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The effect of vibrational excitation of HBr on the H+HBrH2+Br and H+HBrH+HBr reactions has been investigated on the extended LEPS surface (ELEPS) constructed on the basis of quantum chemically calculated points of PES. Together with this surface the LEPS surface of Sudhakaran and Raff [1] was used for comparison at two relative translational energies. A quasiclassical trajectory method was used to study the abstraction and exchange reaction dynamics. The reactive cross section was calculated as a function of the relative collision energy and the vibrational state of HBr. The following conclusions can be drawn from the results of the study: (i) vibrational excitation v=0 v=2 more than doubles the reaction cross section, (ii) the increase in the collision energy is most effectively channelled into the product translational energy.Dedicated to Professor J. Koutecký on the occasion of his 65th birthday 相似文献
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Laser Doppler anemometry is used for the measurements of the plasma and particle velocity profiles in the coil region of an inductively coupled r.f. plasma. Results are reported for a 50 mm i.d. induction plasma torch operated at atmospheric pressure with argon as the plasma gas. The oscillator frequency is 3 MHz and the plate power is varied between 4.6 and 10.5 kW. Plasma velocity measurements are obtained using a fine carbon powder as a tracer. Measurements are also given for larger silicon particles (
) centrally injected into the discharge under different operating conditions.Nomenclature
d
p
particle diameter
-
P
0
plasma power
-
Q
1
powder carrier gas flow rate
-
Q
2
plasma gas flow rate
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Q
3
sheath gas flow rate
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r
distance in the radial direction
-
V
axial plasma velocity
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V
p
axial particle velocity
-
Z
distance in the axial direction
-
standard deviation 相似文献
15.
Human activity prediction has become increasingly valuable in many applications. This paper, initially from the perspective of cognition science, presents a novel approach to learning a hierarchical spatio-temporal pattern of human activities to predict ongoing activities from videos that contain only the onsets of the activities. Spatio-temporal pattern can be learned by a Hierarchical Self-Organizing Map (HSOM), which consists of two self-organizing maps (i.e., action map and actionlet map) connected via associative links trained by Hebbian learning. Ongoing activities can be predicted by Variable order Markov Model (VMM), which provides the means for capturing both large and small order Markov dependencies based on the training actionlet sequences. Experiments of the proposed method on four challenging 3D action datasets captured by commodity depth cameras show promising results. 相似文献
16.
《Journal of Location Based Services》2013,7(4):268-284
Tourist recommendation services provide suggestions for places of interest. While the spatial structure of a tourist's visit has been successfully exploited to improve the quality of place recommendations, its temporal structure has not been taken into account so far. This is surprising because the importance of the visitors' time management is well known from tourism research. We present findings of an empirical study that sheds light on the temporal aspects of tourist exploration behaviour and discuss implications for the design of tourist-recommender systems. The data-set consists of interviews, GPS tracks and geo-referenced photo sequences from visitors of a typical Middle European destination for cultural tourism. Among the results relevant to place recommending are the following: (1) the set of places is often replanned during the visit; (2) comparing place popularity based on photo frequency and place popularity based on staying time, we found notable differences in rank ordering; and (3) the photo frequency and the detour sinuosity of the GPS tracks are decreasing slowly over time. We interpret this last finding as a time-geographic cone effect. Based on the empirical results, we discuss the implications for the design of tourist-recommending services and propose a corresponding user interface utilising a recommendation strategy that tries to counterbalance the time-geographic cone effect, that is, to decelerate the visiting experience. 相似文献
17.
针对履带式移动机器人的轨迹跟踪控制问题进行研究,首先,建立了履带式移动机器人的运动学模型和跟踪误差模型;其次,设计了转速有限时间控制和线速度滑模控制的轨迹跟踪控制律,并给出了考虑运动受限作用下的控制律修正表达式;最后,基于MATLAB对所提控制律进行仿真,对比分析了不考虑运动受限情况下跟踪控制效果;结果表明,设计的跟踪控制律能够实现履带式移动机器人对圆轨迹的有效跟踪,且考虑运动受限作用的控制律更加符合实际;文章研究分析了运动受限作用对于移动机器人轨迹跟踪控制的影响,分析结果对其他移动机器人的运动控制研究具有参考价值。 相似文献
18.
Thordis L. Thorarinsdottir Michael Scheuerer Christopher Heinz 《Journal of computational and graphical statistics》2016,25(1):105-122
Any decision-making process that relies on a probabilistic forecast of future events necessarily requires a calibrated forecast. This article proposes new methods for empirically assessing forecast calibration in a multivariate setting where the probabilistic forecast is given by an ensemble of equally probable forecast scenarios. Multivariate properties are mapped to a single dimension through a prerank function and the calibration is subsequently assessed visually through a histogram of the ranks of the observation’s preranks. Average ranking assigns a prerank based on the average univariate rank while band depth ranking employs the concept of functional band depth where the centrality of the observation within the forecast ensemble is assessed. Several simulation examples and a case study of temperature forecast trajectories at Berlin Tegel Airport in Germany demonstrate that both multivariate ranking methods can successfully detect various sources of miscalibration and scale efficiently to high-dimensional settings. Supplemental material in form of computer code is available online. 相似文献
19.
ABSTRACTNewton trajectories are used for the Frenkel–Kontorova model of a finite chain with free-end boundary conditions. We optimise stationary structures, as well as barrier breakdown points for a critical tilting force were depinning of the chain happens. These special points can be obtained straight forwardly by the tool of Newton trajectories. We explain the theory and add examples for a finite-length chain of a fixed number of 2,?3,?4,?5 and 23 particles. 相似文献
20.