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71.
An Efficient Labelling Approach to Harness Backbone and Side‐Chain Protons in 1H‐Detected Solid‐State NMR Spectroscopy 下载免费PDF全文
Deni Mance Dr. Tessa Sinnige Mohammed Kaplan Siddarth Narasimhan Mark Daniëls Dr. Klaartje Houben Prof. Marc Baldus Dr. Markus Weingarth 《Angewandte Chemie (International ed. in English)》2015,54(52):15799-15803
1H‐detection can greatly improve spectral sensitivity in biological solid‐state NMR (ssNMR), thus allowing the study of larger and more complex proteins. However, the general requirement to perdeuterate proteins critically curtails the potential of 1H‐detection by the loss of aliphatic side‐chain protons, which are important probes for protein structure and function. Introduced herein is a labelling scheme for 1H‐detected ssNMR, and it gives high quality spectra for both side‐chain and backbone protons, and allows quantitative assignments and aids in probing interresidual contacts. Excellent 1H resolution in membrane proteins is obtained, the topology and dynamics of an ion channel were studied. This labelling scheme will open new avenues for the study of challenging proteins by ssNMR. 相似文献
72.
The interactive two-state model of cell membrane ion channels in an electric field is formulated on the Bethe lattice by means
of the exact recursion relations. The probability of channel opening or maximum fractions of open potassium and sodium channels
are obtained by solving a non-linear algebraic equation. Using known parameters for the conventional mean-field theory the
model gives a good agreement with the experiment both at low and high trans-membrane potential values. For intermediate voltages,
the numerical results imply that collective effects are introduced by trans-membrane voltage. 相似文献
73.
频率选择性衰落信道中,接收伪噪声(Pseudo-Noise,PN)码的不确定相位空间中存在多个同相单元。建立检测模型获得了检测过程的检测概率和虚警概率。通过状态转移图结合划分码相位子空间的方法对捕获状态的循环流转进行了描述,获得了捕获性能对信道特性的依赖关系。数值仿真给出了捕获性能随路径数量和接收信噪比等主要参数的变化趋势。 相似文献
74.
75.
Smart DNA Hydrogel Integrated Nanochannels with High Ion Flux and Adjustable Selective Ionic Transport 下载免费PDF全文
Yafeng Wu Dianyu Wang Itamar Willner Ye Tian Prof. Lei Jiang 《Angewandte Chemie (International ed. in English)》2018,57(26):7790-7794
Nanochannels based on smart DNA hydrogels as stimulus‐responsive architecture are presented for the first time. In contrast to other responsive molecules existing in the nanochannel in monolayer configurations, the DNA hydrogels are three‐dimensional networks with space negative charges, the ion flux and rectification ratio are significantly enhanced. Upon cyclic treatment with K+ ions and crown ether, the DNA hydrogel states could be reversibly switched between less stiff and stiff networks, providing the gating mechanism of the nanochannel. Based on the architecture of DNA hydrogels and pH stimulus, cation or anion transport direction could be precisely controlled and multiple gating features are achieved. Meanwhile, G‐quadruplex DNA in the hydrogels might be replaced by other stimulus‐responsive DNA molecules, peptides, or proteins, and thus this work opens a new route for improving the functionalities of nanochannel by intelligent hydrogels. 相似文献
76.
Guozhen Liu Long Cheng Guining Chen Feng Liang Gongping Liu Wanqin Jin 《化学:亚洲杂志》2020,15(15):2364-2370
Mixed matrix membranes (MMMs) made from inorganic fillers and polymers is a kind of promising candidate for gas separation. In this work, two‐dimensional MXene nanosheets were synthesized and incorporated into a polyether‐polyamide block copolymer (Pebax) matrix to fabricate MMM for CO2 capture. The physicochemical properties of MXene nanosheets and MXene/Pebax membranes were studied systematically. The introduction of MXene nanosheets provided additional molecular transport channels and meanwhile enhanced the CO2 adsorption capacity, thereby enhancing both the CO2 peremance and CO2/N2 selectivity of Pebax membrane. The optimized MXene/Pebax membrane with a MXene loading of 0.15 wt % displayed a high separation performance with a CO2 permeance of 21.6 GPU and a CO2/N2 selectivity of 72.5, showing potential application in CO2 capture. 相似文献
77.
