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The present work concerns the study of solvent effects on the geometrical structures, as well as one- and two-photon absorption (TPA) processes, for two series of alkyne and alkene π-bridging molecules, within the framework of the polarization continuum model. Particular emphasis was put on the characterization of solvent effects on the molecular geometrical structures and geometric distortion, which were measured by the bond-length-alternation parameter. The π centres in the compounds are seen to play a decisive role in increasing the TPA cross section and nonlinear optical properties. All studied molecules have relatively strong TPA characteristics, while the alkyne π-bridging ones yield larger TPA cross sections. 相似文献
105.
Shuzhen Fan Qingpu Wang Shutao Li Shuanghong Ding Fufang Su 《Optics Communications》2006,266(2):620-626
A method of more precise determination of the focal length of equivalent thermal lens (TL) is presented in this paper. The method is based on the diffraction theory of aberrations. By numerically calculating the optical path difference (OPD) distribution and the Strehl ratio, the focal lengths for “top-hat” pumping and Gaussian pumping are obtained and the equations for the focal lengths are presented by curve fitting. Also the equations for average pump radii are presented. The experiment on a fiber-coupled LD pumped Nd:YAG laser is carried out. The experimental results verify the validity of the method. 相似文献
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SHI Shi-Wei YANG Qun YI You-Min 《理论物理通讯》2006,46(7)
A deterministic teleportation scheme for an arbitrary two-particle state is proposed in cavity QED. The success probability can reach 1.0. In addition, the scheme is insensitive to both the cavity decay and the thermal field. 相似文献
108.
We propose the methods of generating multipartite entanglement by considering the interaction of a system of N two-level atoms in M cavities of high quality factor with a strong classical driving field. It is shown that, with the cavity detuning, the applied driving field detuning and vacuum Rabi coupling, we can produce an entangled coherent state in two single-mode cavities and generate the entangled coherent cluster states in two bimodal vacuum cavities. Tuning these parameters also allows us to acquire the anti-Jaynes-Cummings (AJC) interaction, with which we can generate the maximally two-photon entangled states, and the two-atom and the two-photon entangled cluster states. 相似文献
109.
High-power operation of diode-pumped fiber lasers at wavelength near 2μm are demonstrated with short length of heavily Tm3 -doped silica glass fibers. With 7-cm long fiber, a laser at near 2 μm is obtained with the threshold of 135 mW, maximum output power of 1.09 W, and slope efficiency of 9.6% with respect to the launched power from a laser diode at 790 nm. The output stability of this fiber laser is within 5%.The dependence of the performance of fiber lasers on the operation temperature and cavity configuration parameters is also investigated. 相似文献
110.
The quantum mechanical phase distribution and the quantum oscillations of population are studied for a cavity field togetherwith
a driven classical field. The atom is sent through the cavity and driven by a classical field. Also the time evolution of
the system including decay is obtained. The graph showing the Rabi oscillations for this system is changed into a bit pattern
from the system without decay. The phase probability function is also affected due to the presence of cavity decay. 相似文献