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171.
S. Canulescu T. Lippert A. Wokaun 《Applied Physics A: Materials Science & Processing》2008,93(3):771-778
The mass distributions of the species generated by laser ablation from a La0.6Ca0.4MnO3 target using laser irradiation wavelengths of 193 nm, 266 nm and 308 nm have been investigated with and without a synchronized
gas pulse of N2O. The kinetic energies of the species are measured using an electrostatic deflection energy analyzer, while the mass distributions
of the species were analyzed with a quadrupole mass filter.
In vacuum (pressure 10−7 mbar), the ablation plume consists of metal atoms and ions such as La, Ca, Mn, O, LaO, as well as multiatomic species, e.g.
LaMnO+. The LaO+ diatomic species are by far the most intense diatomic species in the plume, while CaO and MnO are only detected in small
amounts.
The interaction of a reactive N2O gas pulse with the ablation plume leads to an increase in plume reactivity, which is desired when thin manganite films are
grown, in order to incorporate the necessary amount of oxygen into the film. The N2O gas pulse appears to have a significant influence on the oxidation of the Mn species in the plume, and on the creation of
negative ions, such as LaO−,O− and O2−. 相似文献
172.
G. P. Gupta A. Z. Msezane 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2008,49(2):157-160
Excitation energies from ground state for 97 fine-structure levels as well as oscillator strengths and radiative decay rates
for all electric-dipole-allowed and intercombination transitions among the fine-structure levels of the terms belonging to
the (1s
22s
22p
6)3s
23p, 3s
3
p
2, 3s
23d, 3p
3, 3s3p3d, 3p
23d, 3s3d
2, 3s
24s, 3s
24p, 3s
24d, 3s
24f, and 3s3p4s configurations of Co XV are calculated, using extensive configuration-interaction (CI) wave functions, obtained with the
CIV3 computer code of Hibbert. The important relativistic effects in intermediate coupling are included through the Breit-Pauli
approximation via spin-orbit, spin-other-orbit, spin-spin, Darwin and mass correction terms. Small adjustments to the diagonal
elements of the Hamiltonian matrices have been made. Our calculated excitation energies, including their ordering, are in
excellent agreement with the experimental results and the experimentally compiled energy values of the National Institute
for Standards and Technology (NIST) wherever available. The mixing among several fine-structure levels is found to be very
strong, with most of the strongly mixed levels belonging to the (1s
22s
22p
6)3p
23d and 3s3d
2 configurations. The strong mixing among several fine-structure levels makes it very difficult to identify them uniquely.
Perhaps, that may be the reason for the lack of both experimental and theoretical results for these levels. We believe that
our extensive calculated values can guide experimentalists in identifying the fine-structure levels in their future work.
From our radiative decay rates we have also calculated radiative lifetimes of some fine-structure levels. In this calculation
we also predict new data for several fine-structure levels where no other theoretical and/or experimental results are available. 相似文献
173.
B. Sen B. Das P. Chatterjee 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2008,49(2):211-216
Nonlinear dust acoustic solitary waves in a dusty plasma are studied for nonzero kinematic viscosity. Sagdeev’s potential
can be obtain upto any order in ϕ. The existence of soliton solution is determined by pseudopotential approach. It is seen
that the electron inertia has a significant effect on the existence of solitary waves in presence of kinematic viscosity. 相似文献
174.
H. Kim G. P. Kushto R. C. Y. Auyeung A. Piqué 《Applied Physics A: Materials Science & Processing》2008,93(2):521-526
Fluorine-doped tin oxide (FTO) thin films have been investigated as an alternative to indium tin oxide anodes in organic photovoltaic
devices. The structural, electrical, and optical properties of the FTO films grown by pulsed laser deposition were studied
as a function of oxygen deposition pressure. For 400 nm thick FTO films deposited at 300°C and 6.7 Pa of oxygen, an electrical
resistivity of 5×10−4 Ω-cm, sheet resistance of 12.5 Ω/□, average transmittance of 87% in the visible range, and optical band gap of 4.25 eV were obtained. Organic photovoltaic (OPV)
cells based on poly(3-hexylthiophene)/[6,6]-phenyl-C61-butyric acid methyl ester bulk heterojunctions were prepared on FTO/glass electrodes and the device performance was investigated as a function of FTO
film thickness. OPV cells fabricated on the optimum FTO anodes (∼300–600 nm thick) exhibited power conversion efficiencies
of ∼3%, which is comparable to the same device made on commercial ITO/glass electrodes (3.4%). 相似文献
175.
