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184.
Frédéric André Rodolphe Vaillon Hongsheng Guo 《Journal of Quantitative Spectroscopy & Radiative Transfer》2011,112(3):394-411
A Multi-Spectral Reordering (MSR) scheme is introduced to improve the performances of the Spectral-Line Moment-Based (SLMB) modeling for the handling of full spectrum radiative heat transfer calculations in nonuniform media. Using this simultaneous reordering of the spectrum for several thermophysical conditions together with employing approximate formulations to evaluate path-averaged transmission functions for nonisothermal and nonhomogenous gaseous paths, a novel full spectrum gas radiation modeling method in nonuniform gaseous mixtures is constituted. The method is presented in details as well as the building of associated databases for CO2 and H2O at atmospheric pressure and for the temperature range of 300-2700 K. The new model is validated against line-by-line reference computations for a series of existing benchmarks and for a flame configuration. The MSR-SLMB modeling is shown to perform accurately and better than the standard SLMB one, while involving reasonable additional computational costs. 相似文献
185.
The astrophysical S-factor of the4He+12C radiative capture is calculated in the potential model at the energy range 0.1-2.0 MeV.Radiative capture12C(α,γ)16O is extremely relevant for the fate of massive stars and determines if the remnant of a supernova explosion becomes a black hole or a neutron star.Because this reaction occurs at low energies,the experimental measurements are very difficult and perhaps impossible.In this paper,radiative capture of the12C(α,γ)16O reaction at very low energies is taken as a case study.In comparison with other theoretical methods and available experimental data,good agreement is achieved for the astrophysical S-factor of this process. 相似文献
186.
The potential energy curves of the low-lying electronic states of BeH+ molecular ion are performed by using highly accurate multi-reference configuration interaction with AV5Z basis sets for H atom and ACV5Z basis set for Be atom, 1s inner shell of Be is considered as the core orbit and the active orbit, respectively, which are used to characterise the spectroscopic properties of a manifold of singlet and triplet states. Fourteen electronic states correlated with eight dissociation channels are investigated, we have found that the a3Σ+ and c3Σ+ both are bound states, the 33Σ+ possesses double wells, and the C1Σ+, 33Σ+, 23Π, 21Π, 11Δ, 13Δ, 23Δ and 21Δ states are studied for the first time. Transition dipole moment, Franck–Condon factors qυ′υ″ and Einstein coefficients Aυ′υ″ for A1Σ+–X1Σ+, 21Π–B1Π, c3Σ+–a3Σ+ and b3Π–a3Σ+ systems have been calculated. Radiative lifetime of A1Σ+–X1Σ+ band system has also been determined. 相似文献
187.
Reverse electric field Monte Carlo simulation for vector radiative transfer in the atmosphere 下载免费PDF全文
In this paper, a reverse electric field Monte Carlo (REMC) method is proposed to study the vector radiation transfer in the atmosphere. The REMC is based on tracing the multiply scattered electric field to simulate the vector transmitted radiance. The reflected intensities with different total optical depth values are obtained, which accord well with the results in the previous research. Stokes vector and the degree of polarization are numerically investigated. The simulation result shows that when the solar zenith angle is determined, the zenith angle of detector has two points, of which the degree of polarization does not change with the ground albedo and the optical depth. The two points change regularly with the solar zenith angle. Moreover, our REMC method can be applied to the vector radiative transfer in the atmosphere-ocean system. 相似文献
188.
Riadh Dardouri Héla Habli Brahim Oujia Florent Xavier Gadéa 《Journal of computational chemistry》2013,34(24):2091-2099
For all states dissociating below the ionic limit Li? Rb+, we perform a diabatic study for 1Σ+ electronic states dissociating into Rb (5s, 5p, 4d, 6s, 6p, 5d, 7s, 4f) + Li (2s, 2p, 3s). Furthermore, we present the diabatic results for the 1–11 3σ, 1–8 1,3Π, and 1–4 1,3Δ states. The present calculations on the RbLi molecule are complementary to previous theoretical work on this system, including recently observed electronic states that had not been calculated previously. The calculations rely on ab‐initio pseudopotential, core polarization potential operators for the core‐valence correlation and full valence configuration interaction approaches, combined to an efficient diabatization procedure. For the low‐lying states, diabatic potentials and permanent dipole moments are analyzed, revealing the strong imprint of the ionic state in the 1Σ+ adiabatic states. The transition dipole moment is used to evaluate the radiative lifetimes of the vibrational levels trapped in the 2 1Σ+ excited states for the first time. In addition to the bound–bound contribution, the bound–free term has been evaluated using the Franck–Condon approximation and also exactly added to the total radiative lifetime. © 2013 Wiley Periodicals, Inc. 相似文献
189.
We report the observation of anomalous temperature dependences of degenerate four-wave mixing spectra in CuCl thin films with high crystalline quality. The observed temperature dependence is in good agreement with the phase-decay-constant dependence of calculated induced-polarization spectrum. An excitonic state with large radiative width can be observed at high temperatures as superradiance is faster than the dephasing process. We succeeded in observing the DFWM signal up to room temperature based on the extremely large radiative width peculiar to the thickness region beyond the long-wavelength approximation regime. 相似文献
190.
Tatiana B. Zhuravleva Alexander A. Kokhanovsky 《Journal of Quantitative Spectroscopy & Radiative Transfer》2011,112(8):1353-1368
In this paper the influence of 3D effect on snow reflection function (SRF) and albedo is studied in the framework of the stochastic radiative transfer theory. In particular, the corresponding equations for the averaged intensity of reflected light are solved for the ensemble of realizations of the stochastic field κ(r), describing the distribution of 3D elements on the flat semi-infinite snow layer (SISL). The reflection from the underlying SISL is modeled using the solution of the 1D radiative transfer equation. The corresponding look-up tables were compiled beforehand and used in the simulation process. In accordance with the previous studies, it was found that the albedo of snow layer is reduced (in particular, in the infrared region), if 3D effects are taken into account. There is no such a reduction, if light absorption in snow is absent. The 3D effects may increase or decrease SRF depending on the sastrugi fraction and illumination/observation conditions. 相似文献