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This research reports the development of a biotrickling filter (BTF) to upgrade biogas, which is achieved by adding H2 to reduce CO2. H2 and CO2 (80:20% vol.) were fed to a bench-scale BTF packed with polyurethane foam (PUF) and inoculated with hydrogenotrophic methanogens. Maximum CH4 production rates recorded were as high as 38 m3 CH4 m?3 reactor day?1, which is 5–30 times faster than earlier reports with other kinds of bioreactors. The high rates were attributed to the efficient mass transfer and high density of methanogens in the BTF. The removal efficiencies for H2 and CO2 were 83 and 96%, respectively. 5-Cyano-2,3-ditolyl tetrazolium chloride/DAPI staining revealed that 67% of cells were alive near the gas entrance port, while only 8.3% were alive at the exit. Furthermore, DNA sequencing showed that only 27% of the biomass was composed of Euryarchaeota, the phylum which includes methanogens. These two observations suggest that optimizing the methanogen density and activity could possibly reach even higher biogas upgrading rates. 相似文献
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Th. v. Fellenberg R. S. Alcock M. S. Lukjanowitsch N. P. Fedorow D. N. Bidenko E. Thomae J. Deshusses O. L. Evenson J. A. Kime S. S. Forrest Gesellschaft für Linde Eismaschinen A. S. Wetrow A. M. Kogan K. M. Nassyrowa J. P. Pusstylnikowa W. A. Gluchowzewa W. R. Tschertok Bláhá Láska E. Waser S. Janett B. Hazslinszky A. K. Fitger und CI. R. Dumble 《Fresenius' Journal of Analytical Chemistry》1938,113(5-6):226-235
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Jae‐Hong Lim Nopparat Phiboolsirichit Syed Mubeen Youngwoo Rheem MarcA. Deshusses Ashok Mulchandani NosangV Myung 《Electroanalysis》2010,22(1):99-105
The electrical transport and NH3 sensing properties of randomly oriented and aligned SWNT networks were presented and discussed. The results indicate that aligned SWNT‐FETs have better FET characteristics due to the reduced number of interconnected nodes. This was particularly true as the resistance of the devices increased. Gated electrical breakdown was implemented to selectively remove metallic (m‐) SWNTs, thereby reducing scattering centers. This technique provided significant improvements in FET characteristics resulting in greater on/off ratio (e.g. 104). AC dielectrophoretic alignment followed by selective electrical breakdown of m‐SWNTs can significantly enhance the semiconducting properties of SWNT networks which resulted in highly sensitive sensors. 相似文献
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Th. Fellenberg Dorothea Herrmann Ch. Valencien J. Deshusses M. D. Florentin und Pannwitz 《Fresenius' Journal of Analytical Chemistry》1939,117(3-4):151-154
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J. Deshusses und C. Griebel 《Fresenius' Journal of Analytical Chemistry》1941,121(1-2):77-80
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McNicholas TP Zhao K Yang C Hernandez SC Mulchandani A Myung NV Deshusses MA 《The journal of physical chemistry. C, Nanomaterials and interfaces》2011,115(28):13927-13931
Low-cost, low power consumption gas sensors that can detect or quantify various gas analytes are of increasing interest for various applications ranging from mobile health, to environmental exposure assessment and homeland security. In particular miniature gas sensors based on nanomaterials that can be manufactured in the form of sensor arrays present great potential for the development of portable monitoring devices. In this study, we demonstrate that a chemiresistive nanosensor comprised of single walled carbon nanotubes decorated with gold nanoparticles has impressive sensitivity to elemental mercury (Hg) gas concentrations, with a lower detection limit as low as 2 ppb(v). Furthermore, this nanosensor was found to regenerate, though slowly, without any additional recovery steps. Finally, the mercury vapor sensing mechanism allowed for direct investigations into the origin of Surface Enhanced Raman Scattering (SERS) in carbon nanotubes decorated with Au nanoparticles. 相似文献
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A simplified microbiological assy for inositol involving the use of Schizuscicchurnmyces pombe Lindner is decscribted. The results are very reproducible and the method is simple to operate. 相似文献