费米环境中两个三能级原子系统的纠缠演化

利用负性纠缠度(negativity)研究了两个三能级原子系统在费米环境中的纠缠演化问题-结果表明,两个三能级原子系统的纠缠演化不仅依赖于系统和环境的相互作用强度,而且还依赖于系统所处的具体量子态-通过例子发现,系统和环境相互作用强度越大,纠缠衰减越快;对于纯态,仅当时间趋于无穷时纠缠才被完全破坏;对于混态,则在有限的时间内纠缠即被彻底破坏-通过一般的分析找到了一类免退相干的量子子空间-在这些子空间中,量子态不受环境的影响,故其纠缠不变-研究有助于理解费米环境造成的退相干对玻色系统纠缠的影响- 关键词： 费米环境 纠缠演化 两个三能级原子     

基于2,4′-二羧基二苯甲酮构筑的具有一维梯状链和一维隧道的三维超分子体系

采用水热法设计合成了两个新型三维超分子化合物H₂L·H₂O (1)和[Ag(bpy)₂]·HL·H₂O (2) (其中bpy=2,2'-联吡啶, H₂L=2,4′-二羧基二苯甲酮),晶体结构分析表明,它们均是通过氢键采用不同的连接方式拓展而成。其中,化合物1 是2,4′-二羧基二苯甲酮和水分子通过O–H···O氢键形成的一维梯状链扩展构筑的三维超分子体系;化合物2 则是2,4′-二羧基二苯甲酮和水分子通过两种氢键形成含有一维隧道的三维超分子体系。有趣的是,[Ag(bpy)₂]⁺ 阳离子通过π–π 堆积和弱的Ag···Ag相互作用连在一起,进而以客体形式填充其中。荧光性质研究表明,由于存在bpy的螯合与堆积效应,化合物2相比配体和化合物1,其荧光发射峰发生红移。     

Steady state Behaviour of a Three level Ladder Atomic System with Incoherent Population Pumping in a Squeezed Vacuum

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两束脉冲激光在级联的三能级系统中的传播

利用密度矩阵方程和麦克斯韦传播方程的耦合考虑激光脉冲的横向效应,在柱对称的条件下,研究了两束脉冲在级联系统中的共振传播,考察了脉冲在光学厚介质中的时空演化过程。数值计算中考虑了两个能级的自发辐射速度,给出了脉能量的空间演化及电熟粒子在空间的分布。     

Quantum Phase Transitions in Anisotropic Spin Ladders with Antiferromagnetic Rungs

We apply perturbation theory to study quantum phase transitions in anisotropic two-leg spin ladders with antiferromagnetic rungs in the strong interchain coupling limit. The energy gap is expanded up to the fourth order in the ratio of the intrachain to interchain couplings. The transition point is determined by examing the disappearance of the energy gap. Present results for the anisotropic ferromagnetic-leg spin ladder are consistent qualitatively with the nonlinear σ-model analysis and in good agreement with the numerical results by the diagonalization method.     

三维光子晶体中三能级原子的自发发射

研究了三维光子晶体中三能级原子自发发射的性质.由于各向异性色散关系,能带带边的态密度没有奇异性,局域场可以消失.在一定条件下弥散场会得到加强,并在辐射场中占主导地位.这些性质将与原子能级和能带带边的相对位置有关,且有别于各向同性色散关系的光子晶体中原子自发发射的性质. 关键词： 光子晶体 三能级原子 自发发射     

通过四个最大纠缠三态粒子来实现一未知的三个纠缠三态粒子的隐形传输

提出一种利用4个三态粒子的最大纠缠态作为量子信道来隐形传输一未知的3个三态粒子纠缠态的方案。在此方案中发送者Alice作一次Bell态测量和两次单独粒子的测量,并将测量结果通过经典信道告诉Bob,Bob根据接收到的信息即可通过相应的幺正变换来重建Alice要传输的量子态。     

三能级运动原子与单模场相互作用系统中场(原子)熵的演化

在共振和远离共振情况下,具体讨论了初始平均光子数、原子运动和场模结构参数对三能级运动原子与单模场相互作用系统中场(原子)熵演化的影响.结果显示:原子运动导致场熵演化具有周期性,这种周期性并不依赖场的统计分布和强度而是依赖于原子运动和场模结构参数εp.不论是共振情况还是远离共振情况,在选取合适的参数εp(这种选取在实验上是可能的)时,我们都能得到较长时间的纯态光场.     

Algebraic approach to the asymmetric rigid rotor

A pure algebraic treatment of the eigenvalue equation corresponding to the asymmetric top is presented. The algebraic method employs the Holstein–Primakoff bosonic realization of the angular momentum algebra. Explicit determination of the linear boson transformation coefficients of the eigenstates is carried out by means of the coherent states formalism. No reference to special functions is needed and a completely algebraic approach is achieved. © 2000 John Wiley & Sons, Inc. Int J Quant Chem 77: 704–709, 2000     

Synthesis of ladder polymers containing polydiacetylene backbones connected with methylene chains and their optical properties

The polymers consisting of polydiacetylene (PDA) backbones were obtained from the novel monomer derivatives, R CC CC R′ CC CC R [where R =  (CH₂)₄OCONHCH₂COOC₄H₉, R′ =  (CH₂)_n ; n = 2, 4, 8] [4BCMU4A(n)], in which linear methylene chain is sandwiched between two diacetylene moieties by solid-state 1,4-addition reaction. The polymerization process was investigated in detail by using spectroscopic techniques such as solid-state ¹³C-NMR, visible absorption, and IR absorption spectra. It was estimated that the polymerization of 4BCMU4A(8) and 4BCMU4A(4) takes place by two consecutive 1,4-addition reactions to form two PDA backbones, which constitute the two poles of the respective ladders. The bridging methylene chain length in the monomer was found to play a vital role as far as the polymerization process is concerned. Thus, the monomers with eight or four methylene units could form the ladder–PDAs by a two-step process, whereas the monomer containing two methylene units could only undergo one-step of 1,4-addition reaction. Further, it was found that the crystallinity of the polymers depends on the methylene chain length in the monomers, 4BCMU4A(8) being the most crystalline of all. These structural features strongly affect their absorption spectra. The third-order nonlinear optical susceptibilities (χ⁽³⁾) for these polymers were measured using third-harmonic generation method. The largest χ⁽³⁾ value obtained was 3.4 × 10⁻¹¹ esu for the poly[4BCMU4A(8)] thin film in resonant region. © 1999 John Wiley & Sons, Inc. J Polym Sci A: Polym Chem 37: 3537–3548, 1999