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111.
112.
Using the methods of molecular simulation and HyperChem v.5.0 programs (PM3 method), we carried out calculations of the principal spectroscopic characteristics and of the structure of the laurdan molecule in the ground and the first excited electronic states. The thermal static distribution of molecules over various possible orientations of the plane of methyl groups relative to the plane of the naphthalene bicycle was taken into account. The energies and dipole moments of these electronic states have been calculated as functions of the torsion angle of methyl groups. The existence of an additional mechanism of electronic spectrum broadening is shown; it is associated with thermal mismatch of the equilibrium orientations of the rotational fragment of the molecule and with the dependence of the electron transition frequency on the degree of deviation of the angle from the equilibrium value. The dependence of dipole moments on this angle has been found and calculated. This dependence is the strongest for the ground state. The maximum values of dipole moments in the ground and excited states are 4.0 and 7.6 D. 相似文献
113.
Molecular motions of polycrystalline cellobiose have been investigated by measuring proton spin–lattice relaxation times, T1 and T1ρ, and the second moment, M2, in both protonated and D2O exchanged forms over the temperature range 120–380 K. T1 relaxation is dominated by the motions of hydroxyl groups between 150 and 380 K, characterised by an activation energy of about 8.74 kJ/mol, whereas T1ρ relaxation is driven by the motions of the same groups between 120 and 300 K. T1ρ results suggest that hydroxyl groups have a distribution of dynamics. Motion of methylene groups was detected in the second-moment experiments at about 350 K, characterised by activation energy of about 40 kJ/mol. Consideration of the calculated and observed rigid-lattice second moments suggests that the reported X-ray data are incorrect for the inter-proton distance on C6′. 13C CPMAS spectra of both protonated and deuterated cellobiose have also been measured. Spectra of the deuterated material showed the existence of a second crystalline form in addition to the normal form. 相似文献
114.
针对矩形波导滤波器设计中遇到的探针匹配问题,需要得到探针位于波导宽边任意位置时的输入阻抗。文中利用矩量法和格林函数分析了探针位于波导宽边任意位置时的输入阻抗,并结合三腔体法得到对应两端口散射矩阵,与文献中Ji-Fuh Liang的实验数据相比较,结果较为吻合。进而可以根据滤波器设计所需要的参数决定探针激励位置。 相似文献
115.
Almost-Sure Results for a Class of Dependent Random Variables 总被引:17,自引:0,他引:17
The aim of this note is to establish almost-sure Marcinkiewicz-Zygmund type results for a class of random variables indexed by
d
+
—the positive d-dimensional lattice points—and having maximal coefficient of correlation strictly smaller than 1. The class of applications include filters of certain Gaussian sequences and Markov processes. 相似文献
116.
Min Zhang Aanying Ma Lu Bai Lewei Li Zhensen Wu 《International Journal of Infrared and Millimeter Waves》2005,26(5):701-713
We present an effective numerical technique to characterize the scattering of wide-slot antennas fed by waveguides with arbitrary terminations in terms of the method of moment (MoM) and the mixed potential integral equation (MPIE). In particular, the precorrected-fast Fourier transform (P-FFT) eliminates the need to generate and store the usual square impedance matrix andthus leads to speed up the matrix-vector multiplication in the resultant system. This property makes the Rao-Wilton-Glisson (RWG) functions to be useful in simulating electrically large-scale problems. In addition, the scattering from the finite ground surfaces is accounted for in the total scattered field by using the method of equivalent edge currents. The numerical results are presented and compared with both the traditional method of moment results obtained using the entire-domain basis functions and the experimental results, to demonstrate the proposed method to be a good candidate for study on the scattering of arbitrary wide-slot large array. 相似文献
117.
A. V. Latyshev V. N. Popov A. A. Yushkanov 《Journal of Applied Mechanics and Technical Physics》2004,45(1):17-22
The slip velocity of a rarefied gas with inhomogeneous temperature and mass velocity on a solid spherical surface is calculated with the use of a twomoment boundary condition in the linear approximation in terms of the Knudsen number. The dependence of the slip velocity on accommodation coefficients of the two first moments of the distribution function is studied. 相似文献
118.
119.
We introduce and study matrix Christoffel functions for a matrix
weight W.
We find an explicit expression of the matrix Christoffel functions
in terms of any sequence of orthonormal matrix polynomials with
respect to W. An extremal property related to the matrix moment
problem defined by W is established for the matrix Christoffel
functions. We finally find the relative asymptotic behavior of
the matrix Christoffel functions associated to matrix weights in
the matrix Nevai class. 相似文献
120.
A.A. Zvyagin 《The European Physical Journal B - Condensed Matter and Complex Systems》2003,32(3):351-360
The behavior of charge and spin persistent currents in an integrable lattice ring of strongly correlated electrons with a
magnetic impurity is exactly studied. Our results manifest that the oscillations of charge and spin persistent currents are
similar to the ones, earlier obtained for integrable continuum models with a magnetic impurity. The difference is due to two
(instead of one) Fermi velocities of low-lying excitations. The form of oscillations in the ground state is “saw-tooth”-like,
generic for any multi-particle coherent one-dimensional models. The integrable magnetic impurity introduces net charge and
spin chiralities in the generic integrable lattice system, which determine the initial phase shifts of charge and spin persistent
currents. We show that the magnitude of the charge persistent current in the generic Kondo situation does not depend on the
parameters of the magnetic impurity, unlike the (magneto)resistivity of transport currents.
Received 30 January 2003 / Received in final form 12 March 2003 Published online 11 April 2003
RID="a"
ID="a"e-mail: zvyagin@fy.chalmers.se 相似文献