Emad K. Al-Hussaini Hebat-Allah M. Mourad Fatma A. Newagy 《Wireless Personal Communications》2004,31(3-4):131-148
In this paper, a multi-carrier code division multiple access (MC-CDMA) downlink mobile communication system employing pre-rake and dual transmit diversity is proposed. It combines high spectral efficiency with an immunity to channel dispersion and fading. It also ensures small size, cost and power consumption of the terminal. Theoretical and simulation results for the system under consideration are obtained. Depicted results show appreciable improvements of the proposed system over those previously known.Emad K. Al-Hussaini received his B.Sc degree in Electrical Communication Engineering from Ain-Shams University, Cairo, Egypt, in 1964 and his M.Sc and Ph.D. degrees from Cairo University, Giza, Egypt, in 1974 and 1977, respectively. From 1964 to 1970, he was with the General Egyptian Aeroorganization. Since 1970, he has been with the Department of Electronics and Communications, Faculty of Engineering, Cairo University, and is currently professor there. He was a research fellow at Imperial College, London, UK, and at the Moore School of Electrical Engineering, University of Pennsylvania, Philadelphia, PA, USA, in the academic years 1976/1977 and 1981/1982, respectively. In 1990, he received the Egyptian national encouragement award for outstanding engineering research. He has written several papers for technical international journals and conferences. His research interests include signal processing, fading channel communication, modulation, and cellular mobile radio systems. Dr Al-Hussaini is a senior member of IEEE. He is listed in Marquis Whos Who in the World and in the IBC (International Biographical Center, Cambridge) for outstanding people of the 20th century.Hebat-Allah M.Mourad received her B.Sc, M.Sc and Ph.D degrees in Electrical Communication Engineering from Cairo University, Egypt, in 1983, 1987 and 1994 respectively. Since 1983 she has been with the Electronics and Communications Department, Faculty of Engineering Cairo University and is currently associate professor there. Her research interests include mobile communications, satellite communications and optical fiber communications.Fatma A. Newagy received her B.Sc and M.Sc degrees in electrical communication engineering from Cairo University, Egypt in 1998 and 2002 respectively. Since 1999, she has been a research assistant with the Department of Electronics and Communications, Faculty of Engineering, Cairo University. She is pursuing her Ph.D. there. Her research interests include mobile communications and modulation techniques for spread spectrum and wireless communications. 相似文献
78.
Nikolaos D. Skentos Athanasios G. Kanatas Panagiotis I. Dallas Philip Constantinou 《Wireless Personal Communications》2006,36(4):339-361
This paper reports results from wideband MIMO measurements performed in short range fixed wireless environments at 5.2 GHz. The objective is to provide MIMO channel characterization results for the measured environments and contribute to the limited available similar studies. Two kinds of propagation scenarios are investigated, rooftop to rooftop and street to rooftop, at three different sites always under LOS propagation conditions. The analysis of measurement data is performed in the context of non physical modeling, providing insight into the statistics of the measured channels. In particular, the slow time varying nature of the channel is studied and the narrow Doppler spectrum shape is approximated. Furthermore, frequency correlation results are obtained and the typical delay dispersion measures are extracted. Then, the antenna correlation is studied and the error of the Kronecker product approximation is evaluated. Finally, capacity results are provided and the channel measurements are characterized in terms of spatial multiplexing quality and multipath richness through condition number analysis.
Nikolaos D. Skentos received his Diploma in Electrical and Computer Engineering from the National Technical University of Athens (NTUA), Greece in October 2000. Since January 2001 he has been a research associate at the Mobile Radio Communications Laboratory at the NTUA, and he is currently working towards the Ph.D. degree. His research interests include channel measurements, MIMO channel characterization, MIMO algorithms and space time processing. He has been active in the IST STINGRAY project, the COST 273 Action and the ACE Network of Excellence. He is also a member of the National Technical Chamber of Greece since 2001.
