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51.
A new multireference perturbation series is derived based on the Rayleigh–Schrödinger perturbation theory. It is orbitally invariant. Its computational cost is comparable to the single reference Møller–Plesset perturbation theory. It is demonstrated numerically that the present multireference second‐ and third‐order energies are size extensive by two types of supermolecules composed of H2 and BH monomers. Spectroscopic constants of as well as the ground state energies of H2O, NH2, and CH2 at three bond lengths have been calculated with the second multireference perturbation theory. The dissociation behaviors of CH4 and HF have also been investigated. Comparisons with other approximate theoretical models as well as the experimental data have been carried out to show their relative performances. © 2013 Wiley Periodicals, Inc. 相似文献
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Jeffery M. Tharp Omer Ad Kazuaki Amikura Fred R. Ward Emma M. Garcia Jamie H. D. Cate Alanna Schepartz Dieter Sll 《Angewandte Chemie (International ed. in English)》2020,59(8):3122-3126
By transplanting identity elements into E. coli tRNAfMet, we have engineered an orthogonal initiator tRNA (itRNATy2) that is a substrate for Methanocaldococcus jannaschii TyrRS. We demonstrate that itRNATy2 can initiate translation in vivo with aromatic non‐canonical amino acids (ncAAs) bearing diverse sidechains. Although the initial system suffered from low yields, deleting redundant copies of tRNAfMet from the genome afforded an E. coli strain in which the efficiency of non‐canonical initiation equals elongation. With this improved system we produced a protein containing two distinct ncAAs at the first and second positions, an initial step towards producing completely unnatural polypeptides in vivo. This work provides a valuable tool to synthetic biology and demonstrates remarkable versatility of the E. coli translational machinery for initiation with ncAAs in vivo. 相似文献
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§1Introduction Asweknow,Backlundtransformation[1-3]isaverypowerfulwayforfindingnonline evolutionequations.Inrecentdecades,Painlevéanalysis[4]hasbecomeaverypopu methodtoobtainBacklundtransformation.Inreference[5],fordevelopingthetheory Painlevéanalysis,AndrewPickeringintroduceanewexpansionvariableZwhichsatisf thefollowingRicattiSystem:Zx=1-AZ-BZ2,Zt=-C+(AC+Cx)Z-(D-BC)Z2.(1.Astheapplicationofthenewexpansionvaraible,thepotentialfifth-orderMKd equation(PMKdV5)-vxt+(vxxxxx-10k2v2… 相似文献
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为解决较多图像匹配算法主要通过测量关键点之间的距离来实现特征匹配,忽略了图像的结构信息,使其存在较多的误匹配的问题,本文设计了方差约束耦合几何不变特性的图像匹配算法。借助于Forstner算子计算像素点的兴趣值,以检测图像的特征;计算图像的梯度信息,获取图像的方向值,并切割图像特征的圆形邻域,从而获取扇形子域;以图像的方向值为基础,通过计算扇形子域中的灰度不变矩,输出对应的特征向量;引入区域方差函数,获取图像的结构信息,将其加入至图像特征的匹配过程,以约束欧式距离的测量结果,实现图像特征匹配;最后利用匹配点间的几何不变特性,对匹配特征去伪求真,优化匹配结果。测试数据表明:相对于已有的匹配技术,在对无变换图像、缩放图像以及旋转图像匹配时,所提算法拥有更高的匹配准确度,分别达到了96.56%、95.38%和93.52%。 相似文献
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《Physics letters. A》2020,384(26):126642
A novel method to make Lagrangians Galilean invariant is developed. The method, based on null Lagrangians and their gauge functions, is used to demonstrate the Galilean invariance of the Lagrangian for Newton's law of inertia. It is suggested that this new solution of an old physics problem may have implications and potential applications to all gauge-based theories of physics. 相似文献
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Joachim Zacharias 《Proceedings of the American Mathematical Society》2006,134(7):1909-1916
Recently J.Roe considered the question of whether for a discrete group the reduced group -algebra is the fixed point algebra of Ad acting on the uniform Roe algebra . is said to have the invariant translation approximation property in this case. We consider a slight generalization of this property which, for exact , is equivalent to the operator space approximation property of . We also give a new characterization of exactness and a short proof of the equivalence of exactness of and exactness of for discrete groups.
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研究了一类多因素HIV模型.建立了一个标准型的DI模型,证明了无病平衡点的局部渐近稳定性和全局渐近稳定性. 相似文献