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1.
Simen Gjelseth Antonsen Arne Joakim C. Bunkan Tomas Mikoviny Yngve Stenstrøm Armin Wisthaler 《Molecular physics》2020,118(15)
The kinetics of the O3, OH and NO3 radical reactions with diazomethane were studied in smog chamber experiments employing long-path FTIR and PTR-ToF-MS detection. The rate coefficients were determined to be k CH2NN+O3?=?(3.2?±?0.4)?×?10?17 and k CH2NN+OH?=?(1.68?±?0.12)?×?10?10 cm3 molecule?1 s?1 at 295?±?3?K and 1013?±?30 hPa, whereas the CH2NN?+?NO3 reaction was too fast to be determined in the static smog chamber experiments. Formaldehyde was the sole product observed in all the reactions. The experimental results are supported by CCSD(T*)-F12a/aug-cc-pVTZ//M062X/aug-cc-pVTZ calculations showing the reactions to proceed exclusively via addition to the carbon atom. The atmospheric fate of diazomethane is discussed. 相似文献
2.
Arne Miller 《Radiation Physics and Chemistry》1993,42(4-6):581-584
The activities and services of the accredited Risø High Dose Reference Laboratory are described. The laboratory operates according to the European standard EN 45001 regarding Operation of Testing Laboratories, and it fulfills the requirements of being able to deliver traceable dose measurements for control of radiation sterilization. The accredited services include:
1. 1. Irradiation of dosimeters and test samples with cobalt-60 gamma rays.
2. 2. Irradiation of dosimeters and test samples with 10 MeV electrons.
3. 3. Issue of and measurement with calibrated dosimeters.
4. 4. Measurement of the dosimetric parameters of an irradiation facility.
5. 5. Measurement of absorbed dose distribution in irradiated products.
The paper describes these services and the procedures necessary for their execution. 相似文献
3.
Linear complexity and linear complexity profile are important characteristics of a sequence for applications in cryptography
and Monte-Carlo methods.
The nonlinear congruential method is an attractive alternative to the classical linear congruential method for pseudorandom
number generation.
Recently, a weak lower bound on the linear complexity profile of a general nonlinear congruential pseudorandom number generator
was proven by Gutierrez, Shparlinski and the first author. For most nonlinear generators a much stronger lower bound is expected.
Here, we obtain a much stronger lower bound on the linear complexity profile of nonlinear congruential pseudorandom number
generators with Dickson polynomials. 相似文献
4.
5.
6.
We establish upper and lower bounds for the metric entropy and bracketing entropy of the class of d-dimensional bounded monotonic functions under Lp norms. It is interesting to see that both the metric entropy and bracketing entropy have different behaviors for p<d/(d-1) and p>d/(d-1). We apply the new bounds for bracketing entropy to establish a global rate of convergence of the MLE of a d-dimensional monotone density. 相似文献
7.
Jon Wilkening 《Linear algebra and its applications》2007,427(1):6-25
We present an efficient algorithm for obtaining a canonical system of Jordan chains for an n × n regular analytic matrix function A(λ) that is singular at the origin. For any analytic vector function b(λ), we show that each term in the Laurent expansion of A(λ)−1b(λ) may be obtained from the previous terms by solving an (n + d) × (n+d) linear system, where d is the order of the zero of det A(λ) at λ = 0. The matrix representing this linear system contains A(0) as a principal submatrix, which can be useful if A(0) is sparse. The last several iterations can be eliminated if left Jordan chains are computed in addition to right Jordan chains. The performance of the algorithm in floating point and exact (rational) arithmetic is reported for several test cases. The method is shown to be forward stable in floating point arithmetic. 相似文献
8.
Arne Barinka Stephan Dahlke Wolfgang Dahmen 《Advances in Computational Mathematics》2006,24(1-4):5-34
Recently adaptive wavelet methods have been developed which can be shown to exhibit an asymptotically optimal accuracy/work
balance for a wide class of variational problems including classical elliptic boundary value problems, boundary integral equations
as well as certain classes of noncoercive problems such as saddle point problems. A core ingredient of these schemes is the
approximate application of the involved operators in standard wavelet representation. Optimal computational complexity could
be shown under the assumption that the entries in properly compressed standard representations are known or computable in
average at unit cost. In this paper we propose concrete computational strategies and show under which circumstances this assumption
is justified in the context of elliptic boundary value problems.
Dedicated to Charles A. Micchelli on the occasion of his 60th birthday
Mathematics subject classifications (2000) 41A25, 41A46, 65F99, 65N12, 65N55.
This work has been supported in part by the Deutsche Forschungsgemeinschaft SFB 401, the first and third author are supported
in part by the European Community's Human Potential Programme under contract HPRN-CT-202-00286 (BREAKING COMPLEXITY). The
second author acknowledges the financial support provided through the European Union's Human Potential Programme, under contract
HPRN-CT-2002-00285 (HASSIP) and through DFG grant DA 360/4–1. 相似文献
9.
Ronald H. Nickel Igor Mikolic-Torreira Jon W. Tolle 《Computational Optimization and Applications》2006,35(1):109-126
Deployed US Navy aircraft carriers must stock a large number of spare parts to support the various types of aircraft embarked
on the ship. The sparing policy determines the spares that will be stocked on the ship to keep the embarked aircraft ready
to fly. Given a fleet of ten or more aircraft carriers and a cost of approximately 50 million dollars per carrier plus the
cost of spares maintained in warehouses in the United States, the sparing problem constitutes a significant portion of the
Navy’s resources. The objective of this work is to find a minimum-cost sparing policy that meets the readiness requirements
of the embarked aircraft. This is a very large, nonlinear, integer optimization problem. The cost function is piecewise linear
and convex while the constraint mapping is highly nonlinear. The distinguishing characteristics of this problem from an optimization
viewpoint are that a large number of decision variables are required to be integer and that the nonlinear constraint functions
are essentially “black box” functions; that is, they are very difficult (and expensive) to evaluate and their derivatives
are not available. Moreover, they are not convex. Integer programming problems with a large number of variables are difficult
to solve in general and most successful approaches to solving nonlinear integer problems have involved linear approximation
and relaxation techniques that, because of the complexity of the constraint functions, are inappropriate for attacking this
problem. We instead employ a pattern search method to each iteration of an interior point-type algorithm to solve the relaxed
version of the problem. From the solution found by the pattern search on each interior point iteration, we begin another pattern
search on the integer lattice to find a good integer solution. The best integer solution found across all interations is returned
as the optimal solution. The pattern searches are distributed across a local area network of non-dedicated, heterogeneous
computers in an office environment, thus, drastically reducing the time required to find the solution. 相似文献
10.
Richard P. Fischer Arne W. Fliflet 《International Journal of Infrared and Millimeter Waves》2002,23(9):1297-1313
This paper presents the design and test of asymmetric quasioptical resonators for gyrotron applications, where most of the diffraction output coupling comes from the smaller of two mirrors. A computer code based on scalar diffraction theory is used to calculate the resonator losses and the electric field near the mirrors. Resonators with mirror separations approaching confocal have reduced side lobes in the diffraction patterns, which should allow for better power transmission and focusing. Cold tests have been performed at 94 and 141 GHz to measure the quality factor of the asymmetric resonators as a function of mirror separation and mirror misalignment. Typical resonator parameters include 65 cm mirror separation, 1-3% output coupling and 85% of the losses from the small mirror. A half-symmetric resonator with one flat and one curved mirror has also been investigated. The calculated values of Q are in reasonably good agreement with the cold test measurements. 相似文献