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241.
运用蒙卡程序MCNPX对加速器驱动次临界反应堆系统(简称ADS)的标准散裂中子靶进行了计算研究.计算了在0.6~1.5 GeV的质子轰击下,标准Pb靶发生散裂反应产生的中子产额及分布、中子能谱以及靶内能量沉积分布.计算结果与文献理论数据、实验数据进行了比较. 相似文献
242.
为了讨论PGAI技术分析的准确性,并验证冷中子和热中子应用于PGAI技术的可行性,通过蒙特卡罗模拟计算软件对PGAI技术理想化模型进行了研究,采用高准直的冷中子及热中子束和高纯锗探测器,对一块5 cm× 5 cm×1 cm均匀铁单质样品进行了模拟计算及图像重建,选取的等效体积大小为1 cm×1 cm×1 cm。结果显示:两种能量中子可以用于PGAI技术实现元素分布测量,但无论使用何种能量中子,由于物料体效应带来的中子自屏效应、中子散射效应以及伽马射线自吸收作用,即便在对均匀单质样品进行测量时,图像重建结果也无法保证各位置元素响应的一致性。因此,在后续工作中,需理清PGAI物理机制,建立相应的修正模型。 相似文献
243.
Analysis of Forbush decreases observed using a muon telescope in Antarctica starting on 21 June 2015 下载免费PDF全文
De-Hong Huang Hong-Qiao Hu Ji-Long Zhang Hong Lu Da-Li Zhang Bin-Shen Xue Jing-Tian Lu 《中国物理C(英文版)》2018,42(12):125001-125001
A cosmic-ray muon telescope has been collecting data since the end of 2014, which was shortly after the telescope was built in the Zhongshan Station of Antarctica. The telescope is the first observation device to be built by Chinese scientists in Antarctica. The pressure change is very strong in Zhongshan station. The count rate of the pressure correction results shows that the large variations in the count rate are likely caused by pressure fluctuations. During the period from 18 June to 22 June 2015, four halo coronal mass ejections(CMEs) were ejected from the Sun. These CMEs initiated a series of Forbush decreases(FD) when they reached the Earth. We conducted a comprehensive study of the intensity fluctuations of galactic cosmic rays recorded during FDs. The intensity fluctuations used in this study were collected by cosmic ray detectors of multiple stations(Zhongshan, McMurdo,South Polar, and Nagoya), and the solar wind measurements were collected by ACE and WIND. The profile of the FD of 22 June demonstrated a four-step decrease. The traditional one-or two-step FD classification method does not adequately explain the FD profile results. The interaction between the faster CME that occurred on 21 June 2015 and the two slow CMEs of the earlier few days should be considered. The cosmic ray intensities of the South Pole,McMurdo, and Zhongshan stations have similar hourly variations, whereas the galactic cosmic rays recorded between polar and non-polar locations are distinct. The FD pre-increase of 22 June 2015 for the Nagoya muon telescope(non-polar location) lags those of the McMurdo and Zhongshan stations(polar locations) by 1 h. The FD onset of22 June 2015 for the Nagoya muon telescope lags those of the polar locations by 1 h. 相似文献
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The pre-scission neutrons measured in the reactions 16O 181Ta and 19F 178Hf are studied via a Langevin equation coupled with a statistical decay model. We find that because of the mass asymmetry of different entrance channels, the spin distributions of compound nuclei would be different, consequently, the measured neutrons in these two reactions would also different. This means that the entrance channel will affect the particle emission in the fission process of hot nuclei. 相似文献
247.
K. Kní?ek J. Hejtmánek E. Šantavá J. Buršík P. Beran 《Journal of solid state chemistry》2011,184(8):2231-2237
The layered cobaltate La0.30CoO2 was prepared from NaxCoO2 precursor by a solid-state ionic exchange and was characterized by means of X-ray and neutron diffraction, magnetic, thermal and electric transport measurements. The compound consists of hexagonal sheets of edge-sharing CoO6 octahedra interleaved by lanthanum monolayers. Compared to Na+ in the parent system, the La3+ ions occupy only one-third of available sites, forming a 2-dimensional superstructure. The deviation from the ideal stoichiometry La1/3CoO2 introduces extra hole carriers into the diamagnetic LS Co3+ matrix making the sample Pauli paramagnetic. The temperature dependence of the electrical conductivity in La0.30CoO2 follows Mott's T−1/3 law up to about 400 K, which is in contrast with the standard metallic behavior in the Na+ homolog possessing the same formal doping. The experiments are complemented by electronic structure calculations for La0.30CoO2 and related NaxCoO2 systems. 相似文献
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The determination of seven saponins in crude plant extracts by electrospray ionization mass spectrometry (ESI-MS) and fast atom bombardment mass spectrometry (FAB-MS) is described. Distinct protonated and natriated (Na-adduct) molecular ions in ESI-MS spectra readily provide molecular weight information, which can be further verified using clusters of molecular ions. Saponin mixtures can be analyzed by ESIMS on varying the potential difference between the capillary and skimmer in the ESI source to decompose impurities. ESI-MS uses less amount of sample than that required by FAB-MS. ESI-MS does not produce structural information, however. The FAB-MS spectra consist mainly of protonated and deprotonated molecular ions with limited structural information. (-)-FAB-MS is more suitable for analyzing saponin samples than the (+)-FAB-MS. 相似文献
250.
Dr. Julian J. Holstein Priv.‐Doz. Dr. Birger Dittrich Miriam Simon Dr. Sylvain Prévost Prof. Dr. Michael Gradzielski Prof. Dr. Guido H. Clever 《Angewandte Chemie (International ed. in English)》2018,57(41):13652-13656
A series of metal‐mediated cages, having multiple cavities, was synthesized from PdII cations and tris‐ or tetrakis‐monodentate bridging ligands and characterized by NMR spectroscopy, mass spectrometry, and X‐ray methods. The peanut‐shaped [Pd3L14] cage deriving from the tris‐monodentate ligand L1 could be quantitatively converted into its interpenetrated [5Cl@Pd6L18] dimer featuring a linear {[Pd‐Cl‐]5Pd} stack as an unprecedented structural motif upon addition of chloride anions. Small‐angle neutron scattering (SANS) experiments showed that the cigar‐shaped assembly with a length of 3.7 nm aggregates into mono‐layered discs of 14 nm diameter via solvophobic interactions between the hexyl sidechains. The hepta‐cationic [5Cl@Pd6L18] cage was found to interact with polyanionic oligonucleotide double‐strands under dissolution of the aggregates in water, rendering the compound class interesting for applications based on non‐covalent DNA binding. 相似文献