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1.
Laurens Kooijman Dr. Matthias Schuster Christian Baumann Simon Jurt Dr. Frank Löhr Dr. Boris Fürtig Prof. Dr. Peter Güntert Prof. Dr. Oliver Zerbe 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2020,132(47):21151-21158
To achieve efficient proton pumping in the light-driven proton pump bacteriorhodopsin (bR), the protein must be tightly coupled to the retinal to rapidly convert retinal isomerization into protein structural rearrangements. Methyl group dynamics of bR embedded in lipid nanodiscs were determined in the dark-adapted state, and were found to be mostly well ordered at the cytosolic side. Methyl groups in the M145A mutant of bR, which displays only 10 % residual proton pumping activity, are less well ordered, suggesting a link between side-chain dynamics on the cytosolic side of the bR cavity and proton pumping activity. In addition, slow conformational exchange, attributed to low frequency motions of aromatic rings, was indirectly observed for residues on the extracellular side of the bR cavity. This may be related to reorganization of the water network. These observations provide a detailed picture of previously undescribed equilibrium dynamics on different time scales for ground-state bR. 相似文献
2.
In two dimensional electron systems with Coulomb or dipolar interactions, a direct transition, whether first or second order, from a liquid to a crystalline state is forbidden. As a result, between these phases there must be other (micro-emulsion) phases which can be viewed as a meso-scale mixture of the liquid and crystalline phases. We investigate the transport properties of these new electronic phases and present arguments that they are responsible for the various transport anomalies that have been seen in experiments on the strongly correlated 2DEG in high mobility semiconductor devices with low electron densities. 相似文献
3.
Set-Valued and Variational Analysis - 相似文献
4.
Boris Goldfarb 《Topology and its Applications》2004,140(2-3):267-294
New compactifications of symmetric spaces of noncompact type X are constructed using the asymptotic geometry of the Borel–Serre enlargement. The controlled K-theory associated to these compactifications is used to prove the integral Novikov conjecture for arithmetic groups. 相似文献
5.
We study the complex Ginzburg–Landau equation with zero Neumann boundary conditions on a finite interval and establish that this boundary problem (with suitably chosen parameters) has countably many stable two-dimensional self-similar tori. The case of periodic boundary conditions is also investigated. 相似文献
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7.
Salimgareeva V. N. Polevoi R. M. Kolesov S. V. Ostakhov S. S. Ponomareva V. A. Leplyanin G. V. 《Russian Journal of Applied Chemistry》2003,76(5):804-808
The luminescence and scintillation properties of poly(methyl methacrylate) containing 1,1,3-trimethyl-3-phenylindan were studied. 相似文献
8.
9.
Letters in Mathematical Physics - 相似文献
10.
A. Yu. Kolesov E. F. Mishchenko N. Kh. Rozov 《Proceedings of the Steklov Institute of Mathematics》2007,259(1):101-127
We carry out a detailed analysis of the existence, asymptotics, and stability problems for periodic solutions that bifurcate
from the zero equilibrium state in systems with large delay. The account is based on a specific meaningful example given by
a certain scalar nonlinear second-order differential-difference equation that is a mathematical model of a single-circuit
RCL oscillator with delay in a feedback loop. 相似文献