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941.
G.D. Roston Z.F. Ghatass 《Journal of Quantitative Spectroscopy & Radiative Transfer》2008,109(14):2427-2436
The temperature dependence of the Cd line absorption profile at 326.1 nm perturbed by Kr has been carefully studied over a spectral range extending from 800 cm−1 in the blue wing to 1200 cm−1 in the red wing using a high-resolution double-beam spectrometer. The atomic densities of krypton (NKr) and cadmium (NCd) were (2.015±0.07)×1019 and (3.62±0.05)×1018 cm−3, respectively. The temperature dependence of the studied line profile was analyzed in the framework of the quasi-static theory. The van der Waals coefficient differences between the ground 10+ state and the two excited states 30+ and 31 (ΔC60 and ΔC61) were obtained from the near red wing profile using Kuhn's law. The values of ΔC60 and ΔC61 are found to be equal to 37.8±2 and 58.5±3 eV Å6, respectively. The ground (X 10+), and the excited (31, 30+) state potentials at the internuclear separations from 3.2 to 6.3 Å were determined. The well depths with their positions for these states are respectively equal to 134±7 cm−1, 3.95±0.2 Å; 72.3±4 cm−1, 4.95±0.3 Å; and 471±12 cm−1, 3.6 Å. The obtained well depths with their allowable errors are in good agreement with the values obtained before for the Cd-Kr system from some theoretical results and molecular beams experiments. 相似文献
942.
近年来,为提高磁共振成像(MRI)信号信噪比(SNR)、缩短成像时间,同时多层成像技术受到了极大的关注.为了实现同时多层的选择性激发,现有的多层成像序列大多使用组合射频(RF)脉冲,该脉冲可包含多个独立的幅值相同相位不同的简单脉冲,由于其采用简单的线性叠加方法,该类脉冲射频功率随脉冲数量呈现平方增长,因而应用受限.针对这一问题,基于自旋动力学和优化控制原理,本文提出了一种针对同时多层MRI的选择性射频脉冲的数值优化方法,该方法充分运用射频脉冲的调控机制,获得优化脉冲,并配合层选梯度,可实现任意层厚、层间距、层数的同时高效选择性激发.最后,通过数字模体的同时多层模拟成像实验验证了优化脉冲的有效性. 相似文献
943.
采用双向凝胶电泳和生物质谱技术, 对12对胰腺癌组织和癌旁组织样品、3个胰腺良性疾病样品、3个正常胰腺组织样品的蛋白质进行了分离和鉴定, 获得了重复性较好的双向凝胶电泳图谱; 鉴定了胰腺癌和癌旁组织的差异表达蛋白质, 发现了30个差异表达蛋白质; 应用MALDI-TOF-MS/MS技术对差异表达蛋白质进行鉴定, 共有24个蛋白质得到鉴定, 其中15个蛋白质在胰腺癌组织中表达上调, 9个蛋白质表达下调. 这些蛋白质与胰腺癌的发生相关, 可能成为胰腺癌的分子标志物和药物治疗的靶蛋白. 相似文献
944.
Environmental change in general, and climate change in particular, can lead to changes in distribution of fish stocks. When such changes involve transboundary fish stocks, the countries sharing the stock need to reconsider their harvesting policies. We investigate the effects of changing stock distribution on the optimal fishing policies in a two players’ noncooperative game. We compare reactive management, under which the manager ignores future distributional shifts (knowingly or unknowingly), with proactive management where the manager considers such shifts in his decisions. A dynamic programming model is developed to identify closed‐loop Nash strategies. We show that the role of two players is symmetric under reactive management but asymmetric under proactive management where managers anticipate future changes in stock ownership. The player losing the stock tends to harvest more aggressively compared to the player gaining the stock who acts more conservatively. Strategic interactions show tendency for complementary actions that can change abruptly during the ownership transition. The differences between management regimes vary from quantitative to qualitative; differences are minimal for stocks with little or no schooling, whereas highly schooling stocks may avoid collapse only under proactive management. 相似文献
945.
946.
947.
The mechanism of cycloaddition reaction between singlet state H2Ge=Ge: and acetaldehyde has been investigated with the MP2/6-311++G** method. From the potential energy profile, it could be predicted that the reaction has two competitive dominant reaction pathways. The reaction rule presented is that the two reactants firstly form a four-membered Ge-heterocyclic ring germylene through the [2+2] cycloaddition reaction. As the 4p unoccupied orbital of Ge: atom in the four-membered Ge-heterocyclic ring germylene and the π orbital of acetaldehyde form a π→p donor-acceptor bond, the four-membered Ge-heterocyclic ring germylene further combines with acetaldehyde to give an intermediate. Because the Ge atom in intermediate exhibits sp3 hybridization after transition state, the intermediate isomerizes to a spiro-Ge-heterocyclic ring compound via a transition state. Simultaneously, the ring strain of the four-membered Ge-heterocyclic ring germylene makes it isomerize to a twisted four-membered ring product. 相似文献
948.
Marjan Cosyns Geert Mortier Paul Corthals Sandra Janssens John Van Borsel 《Journal of voice》2011,25(6):759-764
Neurofibromatosis type 1 (NF1) is an autosomal dominant neurocutaneous disorder caused by mutations in the NF1 gene, which is located at the long arm of chromosome 17. Major characteristics include multiple café-au-lait spots and neurofibromas. Voice abnormalities have been reported to occur in this patient group. However, most studies relied on subjective measurements only. The present study reports the results of an objective voice assessment based on a multiparameter approach in 22 adults with NF1. Aerodynamic measurements, voice range profiles, acoustic voice quality and intonation measurements, and dysphonia severity indices were obtained and compared with data from a control group, consisting of 22 healthy adults. It was found that NF1 patients show a poorer overall voice quality compared with controls. Particularly, a reduction of vital capacity and limitations in laryngeal possibilities with respect to frequency and intensity were observed in the NF1 group. 相似文献
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950.