Athanasios G. Kanatas received the Diploma in Electrical Engineering from the National Technical University of Athens, Greece, in 1991, the M.Sc. degree in Satellite Communication Engineering from the University of Surrey, Surrey, UK in 1992, and the Ph.D. degree in Mobile Satellite Communications from the National Technical University of Athens, Greece in February 1997. From 1993 to 1994 he was with National Documentation Center of National Research Institute. In 1995 he joined SPACETEC Ltd. where he was Technical Project Manager for VISA/EMEA VSAT Project in Greece. In 1996 he joined the Mobile Radio Communications Laboratory as a research associate. From 1999 to 2002 he was with the Institute of Communication & Computer Systems. In 2000 he became a member of the Board of Directors of OTESAT S.A. He is an Assistant Professor in the Department of Technology Education and Digital Systems at University of Piraeus. His current research interests include channel characterization and estimation, simulation and modeling for mobile, mobile satellite, and future wireless communication systems. He has been a Senior Member of IEEE since 2002, and is also a member of the Technical Chamber of Greece. In 1999 he was elected Chairman of the Communications Society of the Greek IEEE Section.
Panagiotis I. Dallas was born 1967 in Thessaloniki, Greece. He obtained his diploma and Ph.D. degree from the Electrical and Computer Engineering Department of Aristotle University of Thessaloniki, Greece, in 1990 and 1997, respectively. Since 1998 he joined with INTRACOM where he currently is Section Manager of Advanced Communications Technologies branch of Emerging Technologies & Markets department, leading the next generation of broadband wireless access systems for internal and EU projects. He runs the relevant standardization activities (IEEE 802.16 and ETSI/BRAN HIPERMAN) in INTRACOM and he represents the company in WiMAX forum. Finally, he has over 30 publications in international journals and conferences.
Philip Constantinou received the Diploma in Physics from the National University of Athens in 1972, the Master of Applied Science in Electrical Engineering from the University of Ottawa, Ontario, Canada in 1976, and the Ph.D. degree in Electrical Engineering in 1983 from Carleton University, Ottawa, Ontario, Canada. From 1976 to 1979 he was with Telesat Canada as a Communications System Engineer. In 1980 he joined the Ministry of Communications in Ottawa, Canada where he was engaged in the area of Mobile Communication. From 1984 to 1989 he was with the National Research Center Demokritos in Athens, Greece where he was involved in several research projects in the area of Mobile Communications. In 1989 he joined the National Technical University of Athens where he is currently a Professor and Director of the Mobile Radio Communications Laboratory. His current research interests include Personal Communications, Mobile Satellite Communications, and Interference Problems on Digital Communications Systems. 相似文献
79.
通过建立Stackelberg博弈模型,研究了在混合渠道下零售商创新投入对供应链的影响,分析了零售商创新成本系数信息对称和不对称两种情况下各方的决策变量和利润受创新成本系数,制造商对零售商创新信息掌握的不确定性程度,需求转移系数,市场潜力及创新潜力等的影响关系。研究结果发现制造商总能通过信息分享受益,另外得到了零售商愿意分享成本信息以及使得供应链整体受益的条件,这些为制造商信息分享决策提供了依据。最后通过算例分析对结果进行了验证。 相似文献
80.
提出利用一个两粒子纠缠态传送N粒子GHZ纠缠态的方案,首先考察三粒子GHZ纠缠态在量子信道是最大纠缠态时情形,然后进一步考察量子信道是非最大纠缠态的情形,发现通过对某些粒子执行H操作和von Neumann测量,并引进两个辅助比特,在非最大纠缠态时还需构造一个幺正变换矩阵,可实现三粒子GHZ纠缠态的隐形传态,最后推广至N粒子,该方案相比其它方案最大的优点是节约了量子信道纠缠资源。 相似文献