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1.
Sh. M. Khaliullin V. D. Zhuravlev V. G. Bamburov L. V. Ermakova 《Physics of Atomic Nuclei》2015,78(12):1382-1388
Submicron CaZrO3 powder is obtained in combustion reactions (solution combustion synthesis—SCS) with glycine. It is found that SCS reduces the sintering temperature of CaZrO3 powders. The dielectric properties of calcium zirconate ceramics are studied by the electrochemical impedance method. It is shown that a ceramics of powders obtained by the SCS method has high dielectric characteristics. 相似文献
2.
Raskulova T. V. Volkova L. I. Danilevich Yu. S. Shainyan B. A. Khaliullin A. K. 《Russian Journal of Organic Chemistry》2002,38(5):754-755
Russian Journal of Organic Chemistry - 相似文献
3.
Kataev V. A. Spirikhin L. V. Khaliullin A. N. Gailyunas I. A. 《Russian Journal of Organic Chemistry》2002,38(10):1507-1509
The alkylation of 2-chloro-5(6)-nitrobenzimidazole with 2-chloromethylthiirane was studied for the first time. Depending on the conditions, isomeric mixtures of nitro-substituted 2-chloro-1-(thietan-3-yl)benzimidazoles and dihydrothiazolo[3,2-a]benzimidazoles were obtained. 相似文献
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Russian Journal of Organic Chemistry - 相似文献
7.
F. A. Khaliullin Yu. V. Shabalina R. M. Sharafutdinov 《Russian Journal of Organic Chemistry》2010,46(5):689-692
The protection of the 7-NH group in 8-bromo-3-methyl-3,7-dihydro-1H-pyrine-2,6-dione during the synthesis of 7-ubsubstituted 1-alkyl-8-bromo-3-methyl-3,7-dihydro-1H-pyrine-2,6-diones with a thienyl group was applied that was introduced by the reaction with 2-chloromethylthiirane. The thietanyl
protection was removed by treating with sodium alcoholate after the oxidation with hydrogen peroxide to thietane 1,1-dioxide
group. 相似文献
8.
V. P. Drachev S. V. Perminov S. G. Rautian V. P. Safonov É. N. Khaliullin 《Journal of Experimental and Theoretical Physics》2002,94(5):901-915
A theoretical and experimental study is made into the combined manifestation of local and nonlocal optical responses in a cubic nonlinear isotropic medium such as an aggregated colloidal silver solution. The phenomenological treatment of polarization effects is performed for the general case with due regard for the frequency dispersion of both local and nonlocal nonlinearities and for the noncollinear propagation of pump and probe light waves. The inverse Faraday effect, the optical Kerr effect, and the self-rotation of the polarization ellipse in a fractal-disordered nonlinear medium are observed for the first time. The tensor components of the local and nonlocal cubic nonlinearities of colloidal silver solutions are measured for different degrees of aggregation. It is demonstrated that, as the size of silver aggregate increases, the nonlocal nonlinear response increases much more strongly than the local one. An inference is made that the mechanical motion of metal nanoparticles because of their dynamic interaction with the light wave field can contribute to the nonlinear polarization effects. 相似文献
9.
A hypothetical layered oxide La2NiMO6 where NiO2 and MO2 planes alternate along the c axis of ABO3 perovskite lattice is considered theoretically. Here, M denotes a trivalent cation Al, Ga,... such that MO2 planes are insulating and suppress the c-axis charge transfer. We predict that correlated eg electrons in the NiO2 planes develop a planar x2-y2 orbital order driven by the reduced dimensionality and further supported by epitaxial strain from the substrate. Low-energy electronic states can be mapped to a single-band t - t' - J model, suggesting favorable conditions for high-Tc superconductivity. 相似文献
10.
Molecular hydrogen is known to form stable, "nonclassical" sigma complexes with transition metal centers that are stabilized by donor-acceptor interactions and electrostatics. In this computational study, we establish that strong H2 sorption sites can be obtained in metal-organic frameworks by incorporating open transition metal sites on the organic linkers. Using density functional theory and energy decomposition analysis, we investigate the nature and characteristics of the H2 interaction with models of exposed open metal binding sites {half-sandwich piano-stool shaped complexes of the form (Arene)ML(3- n)(H2)n [M=Cr, Mo, V(-), Mn(+); Arene = C6H5X (X=H, F, Cl, OCH3, NH2, CH3, CF3) or C6H3Y2X (Y=COOH, X=CF3, Cl; L=CO; n=1-3]}. The metal-H2 bond dissociation energy of the studied complexes is calculated to be between 48 and 84 kJ/mol, based on the introduction of arene substituents, changes to the metal core, and of charge-balancing ligands. Thus, design of the binding site controls the H2 binding affinity and could be potentially used to control the magnitude of the H2 interaction energy to achieve reversible sorption characteristics at ambient conditions. Energy decomposition analysis illuminates both the possibilities and present challenges associated with rational materials design. 相似文献