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81.
《Journal of Polymer Science.Polymer Physics》2018,56(12):914-923
N,N‐dialkylaminoethyl methacrylate (DAEA) monomers are extensively used to prepare multi‐responsive polymers. However, these monomers face high risk of hydrolysis in their ester groups when being polymerized in water‐containing medias. Here, NMR spectroscopy was employed to continuously track the hydrolysis and solubility of four widely used DAEA monomers [CH2CH2R1COO(CH2)2N(R2)2; R1 = H or CH3; R2 = CH3, CH2CH3 or CH(CH3)2] under typical polymerization conditions. With this technique, the hydrolysis reactivity and absolute hydrolysis amount of these monomers are separately examined, and then their kinetic correlations with solubility, molecular structure, pH, and temperature are established, so that the hydrolysis of DAEA monomers and even other esters with similar cyclic structure can be predicted. The present efforts are expected to provide a general understanding for the hydrolysis of all the DAEA monomers, benefitting to the optimization of polymerization toward well‐defined DAEA copolymers, as well as the design of smart soft matter for specific applications. © 2018 Wiley Periodicals, Inc. J. Polym. Sci., Part B: Polym. Phys. 2018 , 56, 914–923 相似文献
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83.
The behavior of a two-level entangled atom in an optical field with circular polarization is studied in this paper. The interaction of an optical field and one of the entangled atoms is analyzed in detail. A general solution of the SchrAo¨Gdinger equation about the motion of the entangled atom is obtained. The properties of the action are dependent on the initial state of the atom. By detecting the entangled atom out of the field, we can obtain the state of the other atom moving in the field. It is shown that the state of the atom out of the field will influence the energies of the split-levels of the atom in the field. 相似文献
84.
Ladislav Adamec 《Applications of Mathematics》2005,50(2):93-101
In the theory of autonomous perturbations of periodic solutions of ordinary differential equations the method of the Poincaré mapping has been widely used. For the analysis of properties of this mapping in the case of two-dimensional systems, a result first obtained probably by Diliberto in 1950 is sometimes used. In the paper, this result is (partially) extended to a certain class of autonomous ordinary differential equations of higher dimension.This research was supported by Grant No. 201/99/0295 of the Grant Agency of the Czech Republic.This revised version was published online in April 2005 with a corrected missing date string. 相似文献
85.
采用量子光学中时间演化算符方法,研究了与运动原子相互作用的场的压缩效应,揭示了光场的初始平均光子数和场模结构参数对光场压缩特性的影响,结果表明:适当选择系统参数,可获得在时间上持续压缩的压缩光。 相似文献
86.
本文将移动粒子半隐式法(MPS)的基本算法由二维扩展至三维。将圆柱坐标系引入到初场粒子的布置中,避免了在笛卡儿坐标系下处理不规则形状(如斜边或曲边)问题时粒子初场布置困难和精确度较低的问题,改善了对计算边界条件表达的精确性。引入移动边界模型,对直叶片搅拌器的内部流动进行了三维数值模拟。还提出了一种新的初始粒子布置简易方法,明显简化粒子初始布置时的复杂程度,提高了对三维复杂几何形状问题的可操作性。 相似文献
87.
2×2列联表中二属性相关的假设检验是定性数据分析中的热点问题,针对此问题的研究频率学派已做过大量的工作,其理论方法已趋于成熟.利用Bayes检验研究2×2列联表中二属性的相关性迄今为止国内外的相关文献还为数不多.将依据Bayes理论对此问题提出新的检验方法,推出其Bayes因子计算公式,利用正态近似研究三项假设计算出有关的后验概率,不仅解决了频率学派难以处理的问题,并且为吸烟有害健康提供了理论支撑. 相似文献
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89.
A new cellular automaton (CA) model based on brake light rules is proposed, which considers the influence of deterministic deceleration on randomization probability and deceleration extent. To describe the synchronized flow phase of Kerner’s three-phase theory in accordance with empirical data, we have changed some rules of vehicle motion with the aim to improve speed and acceleration vehicle behavior in synchronized flow simulated with earlier cellular automaton models with brake lights. The fundamental diagrams and spatial–temporal diagrams are analyzed, as well as the complexity of the traffic evolution, the emergence process of wide moving jam. Simulation results show that our new model can reproduce the three traffic phases: free flow, synchronized flow and wide moving jam. In addition, our new model can well describe the complexity of traffic evolution: (1) with initial homogeneous distribution and large densities, the traffic will evolve into multiple steady states, in which the numbers of wide moving jams are not invariable. (2) With initial homogeneous distribution and the middle range of density, the wide moving jam will emerge stochastically. (3) With initial mega-jam distribution and the density close to a point with the low value, the initial mega-jam will disappear stochastically. (4) For the cases with multiple wide moving jams, the process is analyzed involving the generation of narrow moving jam due to “pinch effect”, which leads to wide moving jam emergence. 相似文献
90.
针对远距离复杂背景下红外小目标检测问题,本文提出了一种基于小波高频距离像的方法。该方法首先将处理空间变换到小波域,通过分析残留背景、目标和噪声系数在高频子带的差异,定义基于邻域均值的子带系数表达形式,构造高频子带系数的中心向量,对小波高频图像进行综合形成距离像,得到红外复杂背景的抑制结果。在此基础上,利用恒虚警率算法将单帧背景抑制图像分割成候选目标、残留背景和噪声像素点。最后,在时间域基于目标运动的相关性,利用管道滤波实现红外小目标的最终检测。仿真实验结果表明,相对于经典算法,本文方法可以实现对红外复杂背景的有效抑制,增强目标信号的强度,准确稳定的从红外复杂背景中检测出小目标。 相似文献