Ellipticity dependence of atomic and molecular high harmonic generation

High harmonic generation is compared in the dependence on the ellipticity of the fundamental laser radiation for an atomic and a molecular system. In particular argon and nitrogen are compared employing molecular beams and intense ( 3×10¹⁴ W/cm²) and ultrashort (80 fs) 800 nm laser pulses. It turns out that for all the harmonics under investigation (H5, H13 and H21) the harmonic yield decreases slower with the ellipticity for the molecule than for the atom. This indicates differences in atomic and molecular high harmonic generation. Received 24 April 2002 Published online 24 September 2002     

Classical Effects of Carrier--Envelope Phase on Nonsequential Double Ionization

A classical microcanonical 1＋1-dimensional model is used to investigate the ion momentum distributions in nonsequential double ionization with linearly polarized few-cycle pulses. We find that the ion momentum distribution has a strong dependence on the carrier-envelope phase of the few-cycle pulse, which is consistent with the experimental results qualitatively. Back analysis shows that the ionization probability of the first electron at different phases and its returning kinetic energy play the main role on the ion momentum distributions.     

Sub-Doppler laser absorption spectroscopy of the AΠi − XΣ (1, 0) band of CN: Measurement of the N hyperfine parameters in AΠ CN

Measurements of multiple rotational lines in the (1, 0) band of the A²Π_i − X²Σ⁺ “red” system of the cyanogen radical (CN) at sub-Doppler resolution are reported. The CN radical was produced by 193 nm photodissociation of NCCN (ethane dinitrile) and detected with a Ti:sapphire ring laser operating near 10 900 cm⁻¹. The sample was exposed to a weak, frequency-modulated probe beam and a strong, counterpropagating bleach laser beam. Demodulated probe laser signals display absorption and dispersion features derived from Doppler-free saturation of the hyperfine components as the laser scans across the central region of a Doppler-broadened rotational line spectrum. Hyperfine-resolved transition frequencies were combined with known ground-state X²Σ hyperfine term values to determine A²Π state hyperfine term values, which were analyzed in terms of an effective Hamiltonian for the A²Π state. All the expected hyperfine and ¹⁴N quadrupolar parameters were determined and their values analyzed in terms of a simple molecular orbital picture of the bonding in the radical. Higher sensitivity obtained with 400 kHz amplitude modulation of the bleach laser and additional phase-sensitive detection allowed hyperfine splittings in some rotational lines of ¹³C¹⁴N to be observed in natural abundance. Excited state hyperfine splittings were determined for a selection of rotational states, but not enough to determine the ¹³C hyperfine parameters.     

On the theory of the relativistic cross-sections for stimulated bremsstrahlung on an arbitrary electrostatic potential in the strong electromagnetic field

On the base of relativistic generalized eikonal approximation wave function the multiphoton cross-sections of a Dirac particle bremsstrahlung on an arbitrary electrostatic potential and strong laser radiation field are presented. In the limit of the Born approximation the ultimate analytical formulas for arbitrary polarization of electromagnetic wave have been obtained and numerically analyzed. Received 5 April 2001 / Received in final form 18 March 2002 Published online 28 June 2002     

High harmonic generation at 1 kHz repetition rate with a pulsed valve

High harmonic generation at 1 kHz repetition rate is reported. A piezoelectric pulsed valve together with a femtosecond Ti:Sapphire laser both operating at 1 kHz are employed to generate high harmonic radiation in xenon and argon. The characteristics of the valve have been analyzed by using a fast ion gauge and a time-of-flight mass-spectrometer. Received: 28 May 2001 / Revised version: 29 June 2001 / Published online: 18 July 2001     

Laser influence on positron-antiproton radiative capture collision

The laser-assisted radiative capture between a positron and an antiproton is studied in detail. The theoretical results show that the cross-section for antihydrogen formation is significantly reduced with the application of a laser background. This effect is most marked when the laser polarization is parallelto the incident direction. Received: 13 November 1998 / Received in final form: 16 March 1999     

Su(4) approach to fourfold degenerate electronic states of some hexafluoride molecules

We show that two appropriate realizations of the su(4) algebra allow the construction of all electronic operators needed for the study of vibronic and rovibronic interactions in a G^′ electronic state. In each case a full bosonic realization is made and all matrix elements are calculated. Illustrations of our formalism and comparisons with previous approaches are made in the case of ν₅(F_2g) and ν₃(F_1u) modes.     

Dark-line in optically-thick vapors: inversion phenomena and line width narrowing

An analysis of the phenomenon of coherent population trapping as observed by means of the dark state in the case of optically thick vapors in alkali metal atoms is presented. Very different behaviors are predicted for the observation of the dark state in the fluorescence and transmission spectra of the same atomic sample when the optical length is not negligible. Among other effects, the dark line observed in the fluorescence signal may look inverted appearing as a bright line, while in the transmission signal a narrowing of the line width resonance line is observed for an increase of the atomic density. In the pure three-level scheme a subnatural width is predicted. These effects, related to the electromagnetically induced transparency phenomenon, are readily observed in experiments, which are found to be in excellent agreement with the theory developed. Received 28 March 2001 and Received in final form 3 October 2001     

Electron-Helium Scattering in a Bichromatic Laser Field in the Second-Order Born Approximation

The elastic scattering of electrons in atomic helium assisted by a bichromatic laser field is investigated in the second order Born approximation. The target atom is approximated by a simple screening potential. The dependence of the differential cross section on the relative phase between the two laser components is calculated, and compared with the recent results of first order Born approximation [Sun J F, Liang M C and Zhu Z L 2007 Chin. Phys. Lett. 24 2572].     

An Optimum Scheme to Generate Entangled Photon Pairs

An optimum scheme is proposed to generate a strong entangled photon-pair light source by combining two incident laser lights. Such entangled photon source should have various potential applications in many fields such as quantum metrology, quantum information, and quantum lithography, etc.