We present an experimental and theoretical study of phase-dependent interference effects in multi-photon excitation under bichromatic radio-frequency (rf) field. Using an intense rf pulse, we study the interference between the three-photon and one-photon transition between the Zeeman sub-levels of the ground state of 87Rb that allows us to determine the carrier-envelope phase of the fields even for long pulses. 相似文献
The comparative measurements of helium isotope compositions between marine polymetallic nodules and their surrounding sediments, their magnetic fractions and bulk from C-C Zone of the East Pacific Basin are reported. The4He content and3He/4He ratio of polymetallic nodules and their surrounding sediments are extremely high; the3He,4 He concentrations and most3He/4He ratios of magnetic fractions in nodules and sediments are apparently higher than those in bulk. The helium isotope data points of nodules and sediments are all distributed along or closely to the mixing curve of the interplanetary dust particles (IDPs) and the terrigenous sediments in the chart of3He-3He/4He. In the same sampling site, the3He/4He ratios of nodules and their surrounding sediments are very similar, and the changes of both ratios are synchronous. It shows that the high3He/4He ratios in nodules and sediments may all result from IDPs. So, if the flux of extraterrestrial3He into the nodules and sediments is constant, the growth rate of polymetallic nodules and the sedimentation rate of sediments can be independently calculated according to the concentra-tion of extraterrestrial3He in nodules and sediments.
Due to the pronounced anisotropic response to circularly polarized light, chiral hybrid organic–inorganic metal halides have been regarded as promising candidates for the application in nonlinear chiroptics, especially for the second-harmonic generation circular dichroism (SHG-CD) effect. However, designing novel lead-free chiral hybrid metal halides with large anisotropy factors and high laser-induced damage thresholds (LDT) of SHG-CD remains challenging. Herein, we develop the first chiral hybrid germanium halide, (R/S-NEA)3Ge2I7⋅H2O (R/S-NGI), and systematically investigated its linear and nonlinear chiroptical properties. S-NGI and R-NGI exhibit large anisotropy factors (gSHG-CD) of 0.45 and 0.48, respectively, along with a high LDT of 38.46 GW/cm2; these anisotropy factors were the highest values among the reported lead-free chiral hybrid metal halides. Moreover, the effective second-order nonlinear optical coefficient of S-NGI could reach up to 0.86 pm/V, which was 2.9 times higher than that of commercial Y-cut quartz. Our findings facilitate a new avenue toward lead-free chiral hybrid metal halides, and their implementation in nonlinear chiroptical applications. 相似文献
We have studied the intensity correlations between two orthogonally linearly polarized components of a laser field propagating through a resonant atomic medium. These experiments have been performed in a rubidium atomic vapor. We observe that the correlations between the orthogonally polarized components of the laser beam are maximal in the absence of a magnetic field. The magnitude of the correlations depends on the applied magnetic field, and the magnitude first decreases and then increases with increasing magnetic field. Minimal correlations and maximal rotation angles are observed at the same magnetic fields. The width of the correlation function is directly proportional to the excited state lifetime and inversely proportional to the Rabi frequency of laser field. 相似文献
The comparative measurements of helium isotope compositions between marine poly-metallic nodules and their surrounding sediments, their magnetic fractions and bulk from C-C Zoneof the East Pacific Basin are reported. The ~4He content and ~3He/~4He ratio of polymetallic nodulesand their surrounding sediments are extremely high; the ~3He, ~4He concentrations and most~3He/~4He ratios of magnetic fractions in nodules and sediments are apparently higher than those inbulk. The helium isotope data points of nodules and sediments are all distributed along or closelyto the mixing curve of the interplanetary dust particles (IDPs) and the terrigenous sediments in thechart of ~3He-~3He/~4He. In the same sampling site, the ~3He/~4He ratios of nodules and their surround-ing sediments are very similar, and the changes of both ratios are synchronous. It shows that thehigh ~3He/~4He ratios in nodules and sediments may all result from IDPs. So, if the flux of extrater-restrial ~3He into the nodules and sediments is constant, the growth rate of polymetallic nodules andthe sedimentation rate of sediments can be independently calculated according to the concentra-tion of extraterrestrial ~3He in nodules and sediments. 相似文献
We study the selective reflection of the laser beam from rubidium atomic vapor at the D2 line (wavelength λ = 780 nm) at different atomic densities. We use a tunable free-running diode laser. We observed a measurable signal at a
low atomic density N when the mean distance between resonance atoms reached two wavelengths. In our experiment, the dimensionless parameter N1/3λ varied from 0.5 to 2.8. The reflectivity increased with density monotonically. It is interesting to perform experiments when
the parameter N1/3λ ≪ 1. 相似文献