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1.
The design of new solid-state proton-conducting materials is a great challenge for chemistry and materials science. Herein, a new anionic porphyrinylphosphonate-based MOF ( IPCE-1Ni ), which involves dimethylammonium (DMA) cations for charge compensation, is reported. As a result of its unique structure, IPCE-1Ni exhibits one of the highest value of the proton conductivity among reported proton-conducting MOF materials based on porphyrins (1.55×10−3 S cm−1 at 75 °C and 80 % relative humidity).  相似文献   
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Enhancement of spontaneous emission in a resonant Bragg quantum well (QW) structure with 60 periods of triple InAs monolayers embedded in a GaAs matrix is studied experimentally and theoretically. From measurements of the time‐resolved photoluminescence, besides the QW exciton at 1.47 eV, a specific super‐radiant (SR) emission demonstrating nonlinear properties is found. The SR mode shows a near‐quadratic dependence of intensity on excitation power, while its energy position follows the Bragg condition. It is revealed that the SR mode shows a peculiar non‐monotonic dependence of intensity on direction, with a maximum observed at approximately 40°. The enhancement in the SR emission at a specific direction is correlated well with suggested theoretical consideration of the modal Purcell factor for periodic quantum well structures.  相似文献   
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The three-band two-dimensional repulsive Hubbard model in the formalism of the temperature Green function is investigated. The applicability of the weak coupling approach at the values of the dimensionless coupling constant U/t≈10–11 is justified. The normal state, the antiferromagnetic state with Neel magnetic ordering on the “copper” sublattice, and the superconducting state with nontrivial Cooper pairing in channels with odd angular momenta are studied. The possibility of other magnetic states in the model is discussed. Bibliography: 20 titles. Translated fromZapiski Nauchnykh Seminarov POMI, Vol. 209, 1994, pp. 194–228. Translated by K. Malyshev.  相似文献   
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We construct a new invariant of tangle cobordisms. The invariant of a tangle is a complex of bimodules over certain rings, well-defined up to chain homotopy equivalence. The invariant of a tangle cobordism is a homomorphism between complexes of bimodules assigned to boundaries of the cobordism.

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We consider applications of disjunctive programming to global optimization and problems with equilibrium constraints. We propose a modification of the algorithm of F. Beaumont for disjunctive programming problems and show its numerical efficiency.  相似文献   
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The tape stripping technique is an experimental method frequently used for reconstruction of the in-depth distribution of various topically administered substances within the horny layer of human skin, e.g., compounds contained in sunscreens. Titanium dioxide (TiO2) nanoparticles (25–200 nm in diameter) are one such compound. Optical techniques which apply blue light are found to be suitable for reconstruction. However, the presence of particles affects the light propagation within the skin and therefore causes incorrect determination of strip thickness, leading to an improper reconstructed distribution of nanoparticle concentration revealed from the experimental data. This study evaluates the errors emerging from the use of blue (400 nm) and NIR (800 nm) radiation and finds the use of longer wavelength light more advantageous. Particles of different diameters are considered, and it is revealed that the application of small particles (25–60 nm) results in the lowest rate of error.  相似文献   
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A new approach to observing the effect of electromagnetically induced transparency in gamma optics is proposed. The propagation of a resonant photon in a 57Fe magnetic medium in an applied rf field is considered for this purpose. It is shown that, under crossing-anticrossing conditions, a resonant rf field substantially changes the gamma-optical properties of the medium, which become dependent on the parameters of the field. This opens the possibility for exercising a coherent control of the photon group velocity and a controllable filtration of unpolarized gamma radiation in a sample.  相似文献   
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