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991.
An oriented adsorption behavior of NO2 is disclosed on the WSe2 monolayer in this work regardless the monolayer is perfect or defective based on density functional theory study by large-scale sampling. The presence of typical defects, including selenium vacancy, tungsten vacancy, and antisite defect of selenium on tungsten site, does not modify the anisotropic adsorption behavior of NO2 molecule at all. The adsorbed NO2 exhibits similar behavior on the four kinds of monolayers with its extending orientation all main lines along the two directions of the Se–W bond and the Se–W–Se trough, in spite of the symmetry is decreased somewhat from trigonal of the perfect monolayer to bilateral of the defective monolayers. Molecular dynamic simulations well reproduce these trends. The anisotropic adsorption behavior can be attributed to the polar properties of both heteroatomic bond of the WSe2 monolayer and NO2 molecule itself. Out of plane polarization is believed to play key role in the vertical and then the oriented adsorption behavior formation. The sensitivity is estimated to be very good based on moderate adsorption energy (0.35, 0.42, 0. 95 and 0.78 eV on pure, selenium vacancy, tungsten vacancy, and selenium on tungsten site monolayers) and considerable charge transfer number (0.205, 0.208, 0.164, and 0.160 e, respectively), with different degrees of change by defect. These fantastic findings may provide substantial foundation for wide applications beyond thought. 相似文献
992.
993.
Shilong Pan Pei Zhou Zhenzhou Tang Yamei Zhang Fangzheng Zhang Dan Zhu 《Fiber and Integrated Optics》2015,34(4):185-203
AbstractA polarization modulator together with a polarizer can implement phase modulation, intensity modulation with tunable chirp, and frequency-doubling intensity modulation. If an optical filter is incorporated, frequency-quadrupling and frequency-sextupling intensity modulations and a microwave photonic phase shifter can also be realized. By using a polarization modulator to replace the intensity modulator in an optoelectronic oscillator, various new features are enabled. In this article, an analytical model for the polarization modulator-based systems is established. The recent development in employing polarization modulators for constructing optoelectronic oscillators is discussed. The emerging applications enabled by the polarization modulator-based optoelectronic oscillators and the possible future development are also discussed. 相似文献
994.
Comparative analysis of electric field influence on the quantum wells with different boundary conditions. 下载免费PDF全文
Oleg Olendski 《Annalen der Physik》2015,527(3-4):278-295
Analytical solutions of the Schrödinger equation for the one‐dimensional quantum well with all possible permutations of the Dirichlet and Neumann boundary conditions (BCs) in perpendicular to the interfaces uniform electric field are used for the comparative investigation of their interaction and its influence on the properties of the system. Limiting cases of the weak and strong voltages allow an easy mathematical treatment and its clear physical explanation; in particular, for the small , the perturbation theory derives for all geometries a linear dependence of the polarization on the field with the BC‐dependent proportionality coefficient being positive (negative) for the ground (excited) states. Simple two‐level approximation elementary explains the negative polarizations as a result of the field‐induced destructive interference of the unperturbed modes and shows that in this case the admixture of only the neighboring states plays a dominant role. Different magnitudes of the polarization for different BCs in this regime are explained physically and confirmed numerically. Hellmann‐Feynman theorem reveals a fundamental relation between the polarization and the speed of the energy change with the field. It is proved that zero‐voltage position entropies are BC independent and for all states but the ground Neumann level (which has ) are equal to while the momentum entropies depend on the edge requirements and the level. Varying electric field changes position and momentum entropies in the opposite directions such that the entropic uncertainty relation is satisfied. Other physical quantities such as the BC‐dependent zero‐energy and zero‐polarization fields are also studied both numerically and analytically. Applications to different branches of physics, such as ocean fluid dynamics and atmospheric and metallic waveguide electrodynamics, are discussed.
995.
