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1.
With a suitable combination of ligand-stabilised nanoparticle suspension and ionic salt solutions, it is possible to produce microcrystals that are coated with nanoparticles. The self-assembly process of coating microcrystals by gold nanoparticles (NP) is mediated by the crystal lattice. This is the so-called CLAMS process - a generic process for self-organisation of nanoparticles on the surface of crystals [M. Murugeshan, D. Cunningham, J.-L. Martnez-Albertos, R. Vrcelj, B.D. Moore, Chem. Commun. (2005) 2677]. We are exploring here the structural properties of these self-assembled structures by using different imaging techniques. 相似文献
2.
In this paper a single-degree-of-freedom model is developed to predict the dynamic response of an acoustially excited doubly curved sandwich panel. Three variants of the model are investigated, based on differing assumptions regarding the spatial distribution of the applied loading. When the loading is assumed to be uniform then the model reduces to the Miles approach, and when the loading is assumed to conform to the structural mode shape then the method is very similar to the Blevins approach. The third variant involves a more detailed consideration of the travelling wave characteristics of the applied loading, and this is found to give much improved agreement with experimental results obtained in a progressive wave tube facility. In addition, an approach using the finite element method is presented in which the response to grazing incidence excitation is computed, and this is also found to yield good agreement with the experimental results. 相似文献
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NIKITIN S.; PR?TZEL-WOLTERS D. 《IMA Journal of Mathematical Control and Information》1991,8(4):431-439
In 1983 Morse proved, for unknown scalar one-dimensional linearsystems, the nonexistence of rational or polynomial universalstabilizers (UAS). In 1983, Nussbaum gave an example of an analyticUAS. In our paper, it is shown that there exist time-invariantpolynomial UAS's with multidimensional gain adaptation. Thedesign procedure is developed for linear, minimum-phase systemsof relative degree one. Convergence of the closed-loop systemis proved. Some numerical simulations are provided. 相似文献
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R. Buccellato M. M. Michaelis C. A. Dempers A. Prause P. F. Cunningham 《Optics & Laser Technology》1993,25(4)
The concept of a pulsed gas lens is proposed. Potential applications are envisaged and preliminary experiments with pulsed ray refraction are reported. 相似文献
6.
Kejian Bian Michael F. Cunningham 《Journal of polymer science. Part A, Polymer chemistry》2006,44(1):414-426
Nitroxide‐mediated radical polymerization (NMRP) of 2‐(dimethylamino)ethyl acrylate (DMAEA) was carried out at 100–120 °C, initiated by MONAMS, an alkoxyamine based on N‐tert‐butyl‐N‐(1‐diethyl phosphono‐2,2‐dimethylpropyl)nitroxide, SG1. Controlled polymerization can be achieved by the addition of free SG1 (the initial molar ratio of SG1 to MONAMS ranged from 0.06 to 0.12), giving a linear first‐order kinetic plot up to 55–70% conversion depending on the reaction conditions. The molecular weights show a near linear increase with conversion; however, they deviate to some extent with theoretical values. SG1‐mediated polymerization of DMAEA at 112 °C is also controlled in organic solvents (N,N‐dimethylformide, anisole, xylene). Polymerization rate increases with increasing solvent polarity. Chain transfer to polymer produces ~1 mol % branches in bulk and 1.2–1.9 mol % in organic solvents, typical of those for acrylates. From poly(styrene) (pS) and poly(n‐butyl acrylate) (pBA) macroinitiators, amphiphilic di‐ and triblock copolymers p(S‐b‐DMAEA), p(DMAEA‐b‐S‐b‐DMAEA), p(BA‐b‐DMAEA), and p(DMAEA‐b‐BA‐b‐DMAEA) were synthesized via NMRP at 110 °C. Polymers were characterized by GPC, NMR, surface tension measurements, and DSC. © 2005 Wiley Periodicals, Inc. J Polym Sci Part A: Polym Chem 44: 414–426, 2006 相似文献
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R. J. Smith P. J. Woods R. Chapman J. L. Durell J. N. Mo B. R. Fulton R. A. Cunningham 《Zeitschrift für Physik A Hadrons and Nuclei》1986,324(3):283-287
The ground-state masses of35Si and34Si have been measured using the reactions64Ni(36S,35,34Si)65,66Zn at a36S beam energy of 198 MeV.34,35Si14+ ions were analysed and identified in a QMG/2 magnetic spectrometer and gas-filled focal-plane detector. The experimental mass excess of35Si was determined to be ?14.58± 0.12 0.07 MeV while that of34Si was measured as ?19.961±0.034 MeV. A comparison is made with the results of mass model predictions. 相似文献