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1.
Laurens Kooijman Dr. Matthias Schuster Christian Baumann Simon Jurt Dr. Frank Löhr Dr. Boris Fürtig Prof. Dr. Peter Güntert Prof. Dr. Oliver Zerbe 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2020,132(47):21151-21158
To achieve efficient proton pumping in the light-driven proton pump bacteriorhodopsin (bR), the protein must be tightly coupled to the retinal to rapidly convert retinal isomerization into protein structural rearrangements. Methyl group dynamics of bR embedded in lipid nanodiscs were determined in the dark-adapted state, and were found to be mostly well ordered at the cytosolic side. Methyl groups in the M145A mutant of bR, which displays only 10 % residual proton pumping activity, are less well ordered, suggesting a link between side-chain dynamics on the cytosolic side of the bR cavity and proton pumping activity. In addition, slow conformational exchange, attributed to low frequency motions of aromatic rings, was indirectly observed for residues on the extracellular side of the bR cavity. This may be related to reorganization of the water network. These observations provide a detailed picture of previously undescribed equilibrium dynamics on different time scales for ground-state bR. 相似文献
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In 1976 S. Hawking claimed that “Because part of the information about the state of the system is lost down the hole, the final situation is represented by a density matrix rather than a pure quantum state”. 1 This was the starting point of the popular “black hole (BH) information paradox”. 相似文献
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Mathematische Semesterberichte - 相似文献
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A protocol to correct for intra‐ and interspecific variation in tail hair growth to align isotope signatures of segmentally cut tail hair to a common time line
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Christian Bosse 《Discrete Mathematics》2019,342(12):111595
The Hadwiger number of a graph , denoted , is the largest integer such that contains as a minor. A famous conjecture due to Hadwiger in 1943 states that for every graph , , where denotes the chromatic number of . Let denote the independence number of . A graph is -free if it does not contain the graph as an induced subgraph. In 2003, Plummer, Stiebitz and Toft proved that for all -free graphs with , where is any graph on four vertices with , , or is a particular graph on seven vertices. In 2010, Kriesell subsequently generalized the statement to include all forbidden subgraphs on five vertices with . In this note, we prove that for all -free graphs with , where denotes the wheel on six vertices. 相似文献