A new route has been developed to design plasmonic pollen grain-like nanostructures (PGNSs) as surface-enhanced Raman scattering (SERS)-active substrate. The nanostructures consisting of silver (Ag) and gold (Au) nanoparticles along with zinc oxide (ZnO) nanoclusters as spacers were found highly SERS-active. The morphology of PGNSs and those obtained in the intermediate stage along with each elemental evolution has been investigated by a high-resolution field emission scanning electron microscopy. The optical band gaps and crystal structure have been identified by UV-vis absorption and X-ray powder diffraction (XRD) measurements, respectively. For PGNSs specimen, three distinct absorption bands related to constituent elements Ag, Au, and ZnO were observed, whereas XRD peaks confirmed the existence of Ag, Au, and ZnO within the composition of PGNSs. SERS-activity of PGNSs was confirmed using Rhodamine 6G (R6G) as Raman-active dyes. Air-cooled solid-state laser kits of 532 nm were used as excitation sources in SERS measurements. SERS enhancement factor was estimated for PGNSs specimen and was found as high as 3.5×106. Finite difference time domain analysis was carried out to correlate the electromagnetic (EM) near-field distributions with the experiment results achieved under this investigation. EM near-field distributions at different planes were extracted for s-, p- and 45° of incident polarizations. EM near-field distributions for such nanostructures as well as current density distributions under different circumstances were demonstrated and plausible scenarios were elucidated given SERS enhancements. Such generic fabrication route as well as correlated investigation is not only indispensable to realize the potential of SERS applications but also unveil the underneath plasmonic characteristics of complex SERS-active nanostructures. 相似文献
We propose two schemes for generating a four-atom cluster state in a thermal
cavity. With the assistant of a strong classical field the
photon-number-dependent parts in the effective Hamiltonian are canceled.
Thus the schemes are insensitive to the thermal field. The schemes can also
be used to generate the cluster state for the trapped ions in thermal
motion. 相似文献
The generation of continuous variable entanglement via
atomic coherence in a two-mode three-level cascade atomic system
is discussed according to the entanglement criterion proposed by
Duan et al. [Phys. Rev. Lett. 84, 2722 (2000)].
Atomic coherence between the top and bottom levels is induced with
two photons of a strong external pump field. It shows that
entanglement for the two-mode field in the cavity can be generated
under certain conditions. Moreover, by means of the input-output
theory, we show that the two-mode entanglement could also be
approached at the output. 相似文献
Vibration isolation is one of the most efficient approaches to protecting host structures from harmful vibrations, especially in aerospace, mechanical, and architectural engineering, etc. Traditional linear vibration isolation is hard to meet the requirements of the loading capacity and isolation band simultaneously, which limits further engineering application, especially in the low-frequency range. In recent twenty years, the nonlinear vibration isolation technology has been widely investigated to broaden the vibration isolation band by exploiting beneficial nonlinearities. One of the most widely studied objects is the “three-spring” configured quasi-zero-stiffness (QZS) vibration isolator, which can realize the negative stiffness and high-static-low-dynamic stiffness (HSLDS) characteristics. The nonlinear vibration isolation with QZS can overcome the drawbacks of the linear one to achieve a better broadband vibration isolation performance. Due to the characteristics of fast response, strong stroke, nonlinearities, easy control, and low-cost, the nonlinear vibration with electromagnetic mechanisms has attracted attention. In this review, we focus on the basic theory, design methodology, nonlinear damping mechanism, and active control of electromagnetic QZS vibration isolators. Furthermore, we provide perspectives for further studies with electromagnetic devices to realize high-efficiency vibration isolation.
In a capillary discharge experiment for the neon-like argon lasing, we have proposed an experimental scheme to verify that the multi-spike of X-ray diode (XRD) signal is a multi-pulse laser or is a reflection of the laser pulse in the XRD.The ceramic capillary has an inner diameter of 3mm and a length of 200mm.At the gas pressure of 28Pa and discharge current of 27kA, stable lasing has been realized.The experimental results prove that the multi-spike of XRD signal is a reflection of the electromagnetic signal produced by the laser pulse in the XRD.The improved electrocircuit scheme of the XRD to minimize the reflection phenomena is also found. 相似文献