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1.
Lithium Insertion Mechanism in Iron-Based Oxyfluorides with Anionic Vacancies Probed by PDF Analysis
Dr. Damien Dambournet Dr. Karena W Chapman Dr. Mathieu Duttine Dr. Olaf Borkiewicz Dr. Peter J Chupas Dr. Henri Groult 《ChemistryOpen》2015,4(4):443-447
The mechanism of lithium insertion that occurs in an iron oxyfluoride sample with a hexagonal–tungsten–bronze (HTB)-type structure was investigated by the pair distribution function. This study reveals that upon lithiation, the HTB framework collapses to yield disordered rutile and rock salt phases followed by a conversion reaction of the fluoride phase toward lithium fluoride and nanometer-sized metallic iron. The occurrence of anionic vacancies in the pristine framework was shown to strongly impact the electrochemical activity, that is, the reversible capacity scales with the content of anionic vacancies. Similar to FeOF-type electrodes, upon de-lithiation, a disordered rutile phase forms, showing that the anionic chemistry dictates the atomic arrangement of the re-oxidized phase. Finally, it was shown that the nanoscaling and structural rearrangement induced by the conversion reaction allow the in situ formation of new electrode materials with enhanced electrochemical properties. 相似文献
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J. Łukasik G. Auger M. L. Begemann-Blaich N. Bellaize R. Bittiger F. Bocage B. Borderie R. Bougault B. Bouriquet J. L. Charvet A. Chbihi R. Dayras D. Durand J. D. Frankland E. Galichet D. Gourio D. Guinet S. Hudan P. Lautesse F. Lavaud A. Le Fèvre R. Legrain O. Lopez U. Lynen W. F. J. Müller L. Nalpas H. Orth E. Plagnol E. Rosato A. Saija C. Schwarz C. Sfienti B. Tamain W. Trautmann A. Trzciński K. Turzó E. Vient M. Vigilante C. Volant B. Zwiegliński 《Acta Physica Hungarica A》2006,25(2-4):229-239
Directed and elliptic flow for the 197Au+197Au system at incident energies between 40 and 150 MeV per nucleon has been measured using the INDRA 4π multi-detector. For semi-central collisions, the excitation function of elliptic flow shows a transition from in-plane to out-of-plane emission at around 100 MeV per nucleon. The directed flow changes sign at a bombarding energy between 50 and 60 MeV per nucleon and remains negative at lower energies. Molecular dynamics calculations (CHIMERA) indicate sensitivity of the global squeeze-out transition on the σ NN and demonstrate the importance of angular momentum conservation in transport codes at low energies. 相似文献
4.
E. Liénard G. Ban J. Blieck D. Durand F. Duval X. Fléchard M. Herbane M. Labalme Y. Lemière F. Mauger A. Méry O. Naviliat-Cuncic D. Rodríguez J. C. Thomas 《Hyperfine Interactions》2006,172(1-3):29-33
We report on the status of the LPCTrap experiment, devoted to measure the β–ν angular correlation in the pure Gamow–Teller
decay of 6He. This measurement is motivated by the search for the presence of tensor type contributions to the weak interaction. The
6He ions are confined in a novel transparent Paul trap. The β particles and the recoil ions are detected in coincidence to
deduce the angular correlation parameter. The commissioning run performed in 2005 has given the proof of principle of this
experiment. Up to 105 coincidences were recorded during a second run in 2006. 相似文献
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Durand William A.Pham Ngoc Dinh 《Journal of Mathematical Analysis and Applications》2003,282(1):95-106
An electromagnetic diffraction problem in a wedge shaped region is reduced to a system of coupled functional difference equations by means of Sommerfeld integrals and Malyuzhinets theorem. By introducing an integral operator it is shown that the solutions of this system of functional equations can be defined in terms of integral representations whose kernels are solutions of a singular integral equation of Cauchy-Carleman type for which an explicit solution is given. 相似文献
7.
Labour scheduling plays an important and critical role in Sainsburys day to day operations and profitability. The integrated
workforce management solution for Sainsburys is an intelligent solution for the operational deployment of human resources,
integrated business forecasting, generation and calculation of workload and staff scheduling. The workforce management technology
has provided Sainsburys with a fully web-based and centralised system that produces optimised schedules for all employees
satisfying the forecasted demand of work with granularity of fifteen minutes. The system is configured to respect all operational
and business requirements as well as employee contractual constraints. This paper introduces the workforce management solution
system designed, developed and implemented for Sainsburys. We concentrate on two modelling structures, namely the work pattern
model and optimisation model, and briefly discuss the optimisation process. 相似文献
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B. Tatischeff M. P. Comets Y. Le Bornec N. Willis B. Bonin J. C. Lugol B. Mayer Y. Terrien R. Beurtey A. Boudard J. M. Durand P. Fassnacht F. Hibou 《Zeitschrift für Physik A Hadrons and Nuclei》1987,328(2):147-149
Some evidence is presented for a narrow peak at 1969±2 MeV (FWHM=9±2 MeV) in the missing mass spectrum of the3He(p, d) reaction, with 3 standard deviations. The nature of this state, the mass of which is below the NN threshold, is discussed in connection with structures found in other experiments. 相似文献
10.