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751.
Spatial encoding is a particular kind of spin manipulation that enables the acquisition of multidimensional NMR spectra within a single scan. This encoding has been shown to possess a general applicability and to enable the completion of arbitrary nD NMR acquisitions within a single transient. The present study explores its potential towards the acquisition of 2D DOSY spectra, where the indirect dimension is meant to encode molecular displacements rather than a coherent spin evolution. We find that in its simplest form this extension shows similarities with methods that have been recently discussed for the single-scan acquisition of this kind of traces; still, a number of advantageous features are also evidenced by the “ultrafast” modality hereby introduced. The principles underlying the operation of this new single-scan 2D DOSY approach are discussed, its use is illustrated with a variety of sequences and of samples, the limitations of this new experiment are noted, and potential extensions of the methodology are mentioned. 相似文献
752.
753.
The properties of the asymptotic AdS3 space–times representing flat domain walls (DW's) solutions of the new massive 3D gravity with scalar matter are studied. Our analysis is based on first order BPS-like equations involving an appropriate superpotential. The Brown–York boundary stress-tensor is used for the calculation of DW's tensions as well as of the CFT2 central charges. The holographic renormalization group flows and the phase transitions in specific deformed CFT2 dual to 3D massive gravity model with quadratic superpotential are discussed. 相似文献
754.
《Particuology》2023
The mechanisms of new particle formation (NPF) events that occurred under high aerosol loadings (“polluted” NPF) in the atmosphere have been unclear, which has inhibited the precision of particle pollution control. To deepen the understanding of how the “polluted” NPF events occur, a one-month comprehensive measurement was conducted in the atmosphere of Beijing during the summer of 2016. The “clean” NPF events (frequency = 22%) (condensation sink, CS < 0.015 s−1) were found to be caused by local nucleation and growth. The “polluted” NPF events (frequency = 28%) (CS > 0.015 s−1) were influenced by both local nucleation-growth and regional transport, and the contributions from the two factors to 6–25 nm particle number concentration were 60% and 40%, respectively. This study emphasized the importance of the transport for nanoparticles in relatively polluted atmospheres, and for that the regional joint particle pollution control would be an essential policy. 相似文献