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31.
Guo-Hua Zhong Chao Zhang Xunwang Yan Xiaoguang Li Zheng Du Gexin Jing 《Molecular physics》2017,115(4):472-483
Polycyclic aromatic hydrocarbons doped by metal have exhibited the potential of high temperature superconductivity. Understanding the basic properties of materials is the key to reveal the superconductivity. Here, a systemically theoretical study has been done to explore crystal structures and electronic properties of pristine and potassium-doped 1,2;8,9-dibenzopentacene, compared with [7]phenacenes case. We determined that vdW-DF2 functional is more suitable to describe the non-local interaction in a molecular crystal. Based on this functional, we predicted the crystal structures and investigated in detail the K atomic positions in a system. It was found that the intralayer doping leads to lower total energy. From the calculated formation energy, for each 1,2;8,9-dibenzopentacene molecule, the doping of two electrons is more stable under the relatively K-poor condition while the doping of four electrons is more stable under the K-rich condition. Between these two phases, the three-electron doping phase stabilises in a narrow region of K chemical potential. Combining with the electronic states at Fermi level, we analysed the reasons of superconductivity enhancement in doped 1,2;8,9-dibenzopentacene. This work further deepens the understanding of 1,2;8,9-dibenzopentacene superconductor. 相似文献
32.
从二维系统的Kosterlitz-Thouless (KT) 相变理论出发,在关联长度中引入热激活能和平均钉扎高度,提出了修正的KT相变模型.该模型与库伦气体标度理论和Halperin-Nelson关系具有一致性.应用修正的KT相变模型研究磁场下Tl2Ba2CaCu2Ox(Tl-2212)薄膜电阻转变的标度行为,发现由电阻转变计算得到的平均钉扎高度与温度具有线性依赖关系,实验结果支持修正的KT相变模型.
关键词:
标度行为
各向异性超导体
电阻转变 相似文献
33.
Time differential perturbed angular correlation measurements of the 133–482 keVγ-γ cascade of181Ta in Hf-doped YBa2Cu3O7−x
are presented. The181Hf precurser nuclei are incorporated into the sample by thermal neutron irradiation. Two quadrupole interaction frequencies
are observed in the as-irradiated sample:v
Q1=161±10 MHz with intensityf
1=75%, asymmetry parameterη
1=0.32 and damping parameter Λ1=0.42, andv
Q2=1108±40 MHz withf
2=25%,η
2=0.62, and Λ2=0.60. On annealing the sample in air at various temperaturesT
a and quenching to room temperature,f
1 remained nearly constant forT
a<600°C andv
Q1 for all annealing temperatures indicating that these are insensitive to oxygen stoichiometry. This frequency is interpreted
to be due to181Hf substitutingY sites. BeyondT
a=600°C,f
1 increased and reached a constant value of 90% forT
a=800°C. The value ofv
Q2 showed a slight variation between 1086 and 1160 MHz, whilef
2 remained nearly constant at 25% forT
a<600°C. This component is identified to be due to181Hf substituting Cu 1 sites in the Cu-O chains of YBCO. Above 600°Cv
Q2 decreased and reached a value of 808 MHz beyond 750°C. 相似文献
34.
Film preparation of oxide superconductors, mainly of the 1-2-3 (RBa2Cu3Ox) and Bi-containing (Bi-Sr-Ca-Cu-O) systems, by evaporation of either metals or metal compounds by low pressure is summarized, with a particular focus on the development of oxidation sources essential to the technique. Oxidizing reagents that enable the oxidation of metal evaporates to take place in high (0·1 to 10?3 Pa) or even ultra-high (<10?5 Pa) vacuum are summarized using the experiments of those who tried to apply the molecular beam epitaxy method to atomically controlled fabrication of thin films of the material, especially for device processing. The evaporation in various kinds of oxidizing atmosphere, including the simple method of in situ annealing of the metal layers in oxygen to the more advanced in situ preparation of the films with strong oxidizing reagents such as atomic oxygen, ozone, nitric oxide, etc. along with the thermochemistry of the oxidation of metals by low pressure with these reagents is reviewed. 相似文献
35.
36.
