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M. Brando N. Büttgen V. Fritsch J. Hemberger H. Kaps H.-A. Krug von Nidda M. Nicklas K. Pucher W. Trinkl A. Loidl E.W. Scheidt M. Klemm S. Horn 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,25(3):289-298
We present susceptibility, microwave resistivity, NMR and heat-capacity results for Li1-xZnx(V1-yTiy)2O4 with 0 ?
x
? 0.3 and 0 ?
y
? 0.3. For all doping levels the susceptibility curves can be fitted with a Curie-Weiss law. The paramagnetic Curie-Weiss temperatures
remain negative with an average value close to that of the pure compound Θ≈ - 36 K. Spin-glass anomalies are observed in the susceptibility, heat-capacity and NMR measurements for both type of dopants.
From the temperature dependence of the spin-lattice relaxation rate we found critical-dynamic behavior in the Zn doped compounds
at the freezing temperatures. For the Ti-doped samples two successive freezing transitions into disordered low-temperature
states can be detected. The temperature dependence of the heat capacity for Zn-doped compounds does not resemble that of canonical
spin glasses and only a small fraction of the total vanadium entropy is frozen at the spin-glass transitions. For pure LiV2O4 the spin-glass transition is completely suppressed. The temperature dependence of the heat capacity for LiV2O4 can be described using a nuclear Schottky contribution and the non-Fermi liquid model, appropriate for a system close to
a spin-glass quantum critical point. Finally an (
x
/
y
,
T
)-phase diagram for the low-doping regime is presented.
Received 16 March 2001 and Received in final form 30 October 2001 相似文献
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Mingxin Wang 《Journal of Mathematical Analysis and Applications》2002,274(1):424-436
This paper deals with positive solutions of degenerate and quasilinear parabolic systems not in divergence form: ut=up(Δu+av), vt=vq(Δv+bu), with null Dirichlet boundary conditions and positive initial conditions, where p, q, a and b are all positive constants. The local existence and uniqueness of classical solution are proved. Moreover, it will be proved that all solutions exist globally if and only if ab?λ12, where λ1 is the first eigenvalue of −Δ in Ω with homogeneous Dirichlet boundary condition. 相似文献
27.
Fillmore在[1]中得到一个定理:设A,T是Banach空间X上的线性变换,A有界,若Lat(A) Lat(T)且AT=TA,则T是A的多项式.在本文里,以此作为引理,讨论了Banach空间上可逆线性变换A在什么情况下,A-1可表示为A的多项式.本文最主要的结论是定理3.4:设X是Banach空间,A是X上的有界线性变换,且可逆,则A-1是A的多项式当且仅当A-1是A的局部多项式. 相似文献
28.
We extend the matrix version of Cochran's statistical theorem to outer inverses of a matrix. As applications, we investigate the Wishartness and independence of matrix quadratic forms for Kronecker product covariance structures. 相似文献
29.
We discuss the problem of transmitting polarized pulses along optical fibers with variable dispersion. The dissipation and mean dispersion are assumed to be zero, which allows using the model of the vector nonlinear Schrödinger equation. We consider an optical fiber consisting of arms of equal length, which is assumed to be large. We propose an asymptotic recursive procedure for calculating the amplitude and the phase of an optical pulse propagating along the optical cable with variable dispersion. 相似文献
30.
Vincenzo Santagada Ferdinando FiorinoElisa Perissutti Beatrice SeverinoSara Terracciano Giuseppe CirinoGiuseppe Caliendo 《Tetrahedron letters》2003,44(6):1145-1148
A novel and convenient microwave-assisted dimerization of an active peptide compound using the DKPs as scaffold is described. The key reaction giving rise to the diketopiperazine scaffold is the intermolecular coupling. No epimerization was detected in the reactions used. Conventional and microwave heating of the reactions are compared. Synthesis by microwave irradiation gave the desired compounds in higher yields and in shorter reaction times than those obtained by conventional heating. 相似文献