S. Gaspard M. Oujja R. de Nalda M. Castillejo L. Bañares S. Lazare R. Bonneau 《Applied Physics A: Materials Science & Processing》2008,93(1):209-213
We have recently shown that irradiation of self-standing films of the biopolymers collagen and gelatine with single femtosecond
laser pulses produces a nanofoaming layer with regular bubble size which can be controlled by wavelength selection. Following
these initial studies, here we report on the temporal evolution of the foaming effect by measurements in situ and in real
time of the change in the transmittance of a cw probe HeNe laser through the irradiated films. Self standing films of the
biopolymers were irradiated with 90 fs laser pulses at 800, 400, and 266 nm. For fluences below and above the modification
threshold a permanent attenuation of the transmission occurs (increasing with fluence). The initial decay of the transmission
is fast (around few tens of ns), and is followed by dynamics in the longer timescale (micro and milliseconds). The temporal
evolution of the transmission measured upon fs laser irradiation is similar with that determined in the irradiation of the
biopolymer films at 248 nm with 25 ns laser pulses. The method allows separating in time the different processes occurring
after irradiation that lead to a permanent nanofoaming structure, while the results allow us to understand the mechanisms
of femtosecond laser processing of the biopolymers and their interest in biomedical applications. 相似文献
176.
S. Mahmood N. Akhtar 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2008,49(2):217-222
Linear and nonlinear ion acoustic waves in the presence of adiabatically heated ions in magnetized electron-positron-ion plasmas
are studied. The Sagdeev potential approach is employed to obtain the energy integral equation in such a mulitcomponent plasma
using fluid theory. It is found that electron density humps are formed in the subsonic region in magnetized electron-positron-ion
plasmas. The amplitude of electron density hump is decreased with the increase of hot ion temperature in electron-positron-ion
plasmas. However, the increase in positron concentration and obliqueness of the wave increases the amplitude of nonlinear
structure. The increase in positron concentration also reduces the width of the nonlinear structure in a magnetized multicomponent
plasma. The numerical solutions in the form of solitary pulses are also presented for different plasma cases. The results
may be applicable to astrophysical plasma situations, where magnetized electron-positron-ion plasma with hot ions can exist. 相似文献
177.
S. Kang Y.-M. Liu T.-Y. Shi 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,63(1):37-42
The energy spectra of H2
+-like impurities confined in
finite spherical quantum dots have been calculated as a function
of the distance between nuclear with different sizes on the basis
of effective-mass approximation by linear variational method.
B-splines have been used as basis functions, which can easily
construct the trial wavefunctions with appropriate boundary and
cusp conditions. The quantitative analyses of the partial wave
weights for ground state and some low lying states have been done. 相似文献
178.
A. Shabunin A. Efimov 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,65(3):387-393
A spatio-temporal process in the Lattice Lotka Volterra (LLV) model, when realized on low dimensional support, is studied.
It is shown that the introduction of a long-range mixing causes a drastic change in the system’s behavior, which transits
from small random-like fluctuations to global oscillations when the mixing rate transcends above a critical point. The amplitude
of the induced oscillations is well defined by the mixing rate and is insensitive to the initial conditions and the lattice
size variations. The observed behavior essentially differs from that predicted by the Mean-Field model which is conservative.
The oscillations are of limit-cycle type and appear as a stochastic analog of a Hopf bifurcation. 相似文献
179.
A. Fiasconaro W. Ebeling E. Gudowska-Nowak 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,65(3):403-414
We give an overview over recent studies on the model of Active Brownian Motion (ABM) coupled to reservoirs providing free
energy which may be converted into kinetic energy of motion. First, we present an introduction to a general concept of active
Brownian particles which are capable to take up energy from the source and transform part of it in order to perform various
activities. In the second part of our presentation we consider applications of ABM to ratchet systems with different forms
of differentiable potentials. Both analytical and numerical evaluations are discussed for three cases of sinusoidal, staircaselike
and Mateos ratchet potentials, also with the additional loads modelled by tilted potential structure. In addition, stochastic
character of the kinetics is investigated by considering perturbation by Gaussian white noise which is shown to be responsible
for driving the directionality of the asymptotic flux in the ratchet. This stochastically driven directionality effect is visualized as a strong nonmonotonic dependence of the statistics of the right versus left trajectories of motion
leading to a net current of particles. Possible applications of the ratchet systems to molecular motors are also briefly discussed. 相似文献
180.
When the processive motor protein kinesin walks along the biopolymer microtubule it can occasionally make a backward step.
Recent single molecule experiments on moving kinesin have revealed that the forward-to-backward step ratio decreases exponentially
with the load force. Carter and Cross (Nature 435, 308-312, 2005) found that this ratio tightly followed 802 × exp[−0.95F], where F is the load force in piconewtons. A straightforward analysis of a Brownian step leads to L/(2k
B
T) as the factor in front of the load force, where L is the 8 nm stepsize, k
B
is the Boltzmann constant, and T is the temperature. The factor L/(2k
B
T) does indeed equal 0.95 pN−1. The same analysis shows how the 802 prefactor derives from the power stroke energy G as exp[G/(2k
B
T)]. There are indications that the power stroke derives from the entropically driven coiling of the 30 amino acid neck linker
that connects the two kinesin heads. This idea is examined and consequences are deduced. 相似文献