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81.
82.
Khaneja N Reiss T Kehlet C Schulte-Herbrüggen T Glaser SJ 《Journal of magnetic resonance (San Diego, Calif. : 1997)》2005,172(2):296-305
In this paper, we introduce optimal control algorithm for the design of pulse sequences in NMR spectroscopy. This methodology is used for designing pulse sequences that maximize the coherence transfer between coupled spins in a given specified time, minimize the relaxation effects in a given coherence transfer step or minimize the time required to produce a given unitary propagator, as desired. The application of these pulse engineering methods to design pulse sequences that are robust to experimentally important parameter variations, such as chemical shift dispersion or radiofrequency (rf) variations due to imperfections such as rf inhomogeneity is also explained. 相似文献
83.
Velan SS 《Journal of magnetic resonance (San Diego, Calif. : 1997)》2004,171(2):40-352
Longitudinal multispin orders provide an effective way for measurement of scalar couplings and also to probe molecular interactions and dynamics. Analysis of longitudinal orders has been made in strongly coupled AB and ABX spin systems to determine the dependence of strong coupling parameter on these orders. Experimental and simulated spectra of various longitudinal orders are illustrated for these spin systems. This general procedure can be extended to broad range of spin systems to understand the influence of strong coupling on longitudinal orders. 相似文献
84.
B. Macke B. Ségard 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2003,23(1):125-141
This paper deals with the apparent superluminal propagation of electromagnetic pulses in a linear dispersive medium. One specifically
examines the possibility that the pulse leaving the medium may be nearly identical to the incident one (low distortion) and
in significant advance of it (strongly negative group-delays). Favourable conditions are obtained in a dilute medium where
the required anomalous dispersion originates in an ensemble of narrow absorption or gain lines. Analytical expressions of
the advancement of the pulse centre-of-gravity and of the lowest order distortion are established from the transfer-function
of the medium. The experiments already achieved with arrangements involving a single absorption-line or a gain-doublet are
analysed in detail and compared. The considerable difficulties to overcome in order to attain advancements comparable to the
pulse width without important distortion are pointed out. New and promising schemes involving a narrow dip in a gain profile
or absorption-doublets are proposed.
Received 4 July 2002 / Received in final form 8 November 2002 Published online 4 February 2003
RID="a"
ID="a"e-mail: bruno.macke@univ-lille1.fr
RID="b"
ID="b"Unité Mixte de Recherche de l'Université et du CNRS (UMR 8523) 相似文献
85.
Iuga D Schäfer H Verhagen R Kentgens AP 《Journal of magnetic resonance (San Diego, Calif. : 1997)》2000,147(2):192-209
We have recently shown that the sensitivity of single- and multiple-quantum NMR experiments of half-integer (N/2) quadrupolar nuclei can be increased significantly by introducing so-called double frequency sweeps (DFS) in various pulse schemes. These sweeps consist of two sidebands generated by an amplitude modulation of the RF carrier. Using a time-dependent amplitude modulation the sidebands can be swept through a certain frequency range. Inspired by the work of Vega and Naor (J. Chem. Phys. 75, 75 (1981)), this is used to manipulate +/-(m - 1) <--> +/-m (3/2 < or = m < or = N/2) satellite transitions in half-integer spin systems simultaneously. For (23)Na (I = 3/2) and (27)Al (I = 5/2) spins in single crystals it proved possible to transfer the populations of the outer +/-m spin levels to the inner +/-1/2 spin levels. A detailed analysis shows that the efficiency of this process is a function of the adiabaticity with which the various spin transitions are passed during the sweep. In powders these sweep parameters have to be optimized to satisfy the appropriate conditions for a maximum of spins in the powder distribution. The effects of sweep rate, sweep range, and RF field strength are investigated both numerically and experimentally. Using a DFS as a preparation period leads to significantly enhanced central transition powder spectra under both static and MAS conditions, compared to single pulse excitation. DFSs prove to be very efficient tools not only for population transfer, but also for coherence transfer. This can be exploited for the multiple- to single-quantum transfer in MQMAS experiments. It is demonstrated, theoretically and experimentally, that DFSs are capable of transferring both quintuple-quantum and triple-quantum coherence into single-quantum coherence in I = 5/2 spin systems. This leads to a significant enhancement in signal-to-noise ratio and strongly reduces the RF power requirement compared to pulsed MQMAS experiments, thus extending their applicability. This is demonstrated by (27)Al 3QMAS experiments on 9Al(2)O(3). 2B(2)O(3) and the mineral andalusite. In the latter compound, Al experiences a quadrupolar-coupling constant of 15.3 MHz in one of the sites. Finally a 5QMAS spectrum on 9Al(2)O(3). 2B(2)O(3) demonstrates the sensitivity enhancement of this experiment using a double frequency sweep. 相似文献
86.
提出了实时条件下裸手单目的手部定位和跟踪算法。结合改进的差分法提出了实用的手部约束条件,从每帧图像中提取手部图像,确定感兴趣区域(ROI,region of interesting),得到较为满意的手部分割结果,再对手部图像特征进行深入分析和提取,利用改进的相干映射算法(VCM,vector coherence mapping)进行跟踪,针对手的运动增加了约束,保证了顽健性。在这个基础上,提出了时间相关的运动预测模型,满足了实时性的要求,保证前后分析结果的一致性。实验结果证明,在不同光照和复杂背景下系统有最高达99%的识别率,与已有的系统相比,性能显著提高。 相似文献
87.
88.
K. Jin Z. C. Wang Q. Zhang 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2007,42(2):325-332
We study the absorption spectra of a degenerate V-type
atom, where a resonant driving field and a probe field drive
different branches of transitions and a dc field is applied to
drive the transition between two excited states. The effects of
vacuum induced coherence (VIC) on the absorption spectra are
investigated. It is demonstrated that in some special cases the
VIC can lead to the depression of absorption and narrow resonance.
The origin of these features are discussed. When the pump field
and the dc field have the same intensity, it is interesting to
find that the whole absorption spectrum comes mainly from the
absorptions induced by the interferences among different
transitions between dressed states. 相似文献
89.
A simple method to measure the complex degree of spatial coherence of a partially coherent quasi-monochromatic light field is presented. The Fourier spectrum of the far-field interferogram generated by a mask with multiple apertures (small circular holes) is analyzed in terms of classes of aperture pairs. A class of aperture pairs is defined as the set of aperture pairs with the same separation vector. The height of the peaks in the magnitude spectrum determines the modulus of the complex degree of spatial coherence and the corresponding value in the phase spectrum determines the phase of the complex degree of spatial coherence. The method is illustrated with experimental results. 相似文献
90.
A method of contrast enhancement of optical coherence tomography (OCT) images based on least squares fitting and histogram matching is presented. Several different functions are adopted as the probability density functions of the gray levels to fit the normalized histogram of an OCT image and histogram matching is used to enhance the OCT image automatically. The effectiveness of the method is proved by the experimental results. 相似文献