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31.
H. Langguth H.-U. Försterling J. Schmidt 《Isotopes in environmental and health studies》2013,49(10):342-344
Die Strahlenresistenz von reinem und an Aktivkohle sorbiertem Dimethylglyoxim (DMG), das für die selektive Abtrennung von Palladium aus Abfallösungen der Kernbrennstoffwiederaufarbeitung geeignet ist, wurde untersucht. Die Bestrahlung erfolgte bei 20–40 °C mit einer 60Co-γ-Bestrahlungsanlage mit Dosisleistungen von 0,6 bis 1,7 Gy/s in einem Dosisbereich von 2 kGy bis 5 MGy. Die Radiolyseprodukte wurden mit verschiedenen Methoden analysiert und die G-werte bestimmt. Es wurde gezeigt, daβ DMG bis zu Dosen von etwa 110 kGy relativ strahlenresistent ist. Bei höheren Dosen werden die reaktiven NOH-Gruppen des DMG teilweise zerstört, so daβ sie nicht mit Palladium reagieren können. In Verfahren zur Abtrennung von Palladium aus radioaktiven Abfallösungen werden diese Dosen jedoch nicht erreicht. Auf eine unzureichende Strahlenresistenz von DMG zurückzuführende Komplikationen können deshalb ausgeschlossen werden. 相似文献
32.
Dietmar Weiss 《Isotopes in environmental and health studies》2013,49(3):254-264
Extensive investigations on radioactive contamination and on its spatial and temporal changes in the Baltic Sea have been carried out by the National Board for Atomic Safety and Radiation Protection since 1986. The results were compared with data obtained in the years prior to the Chernobyl accident. Due to the composition of the accidental releases and the physical half-life of the released radionuclides, special emphasis was laid on Cs-134 and Cs-137. Other radionuclides, such as H-3, Sr-90, Ru-103 and Ru-106 turned out to be insignificant compared with the caesium isotopes. The radionuclides Cs-134 and Cs-137 accounting for the highest percentage of the released long-lived radionuclides were deposited on the sea surface with an initial ratio of 0.5. Their distribution pattern on the sea surface was affected by the meteorological conditions prevailing during the release period. The horizontal dislocation of higher contaminated water masses and the vertical penetration of radioactive caesium resulted in a prolonged uniformity of the contamination level of the Baltic Sea. 相似文献
33.
We have used vibrational spectroscopy to study the formula and molecular structure of the mineral penkvilksite Na 2TiSi 4O 11·2H 2O. Penkvilksite is a mineral which may be used in the uptake of radioactive elements. Both Raman and infrared spectroscopies identify a band at ~3638 cm?1 attributed to an OH-stretching vibration of hydroxyl units. The inference is that OH units are involved in the structure of penkvilksite. The formula may be well written as Na 2TiSi 4O 10(OH)2·H 2O. The mineral is characterised by a very intense Raman band at 1085 cm?1 and a broad infrared band at 1080 cm?1 assigned to SiO-stretching vibrations. Raman bands at 620, 667 and 711 cm?1 are attributed to SiO and TiO chain bonds. Water-stretching vibrations are observed as Raman bands at 3197, 3265, 3425 and 3565 cm?1. Vibrational spectroscopy enables aspects of the molecular structure of the mineral penkvilksite to be ascertained. Penkvilksite is a mineral which can incorporate actinides and lanthanides from radioactive waste. 相似文献
34.
Manuel A.P. Segurado Margarida F.B. Silva Rita Castro 《International Journal of Mathematical Education in Science & Technology》2013,44(5):664-679
The mathematical language and its tools are complementary to the formalism in chemistry, in particular at an advanced level. It is thus crucial, for its understanding, that students acquire a solid knowledge in Calculus and that they know how to apply it. The frequent occurrence of indeterminate forms in multiple areas, particularly in Physical Chemistry, justifies the need to properly understand the limiting process in such cases. This article emphasizes the importance of the L’Hôpital's rule as a practical tool, although often neglected, to obtain the more common indeterminate limits, through the use of some specific examples as the radioactive decay, spectrophotometric error, Planck's radiation law, second-order kinetics, or consecutive reactions. 相似文献
35.
36.
Jerzy Falandysz Michał Saniewski Tamara Zalewska Ji Zhang 《Isotopes in environmental and health studies》2019,55(3):317-324
Amanita muscaria collected from a forested area in northern Poland in 2015 were analysed for activity concentrations of 137Cs and 40K. Total K concentration values were calculated from 40K data. Mushrooms were grouped in six fruiting bodies size classes regarding to their developmental stage. The 137Cs activity concentrations declined in A. muscaria as the fruiting bodies maturated. The contents of 40K/K activity remained constant in caps at different developmental stage, while for stipes an increase was around twofold (40K from 925?±?55 Bq kg?1 dry biomass in the baby individuals and 1600?±?63–1700?±?53 Bq kg?1 dry biomass in two oldest classes). A. muscaria is a weak accumulator of 137Cs, while a steep drop in activity concentrations of this nuclide in the fruiting bodies as they maturate has not been reported earlier for mushrooms. Clearly, a fate of 137Cs in A. muscaria is highly different from that of 40K/K that is an essential element to fungi. In parallel, an observed increase in the content of 40K/K in stipes of fruiting bodies with developmental state can be related to its ‘hardening’ and more fibrous nature with age and basic function to support the cap, but this has not been studied. 相似文献
37.