We have studied the tunneling conductance in ferromagnet/insulator/p-wave superconductor junctions, taking into account the
rough interface scattering effect. We find that there exist zero-bias conductance peaks and single-minimum structure in tunneling
spectroscopy. As the exchange energy increases, the Andreev reflection is always suppressed and the differential conductance
decreases. The differential conductance depends on the barrier strength and the roughness at the interface.
Supported by the Natural Science Foundation of Jiangsu Higher Education Institutions, China (Grant No. 06KJB140009) 相似文献
37.
三电平大功率并联逆变电源在EAST系统中的应用 总被引:1,自引:0,他引:1
针对EAST超导托卡马克装置中的等离子体位移快控电源大电流快速响应的要求,采用三电平结合移相PWM多重化技术,实现多组变流器并联运行,提高了变流器的等效开关频率控制性能,从而改善了电流波形品质。分析了快控电源系统的设计方案和控制方法,并针对移相PWM多重化技术,采用Matlab进行了仿真,验证了设计思想。实验结果表明,该系统设计方案合理、控制策略有效,具备良好的大电流输出和快速响应能力。 相似文献
38.
Aram A. Sahakyan Sergei K. Nikoghosyan Hrant N. Yeritsyan 《Central European Journal of Physics》2008,6(4):797-801
The influence of irradiation by electrons with an energy of 8 MeV, at dose intervals between 1013 and 2×1018el/cm2, on the properties of impurity doped, high-temperature superconductor YBa2Cu3−x
M
x
O
y
(M = Fe, Ni; x=0; x=0:01) ceramics has been studied.
It has been established that, as the irradiation dose is increased, the onset temperature of the transition to the superconducting
state (T
c
on
), and the intergranular weak link coupling temperature between granules (T
m
J
), exhibit an oscillation around their initial values of approximately about 1–1.5 K. This oscillation indicates that the
process of radiation defect formation in HTSC occurs in multiple stages. It was also found that the critical current (J
c
)decreases with an increase of the irradiation dose, and exhibits a local minimum at a dose of 8×1016el/cm2coinciding with minima for T
c
on
and T
m
J
at this dose. It was found that the introduction of Fe atoms to the ceramic decreases T
m
J
, while introducing Ni atoms decreases both T
c
on
and T
m
J
; it is suggested that this is a result of Ni substitution of Cu both in Cu2 plane sites and Cu1 chain sites. The introduction
of Ni causes a large change in the intergranular critical current density, J
c
. A critical irradiation dose is obtained (2×1018)after which all HTSC parameters strongly decrease, i. e. the superconductivity of HTSC is destroyed.
相似文献
39.
Physical properties of titanates,semiconductors and nickelates derived from ionization energy theory
《Physics letters. A》2020,384(36):126917
Ionization energy theory is exploited to predict the changes to atomic polarizability for both anions and cations, the polarization in doped titanates and the energy gap in III–V and II–VI semiconductors. We then extend the above analysis to discuss the physics of metallic and superconducting phases in the recently discovered superconducting nickelates. In doing so, we are able to prove the existence of Ni2+ cations and oxygen vacancy in the metallic normal state of nickelates. We find that the normal state resistivity of the nickelates follows exactly as predicted by the ionization energy theory. Quantitative estimates are also given for the concentrations of Ni2+ and oxygen vacancy in superconducting nickelates. 相似文献
40.
太赫兹(THz)波段一般定义为0.1–10 THz的频率区间, 对应波长范围3 mm–30 μm, 覆盖短毫米波至亚毫米波段(远红外). 尽管人们早已认识到太赫兹波段具有非常重要的科学意义和广泛的应用前景, 但该波段仍然是一个有待全面研究和开发的电磁频率窗口. 因此, 太赫兹波段的天文观测在天体物理及宇宙学研究中具有不可替代的作用, 对于理解宇宙状态和演化具有非常重要的意义. 具有超高灵敏度的太赫兹超导探测器, 已经成为太赫兹波段观测的主要手段. 本文主要阐述了太赫兹超导探测器的基本类型和工作原理, 以及中国科学院紫金山天文台在该领域的主要研究成果和进展. 相似文献