从理论和实验两个方面研究角向偏振无衍射光束在自由空间和障碍物空间中的传输特性. 理论上模拟了角向偏振无衍射光束在自由空间以及障碍物空间传播过程中的光强分布与偏振态变化情况. 实验中利用高斯光束先通过偏振转换仪, 再入射到轴棱锥上产生角向偏振无衍射光束. 进而研究其在空间中的传输情况, 并通过分析其经过扇形障碍物后光强分布变化情况讨论障碍物对偏振态的影响和光束的自重建特性. 结果表明: 障碍物遮挡区域光强沿z轴方向逐渐恢复, 且阴影区域沿障碍物所在位置的相反方向移动; 光束的偏振态局部发生变化, 该变化与障碍物所在位置有关. 理论仿真和实验结果一致. 相似文献
996.
相对于传统的光学遥感, 多角度偏振遥感不仅可以获取辐射强度信息, 而且可以获取偏振强度信息. 基于多角度偏振卫星载荷观测的中国典型地物的偏振反射率数据, 获取了地表偏振双向反射模型——Nadal模型的中国区域模型参数值. 在此基础上, 基于修正的Nadal模型研究了中国区域森林、草地、沙漠三种典型地物的多角度偏振特性. 研究表明: 1)各地物的偏振反射率均随着散射角的增大而减小, 随着太阳天顶角和卫星观测天顶角的增大而增大; 2)森林、草地和沙漠三种典型地表偏振反射率存在明显差别, 森林的偏振反射率最低, 草地的偏振反射率次之, 沙漠的偏振反射率大约为森林的两倍; 3)不同地物之间的偏振反射率差值均随着卫星观测天顶角和太阳天顶角的增大而增大. 研究结果可为基于多角度偏振遥感数据探测地表偏振特性和反演气溶胶参数提供先验知识. 相似文献
997.
提出了基于椭圆偏振光注入下垂直腔表面发射激光器(VCSEL)输出的正交偏振模式单周期(P1)振荡来同时获取两路光子微波的实现方案, 并进行了相关仿真研究. 结果表明: 在合适的参数条件下, 一个自由运行的VCSEL(定义为主VCSEL, M-VCSEL)可输出椭圆偏振光, 其X偏振分量和Y 偏振分量具有相同的激射频率; 将M-VCSEL输出的椭圆偏振光注入到另外一个VCSEL(定义为副VCSEL, S-VCSEL), 在给定主副VCSEL间频率失谐的条件下, 通过选择合适的注入强度可使S-VCSEL 中两个偏振分量均呈现单周期(P1)振荡, 从而可获得两正交的光子微波信号; 随着注入强度的增加, 光子微波的频率以及功率均呈现增加的趋势; 结合微波频率、功率以及输出光谱中第一边带和第二边带的幅度差在由注入强度和频率失谐所构成参数空间下的分布图, 可确定获取高品质微波信号的优化注入参数范围. 相似文献
998.
对新月形超辐射发光二极管的液相外延生长过程进行了机理分析。利用Matlab软件对建立的非平面生长模型进行了理论计算,并利用扫描电镜(SEM)对液相外延生长的形貌进行了分析,通过理论计算与实验分析设计了获得低偏振、高功率超辐射发光二极管的外延结构。利用该结构研制的超辐射发光二极管芯片在100 mA工作电流、25 ℃工作温度下输出功率达到3.6 mW,相应的输出波长为1 306 nm, 光谱半宽为39 nm,光谱波纹为0.17 dB,偏振度为2%。 相似文献
999.
1000.
We theoretically studied the spontaneous spin polarization properties of organic molecule rubrene by using density functional theory calculations. Our investigations show that normally nonmagnetic molecule rubrene could be spin polarized by spinless-hole injection. Magnetic moment of the molecule increases linearly with the extra hole charge amount only when the injected hole charges reach a certain value. The spin density resides predominantly on the carbon atoms in the tetracene backbone of rubrene molecule and also the bond lengths change differently due to the injected charge. Spontaneous spin polarization can be explained as the preferably filling of the spin-splitted carbon pz orbitals near the Fermi energy for the injected charge. 相似文献