J Benlliure S Steinhäuser C Böckstiegel A Grewe H-G Clerc A heinz M de Jong A R Junghans J Müller K-H Schmidt M Pfützner 《Pramana》1999,53(3):637-646
Nuclear fission from excitation energies around 11 MeV was studied at GSI, Darmstadt for 76 neutron-deficient actinides and
pre-actinides by use of relativistic secondary beams. The characteristics of multimodal fission of nuclei around 226Th are systematically investigated and related to the influence of shell effects on the potential-energy and on the level
density between saddle point and scission. A systematic view on the large number of elemental yields measured gave rise to
a new interpretation of the enhanced production of even elements in nuclear fission and allowed for a new understanding of
pair breaking in fission. 相似文献
38.
D. Habs O. Kester T. Sieber H. Bongers S. Emhofer P. Reiter P.G. Thirolf G. Bollen J. Aystö O. Forstner H. Ravn T. Nilsson M. Oinonen H. Simon J. Cederkall F. Ames P. Schmidt G. Huber L. Liljeby O. Skeppstedt K.G. Rensfelt F. Wenander B. Jonson G. Nyman R. von Hahn H. Podlech R. Repnow C. Gund D. Schwalm A. Schempp K.-U. Kühnel C. Welsch U. Ratzinger G. Walter A. Huck K. Kruglov M. Huyse P. Van den Bergh P. Van Duppen L. Weissman A.C. Shotter A.N. Ostrowski T. Davinson P.J. Woods J. Cub A. Richter G. Schrieder 《Hyperfine Interactions》2000,129(1-4):43-66
The Radioactive Beam Experiment REX-ISOLDE [1–3] is a pilot experiment at ISOLDE (CERN) testing the new concept of post acceleration
of radioactive ion beams by using charge breeding of the ions in a high charge state ion source and the efficient acceleration
of the highly charged ions in a short LINAC using modern ion accelerator structures. In order to prepare the ions for the
experiments singly charged radioactive ions from the on-line mass separator ISOLDE will be cooled and bunched in a Penning
trap, charge bred in an electron beam ion source (EBIS) and finally accelerated in the LINAC. The LINAC consists of a radiofrequency
quadrupole (RFQ) accelerator, which accelerates the ions up to 0.3 MeV/u, an interdigital H-type (IH) structure with a final
energy between 1.1 and 1.2 MeV/u and three seven gap resonators, which allow the variation of the final energy. With an energy
of the radioactive beams between 0.8 MeV/u and 2.2 MeV/u a wide range of experiments in the field of nuclear spectroscopy,
astrophysics and solid state physics will be addressed by REX-ISOLDE.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
39.
本总结了中能重离子碰撞产生同位素分布的计算方法和模型,包括参数化公式,擦碎模型和统计擦碎模型。介绍了模型的物理基础和计算方法,并讨论了对擦碎模型和统计擦碎模型的修正。同时用统计擦碎模型探讨了碎裂瓜在产生的同位素分布的同位旋效应。然后介绍了放射性核束的产生方法,并对放射性束流物理的发展前景作了简要介绍。 相似文献
40.
质量是原子核的基本性质之一,在核物理和核天体物理中都有重要的应用。原子核质量测量是目前核物理研究的一个前沿热点课题,国际上各个核物理实验室积极发展新设备和新技术,在短寿命放射性核素测量和超高精度质量测量方面取得了重要进展,本文对此进行了总结评述。在兰州重离子加速器冷却储存环(HIRFL-CSR)上利用等时性质量谱仪测量了一些原子核的质量,本文对其在测量精度、核态最短寿命等前沿进展做了简要介绍,并介绍了正在发展的双飞行时间质量谱仪。原子质量评估收集所有与原子核质量相关的实验数据,经过评估后推荐出质量值及相应误差。原子质量评估AME2016于2017年3月发表,为科技工作者提供基准数据。Mass is a fundamental property of the atomic nucleus. Nuclear mass data play an important role in nuclear physics and nuclear astrophysics. Thanks to the developments of novel mass spectrometers and radioactive nuclear beam facilities, the experimental knowledge of nuclear masses has been continuously expanding along two main directions, including:measurements aimed at high-precision mass values and at the most exotic nuclei far from the stability. The latest progress are reviewed in the paper. In the past few years, mass measurements of short-lived nuclides were performed using isochronous mass spectrometry based on the Cooler Storage Ring at the Heavy Ion Research Facility in Lanzhou(HIRFL-CSR). The progresses on the frontiers of short half-life and high precision are introduced. The Atomic Mass Evaluation (AME) is the most reliable source for the comprehensive information related to the atomic (nuclear) masses. The latest version of the AME, i.e., AME2016, was published in March, 2017, serving the research community with the benchmark data. 相似文献