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81.
P. Rudolf R. Raval P. Dumas G.P. Williams 《Applied Physics A: Materials Science & Processing》2002,75(1):147-153
Infrared (IR) spectroscopy of chemisorbed C60 on Ag (111), Au (110) and Cu (100) reveals that a non-IR-active mode becomes active upon adsorption, and that its frequency
shifts proportionally with the charge transferred from the metal to the molecule by about 5 cm-1 per electron. The temperature dependence of the frequency and the width of this IR feature have also been followed for C60/Cu (100) and were found to agree well with a weak anharmonic coupling (dephasing) to a low-frequency mode, which we suggest
to be the frustrated translational mode of the adsorbed molecules.
Additionally, the adsorption is accompanied by a broadband reflectance change, which is interpreted as due to the scattering
of conduction electrons of the metal surface by the adsorbate. The reflectance change allows determination of the friction
coefficient of the C60 molecules, which results in rather small values (∼2×109 s-1 for Ag and Au, and ∼1.6×109 s-1for Cu), consistent with a marked metallic character of the adsorbed molecules.
Pre-dosing of alkali atoms onto the metal substrates drastically changes the IR spectra recorded during subsequent C60 deposition: anti-absorption bands, as well as an increase of the broadband reflectance, occur and are interpreted as due
to strong electron–phonon coupling with induced surface states.
Received: 6 June 2001 / Accepted: 23 October 2001 / Published online: 3 April 2002 相似文献
82.
An experimental method for determining the real-time depth of laser-drilled holes is presented. The proposed method involves
detecting the laser-induced optoacoustic waves generated during the interaction of the laser beam with the material. Our optodynamic
study involved measuring the propagation times of these waves as they traveled through the material and analyzing their temporal
behavior during the drilling process. The experimental observations revealed an exponential relationship between the propagation
time of the longitudinal stress wave and the number of consecutive laser pulses.
Received: 25 October 2001 / Accepted: 27 October 2001 / Published online: 20 December 2001 相似文献
83.
G. Tiana M.H. Jensen K. Sneppen 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,29(1):135-140
A feedback mechanism that involves the proteins p53 and mdm2, induces cell death as a controlled response to severe DNA damage.
A minimal model for this mechanism demonstrates that the response may be dynamic and connected with the time needed to translate
the mdm2 protein. The response takes place if the dissociation constant k between p53 and mdm2 varies from its normal value. Although it is widely believed that it is an increase in k that triggers the response, we show that the experimental behaviour is better described by a decrease in the dissociation
constant. The response is quite robust upon changes in the parameters of the system, as required by any control mechanism,
except for few weak points, which could be connected with the onset of cancer.
Received 8 May 2002 / Received in final form 9 July 2002 Published online 17 September 2002 相似文献
84.
85.
86.
M.V. Kossov 《The European Physical Journal A - Hadrons and Nuclei》2002,14(3):377-392
Photonuclear interaction cross-sections from the GEANT4 database are approximated for all nuclei and all energies (from the
hadron production threshold to about 40 TeV). The approximation methods in the giant-dipole resonance region, nucleon resonance
region, and high-energy region are improved with respect to existing approximations. As an application of the approximation
for photonuclear cross-sections, an improved method of calculating electronuclear cross-sections is developed. The interaction
cross-section of virtual photons with nuclei at high Q2 are approximated and a simple algorithm for describing the electronuclear reactions, including high-Q2 scattering, is proposed.
Received: 22 February 2002 / Accepted: 6 May 2002 相似文献
87.
88.
混合判断矩阵排序方法研究 总被引:2,自引:0,他引:2
本文介绍了混合判断矩阵及完全一致性混合判断矩阵的概念,提出了混合判断矩阵排序的一种最小偏差法,并给出了其收敛性迭代算法,最后通过算例说明了方法的可行性。 相似文献
89.
[Na(18-C-6)]2[Cu(i-mnt)2]的合成与结构分析 总被引:2,自引:2,他引:0
研究了18-冠-6与Na2[Cu(i-mnt)2][i-mnt=异丁二腈烯二硫醇阴离子,S2CC(CN)2-2]的反应,得到的配合物[Na(18-C-6)]2[Cu(i-mnt)2](1)通过元素分析、红外光谱、X射线单晶衍射进行了结构分析.配合物为单斜晶系,空间群P2(1)/c.晶体学结构数据a=1.2819(11),b=1.1793(10),c=1.4928(13)nm,β=99.121(16)°,V=2.228(3)nm3,Z=2,Dcaled.=1.369g/cm3,F(000)=958,R1=0.0521,wR2=0.1003.1中的[Cu(i-mnt)2]基团通过配体i-mnt的氮原子与两个[Na(18-C-6)]基团中的钠原子成键,形成稳定的中性配合物. 相似文献
90.
A. Khrennikov 《Annalen der Physik》2003,12(10):575-585
We study the probabilistic consequences of the choice of the basic number field in the quantum formalism. We demonstrate that by choosing a number field for a linear space representation of quantum model it is possible to describe various interference phenomena. We analyse interference of probabilistic alternatives induced by real, complex, hyperbolic (Clifford) and p‐adic representations. 相似文献