Kinetics of dark excitons and excitonic trions in InGaAs single quantum well

Magnetooptical studies performed on a wide InGaAs/GaAs single quantum well indicate that optically non-active (dark) excitons with total angular momentum play the role of a reservoir for the creation of free multiparticle excitonic complexes. After analyzing the magnetic field evolution of the circularly polarized components of the low energy structure appearing in the main excitonic luminescence line we assign this feature to the excitonic trion formation. The binding energy of the excitonic trions was estimated to be of the order of 1 meV. Received: 29 October 1997 / Received in final form: 20 February 1998 / Accepted: 21 February 1998     

Magnetic susceptibility, heat capacity, and optical conductivity of LiPc and LiPcI

The magnetic susceptibility, using dc and electron spin resonance (ESR) methods, the specific heat, and the infrared properties of the one-dimensional molecular semiconductors lithium phthalocyanine (LiPc) and the iodinated compound LiPcI have been investigated for temperatures K. LiPc has a half-filled conduction band and is expected to be an organic metal. However, due to the strong Coulomb repulsion the system is a one-dimensional Mott-Hubbard insulator with a Hubbard gap of 0.75 eV as inferred from optical measurements. The localized electrons along the molecular stacks behave like a S = 1/2 antiferromagnetic spin chain. The spin susceptibility, as determined by ESR experiments, and the magnetic contribution to the heat capacity show a Bonner-Fisher type of behavior with an exchange constant K. LiPcI is an intrinsic narrow-gap semiconductor with an optical gap of 0.43 eV. In ESR experiments it is silent, indicating that all the unpaired electrons have been removed from the macrocycle via doping with iodine. Received: 16 June 1998 / Accepted: 14 July 1998     

Finite Range of Large Perturbations in Hamiltonian Dynamics

The dynamics defined by the Hamiltonian , where the _m are fixed random phases, is investigated for large values of A, and for . For a given P ^* and for , this Hamiltonian is transformed through a rigorous perturbative treatment into a Hamiltonian where the sum of all the nonresonant terms, having a Q dependence of the kind cos(kQ – nt + _m) with \Delta \upsilon$$ " align="middle" border="0"> , is a random variable whose r.m.s. with respect to the _m is exponentially small in the parameter . Using this result, a rationale is provided showing that the statistical properties of the dynamics defined by H, and of the reduced dynamics including at each time t only the terms in H such that , can be made arbitrarily close by increasing . For practical purposes close to 5 is enough, as confirmed numerically. The reduced dynamics being nondeterministic, it is thus analytically shown, without using the random-phase approximation, that the statistical properties of a chaotic Hamiltonian dynamics can be made arbitrarily close to that of a stochastic dynamics. An appropriate rescaling of momentum and time shows that the statistical properties of the dynamics defined by H can be considered as independent of A, on a finite time interval, for A large. The way these results could generalize to a wider class of Hamiltonians is indicated.     

Ground-state complex formation of perylene with pyromellitic dianhydride studied by static fluorescence quenching

The association of complex formation with static quenching in CT systems was investigated. Evaluation of the data made evident that the inner filter effect must be allowed for. Time-resolved and temperature-dependent stationary measurements of fluorescence led to the separation of dynamic and static quenching components. The static quenching constant is discussed with respect to the equilibrium constant of complex formation determined by absorption spectroscopy.     

Ferromagnetic ground state in the Kondo lattice model

We present a series of rigorous examples of the Kondo lattice model that exhibit full ferromagnetism in the ground state. The models are defined in one-, two- and three-dimensional lattices, and are characterized by a range of hopping terms, specific electron filling, and large ferromagnetic coupling. Our examples show that a sufficient strong but finite exchange coupling between conduction electrons and localized spins could overcome the competition from mobility of a finite density of electrons and drive the system from a paramagnetic phase to a ferromagnetic phase. We also establish a relation of ferromagnetism between the Hubbard model and Kondo lattice model. Meanwhile some rigorous results on ferromagnetism in the corresponding Hubbard model are presented. Received: 10 September 1997 / Revised: 15 October 1997 / Accepted: 17 October 1997     

Resonant magnetopolaron effects in GaAs/AlGaAs multiple quantum well structures

A detailed experimental study of electron cyclotron resonance (CR) has been carried out at 4.2 K in three modulation-doped GaAs/Al_0.3Ga_0.7As multiple quantum well samples in fields up to 30 T. A strong avoided-level-crossing splitting of the CR energies due to resonant magnetopolaron effects is observed for all samples near the GaAs reststrahlen region. Resonant splittings in the region of AlAs-like interface phonon modes of the barriers are observed in two samples with narrower well width and smaller doping concentration. The interaction between electrons and the AlAs interface optical phonon modes has been calculated for our specific sample structures in the framework of the memory-function formalism. The calculated results are in good agreement with the experimental results, which confirms our assignment of the observed splitting near the AlAs-like phonon region is due to the resonant magnetopolaron interaction of electrons in the wells with AlAs-like interface phonons.     

用玻色子组态混合和玻色子表面δ相互作用研究核谱

用玻色子组态混合波函数和玻色子表面δ相互作用研究了三玻色子核⁴⁶Ti和⁵⁴Cr的sdgIBMI的能谱和E2跃迁概率,理论计算结果令人满意,比sdIBMI能拟合出更多的能级和E2跃迁概率,而且它们的误差更小. 说明g玻色子在振动区也起着重要的作用,同时进一步证明了这种玻色子组态混合模型是成功的.     

The intermediate regime of light diffraction by ultrasound in planar gyrotropic optical waveguides in an external electric field

A theoretical investigation is carried out for an intermediate regime of optoacoustic interaction, close to the Bragg one, by ultasonic Rayleigh surface waves in gyrotropic planar waveguides in an external electric field. A system of equations of associated waves is presented which describes the planar optoacoustic interaction in intermediate, Raman—Nath, and Bragg regimes of diffraction by ultrasonic surface waves in gyrotropic crystals with electrically induced anisotropy. It is shown that the intermediate (transition) regime of optoacoustic interaction, which is characterized by an angular selectivity and by the presence of several diffraction maxima, is the basic regime of diffraction. In this case diffracted light is generally elliptically polarized with an ellipticity and polarization azimuth that depend on the external electric field intensity. Translated from Zhurrnal Prikladnoi Spektroskopii, Vol. 66, No. 1, pp. 30–35, January–February, 1999.     

Problems of the electronic structure of nonmetals in a wide energy region of fundamental absorption (review)

The article surveys the main unsolved problems of the electronic structure of nonmetals in a wide energy region of fundamental absorption. Udmurtia State University, 71, Krasnogeroiskaya Str., Izhevsk, 426034, Russia. Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 66, No. 3, pp. 299–315, May–June, 1999.     

On the Specific Heat of Fermi–Pasta–Ulam Systems and Their Glassy Behavior

The specific heat of Fermi–Pasta–Ulam systems has until now been estimated through the energy fluctuations of a suitable subsystem, and opposite answers were apparently provided concerning its possible vanishing for vanishing temperatures. In the present paper a more realistic numerical implementation of the specific heat measurement is discussed, which mimics the interaction of the FPU system with a calorimeter. It is found that there exists a freezing critical temperature below which the relaxation times to equilibrium between FPU system and calorimeter become relevant, so that the system presents aging and hysteresis features very similar to those familiar in glasses and spin glasses. In particular, in the framework of such a point of view involving finite long times, the specific heat appears to vanish for vanishing temperatures.