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11.
12.
Lithium Insertion Mechanism in Iron-Based Oxyfluorides with Anionic Vacancies Probed by PDF Analysis
Dr. Damien Dambournet Dr. Karena W Chapman Dr. Mathieu Duttine Dr. Olaf Borkiewicz Dr. Peter J Chupas Dr. Henri Groult 《ChemistryOpen》2015,4(4):443-447
The mechanism of lithium insertion that occurs in an iron oxyfluoride sample with a hexagonal–tungsten–bronze (HTB)-type structure was investigated by the pair distribution function. This study reveals that upon lithiation, the HTB framework collapses to yield disordered rutile and rock salt phases followed by a conversion reaction of the fluoride phase toward lithium fluoride and nanometer-sized metallic iron. The occurrence of anionic vacancies in the pristine framework was shown to strongly impact the electrochemical activity, that is, the reversible capacity scales with the content of anionic vacancies. Similar to FeOF-type electrodes, upon de-lithiation, a disordered rutile phase forms, showing that the anionic chemistry dictates the atomic arrangement of the re-oxidized phase. Finally, it was shown that the nanoscaling and structural rearrangement induced by the conversion reaction allow the in situ formation of new electrode materials with enhanced electrochemical properties. 相似文献
13.
G.E. Farr 《Discrete Mathematics》2019,342(5):1510-1519
This paper continues the study of combinatorial properties of binary functions — that is, functions such that , where is a finite set. Binary functions have previously been shown to admit families of transforms that generalise duality, including a trinity transform, and families of associated minor operations that generalise deletion and contraction, with both these families parameterised by the complex numbers. Binary function representations exist for graphs (via the indicator functions of their cutset spaces) and indeed arbitrary matroids (as shown by the author previously). In this paper, we characterise degenerate elements – analogues of loops and coloops – in binary functions, with respect to any set of minor operations from our complex-parameterised family. We then apply this to study the relationship between binary functions and Tutte’s alternating dimaps, which also support a trinity transform and three associated minor operations. It is shown that only the simplest alternating dimaps have binary representations of the form we consider, which seems to be the most direct type of representation. The question of whether there exist other, more sophisticated types of binary function representations for alternating dimaps is left open. 相似文献
14.
《Annales de l'Institut Henri Poincaré (C) Analyse Non Linéaire》2020,37(2):417-456
We study the energy-critical nonlinear wave equation in the presence of an inverse-square potential in dimensions three and four. In the defocussing case, we prove that arbitrary initial data in the energy space lead to global solutions that scatter. In the focusing case, we prove scattering below the ground state threshold. 相似文献
15.
Ratnabali Biswas Kaushik Chowdhury Dharma P. Agrawal 《International Journal of Wireless Information Networks》2006,13(4):303-315
Wireless sensor network is an emerging technology that enables remote monitoring of large geographical regions. In this paper, we address the problem of distributing attributes over such a large-scale sensor network so that the cost of data retrieval is minimized. The proposed scheme is a data-centric storage scheme where the attributes are distributed over the network depending on the correlations between them. The problem addressed here is similar to the Allocation Problem of distributed databases. In this paper, we have defined the Allocation Problem in the context of sensor networks and have proposed a scheme for finding a good distribution of attributes to the sensor network. We also propose an architecture for query processing given such a distribution of attributes. We analytically determine the conditions under which the proposed architecture is beneficial and present simulation results to demonstrate the same. To the best of our knowledge, this is the first attempt to determine an allocation of attributes over a sensor network based on the correlations between attributes. 相似文献
16.
论文提出利用用户提供的个性化信息来随机产生关联大素数,保证了素数选取的随机化、个性化,提高了RSA算法的安全性。 相似文献
17.
蔡剑锋 《信息安全与通信保密》2006,(9):142-144
论文通过对病毒及反病毒技术的发展分析,总结了现有一些较优秀的杀毒软件的优缺点,提出了基于新理念的攻防查杀型杀毒软件的实现模型。 相似文献
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19.
径向基函数神经网络的再学习算法及其应用 总被引:3,自引:1,他引:2
谭建辉 《微电子学与计算机》2006,23(5):115-117,120
为了应用径向基函数神经网络逐步地识别待研究系统,文章针对径向基函数神经网络的再学习算法开展了深入的研究.应用严格的数学推理方法,将径向基函数神经网络的再学习问题转化为矩阵求逆的附加运算.详细给出了径向基函数神经网络再学习算法中增加新训练样本和增加新基函数的数学公式,同时对如何获取新的训练样本进行了研究. 相似文献
20.
虚拟演播室是传统视频技术与计算机虚拟现实技术相结合的产物 ,它可以把现场视频与计算机影像等实时、无缝地合成在—起 ,是对传统电视演播室的一次重大变革。主要讨论虚拟演播室的工作原理、功能及其应用 相似文献