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1.
Simen Gjelseth Antonsen Arne Joakim C. Bunkan Tomas Mikoviny Yngve Stenstrøm Armin Wisthaler 《Molecular physics》2020,118(15)
The kinetics of the O3, OH and NO3 radical reactions with diazomethane were studied in smog chamber experiments employing long-path FTIR and PTR-ToF-MS detection. The rate coefficients were determined to be k CH2NN+O3?=?(3.2?±?0.4)?×?10?17 and k CH2NN+OH?=?(1.68?±?0.12)?×?10?10 cm3 molecule?1 s?1 at 295?±?3?K and 1013?±?30 hPa, whereas the CH2NN?+?NO3 reaction was too fast to be determined in the static smog chamber experiments. Formaldehyde was the sole product observed in all the reactions. The experimental results are supported by CCSD(T*)-F12a/aug-cc-pVTZ//M062X/aug-cc-pVTZ calculations showing the reactions to proceed exclusively via addition to the carbon atom. The atmospheric fate of diazomethane is discussed. 相似文献
2.
3.
Arne Barinka Stephan Dahlke Wolfgang Dahmen 《Advances in Computational Mathematics》2006,24(1-4):5-34
Recently adaptive wavelet methods have been developed which can be shown to exhibit an asymptotically optimal accuracy/work
balance for a wide class of variational problems including classical elliptic boundary value problems, boundary integral equations
as well as certain classes of noncoercive problems such as saddle point problems. A core ingredient of these schemes is the
approximate application of the involved operators in standard wavelet representation. Optimal computational complexity could
be shown under the assumption that the entries in properly compressed standard representations are known or computable in
average at unit cost. In this paper we propose concrete computational strategies and show under which circumstances this assumption
is justified in the context of elliptic boundary value problems.
Dedicated to Charles A. Micchelli on the occasion of his 60th birthday
Mathematics subject classifications (2000) 41A25, 41A46, 65F99, 65N12, 65N55.
This work has been supported in part by the Deutsche Forschungsgemeinschaft SFB 401, the first and third author are supported
in part by the European Community's Human Potential Programme under contract HPRN-CT-202-00286 (BREAKING COMPLEXITY). The
second author acknowledges the financial support provided through the European Union's Human Potential Programme, under contract
HPRN-CT-2002-00285 (HASSIP) and through DFG grant DA 360/4–1. 相似文献
4.
Richard P. Fischer Arne W. Fliflet 《International Journal of Infrared and Millimeter Waves》2002,23(9):1297-1313
This paper presents the design and test of asymmetric quasioptical resonators for gyrotron applications, where most of the diffraction output coupling comes from the smaller of two mirrors. A computer code based on scalar diffraction theory is used to calculate the resonator losses and the electric field near the mirrors. Resonators with mirror separations approaching confocal have reduced side lobes in the diffraction patterns, which should allow for better power transmission and focusing. Cold tests have been performed at 94 and 141 GHz to measure the quality factor of the asymmetric resonators as a function of mirror separation and mirror misalignment. Typical resonator parameters include 65 cm mirror separation, 1-3% output coupling and 85% of the losses from the small mirror. A half-symmetric resonator with one flat and one curved mirror has also been investigated. The calculated values of Q are in reasonably good agreement with the cold test measurements. 相似文献
5.
Arne Schirrmacher 《Physics in Perspective (PIP)》2003,5(1):4-20
David Hilbert (1862-1943) played an important role in establishing quantum physics in Göttingen. I analyze the ways in which his influence was decisive by comparison with Woldemar Voigt (1850-1919). Voigt was the leading Göttingen theoretical physicist before the arrival of Peter Debye (1884-1966), who was appointed to a new professorship in 1914 at Hilbert's instigation. I portray the Göttingen mathematicians, above all Hermann Minkowski (1864-1909) and David Hilbert, as planting the seeds for the blossoming of quantum physics under their student Max Born (1882-1970) in the 1920s. 相似文献
6.
7.
During irradiation of liquid samples of 1-vinylimidazole, 2-vinylnaphthalene, 2-vinylpyridine, 4-vinylpyridine and 1,1-diphenylethene
with positive muons, radicals of the type MuCH2ĊHAr (Ar=the appropriate aromatic group), and the MuCH2ĊPh2 radical were observed by transverse field μSR; the muon hyperfine couplings are considered in the context of the effectiveness
of the aryl groups in delocalising the unpaired electron. 相似文献
8.
The modified wave and scattering operators are shown to be bounded between weighted L
2-spaces for two-body Schrödinger operators with long range potentials. 相似文献
9.
Gašper Jaklič Jernej Kozak Marjeta Krajnc Vito Vitrih Emil Žagar 《Numerical Algorithms》2007,45(1-4):49-60
In this paper, three-pencil lattices on triangulations are studied. The explicit representation of a lattice, based upon barycentric
coordinates, enables us to construct lattice points in a simple and numerically stable way. Further, this representation carries
over to triangulations in a natural way. The construction is based upon group action of S
3 on triangle vertices, and it is shown that the number of degrees of freedom is equal to the number of vertices of the triangulation.
相似文献
10.
Juan Pablo Trelles Emil Pfender Joachim Heberlein 《Plasma Chemistry and Plasma Processing》2006,26(6):557-575
The dynamics of the electric arc inside a direct current non-transferred arc plasma torch are simulated using a three-dimensional, transient, equilibrium model. The fluid and electromagnetic equations are solved numerically in a fully coupled approach by a multiscale finite element method. Simulations of a torch operating with argon and argon–hydrogen under different operating conditions are presented. The model is able to predict the operation of the torch in steady and takeover modes without any further assumption on the reattachment process except for the use of an artificially high electrical conductivity near the electrodes, needed because of the equilibrium assumption. The results obtained indicate that the reattachment process in these operating modes may be driven by the movement of the arc rather than by a breakdown-like process. It is also found that, for a torch operating in these modes and using straight gas injection, the arc will tend to re-attach to the opposite side of its original attachment. This phenomenon seems to be produced by a net angular momentum on the arc due to the imbalance between magnetic and fluid drag forces. 相似文献