two mainstream microchannels interconnected by nanochannels. DNA, once trapped within the nanochannel, has been tracked throughout the length of the channel and the data have been recorded and analysed. 相似文献
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In continuation of our previous work,1–2 the effects of polishing time, sp. gr. of the electrolyte, addition of EDTA, electrolyte level, etc., on the position, size and shape of the variously polished bands obtained in a Hull cell have now been studied. I–V measurement when carried out showed that total cell voltage increases regularly with total cell current, thereby affording no explanation for the variously polished bands. However, with a specially designed probe electrode,3 it has been possible to study the current distribution as existing during polarisation at different points of the anode surface and thus offer some explanation for the appearance of variously polished bands which could not be interpreted earlier in terms of electrode potentials. 相似文献
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