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Journal of Radioanalytical and Nuclear Chemistry - Responses of the hand-held gamma monitors available for the ambient dose equivalent rate measurements in the Federation of Bosnia and Herzegovina...  相似文献   
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Journal of Radioanalytical and Nuclear Chemistry - This work presents measurements of activity concentrations and estimation of population exposure from the naturally occurring radionuclides 238U,...  相似文献   
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Azido 18F‐arenes are important and versatile building blocks for the radiolabeling of biomolecules via Huisgen cycloaddition (“click chemistry”) for positron emission tomography (PET). However, routine access to such clickable agents is challenged by inefficient and/or poorly defined multistep radiochemical approaches. A high‐yielding direct radiofluorination for azido 18F‐arenes was achieved through the development of an ortho‐oxygen‐stabilized iodonium derivative (OID). This OID strategy addresses an unmet need for a reliable azido 18F‐arene clickable agent for bioconjugation reactions. A ssDNA aptamer was radiolabeled with this agent and visualized in a xenograft mouse model of human colon cancer by PET, which demonstrates that this OID approach is a convenient and highly efficient way of labeling and tracking biomolecules.  相似文献   
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The knowledge of neutron energy spectra contributes to unambiguous identification of neutron sources in the fields of nuclear safeguards and nuclear non-proliferation. Since a real scenario situation includes the presence of shielding around the source, we have investigated the influence of the potential shielding surrounding the source on the shape of energy spectra for a few neutron sources. We have applied the maximum-likelihood, expectation–maximisation (MLEM) method with one-step-late (OSL) algorithm for neutron spectra unfolding. The pulse height distributions used in the unfolding procedures were simulated with the high accuracy by using the MCNP-PoliMi code based on the Monte Carlo method. A possibility to identify the shielded neutron sources by using the unfolding method was examined with two continuous-in-energy sources, such as 252Cf and 241Am–Be in source-shielding configurations with lead (Pb) and polyethylene (PE) blocks. The results of calculations have shown that the identification of 252Cf and 241Am–Be sources with 2.5 cm of Pb and PE shield can be achieved successfully by using the MLEM method with the OSL algorithm. However, the unfolded results for 252Cf and 241Am–Be sources with 10 cm of PE shield significantly deviate from the reference spectra and the sources cannot be correctly identified on the basis of their unfolded energy spectra.  相似文献   
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Journal of Radioanalytical and Nuclear Chemistry - This paper deals with the first study of the indoor to outdoor ambient dose equivalent rates ratio measured in and around the historic objects at...  相似文献   
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