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901.
不同碰撞系统在碰撞过程中转动传能的量子干涉角度并不相同.而对干涉角的计算需采取最符合系统的相互作用势.从含时微扰的一级波恩近似出发,利用各向异性相互作用势,进一步研究了CO单三混合态在和He做碰撞伴时其跃迁振幅和干涉相位角的时间特性,计算显示跃迁振幅随时间显现衰减的震荡;对于给定的碰撞参数和碰撞速度,跃迁振幅变化非常明显并与跃迁前后的状态、能级差相关. 相似文献
902.
喷动床气固流动特性的三维CFD-DEM数值模拟 总被引:1,自引:0,他引:1
开展了柱锥形气固流动特性的CFD-DEM耦合三维数值模拟研究。气相场采用基于欧拉坐标体系的k-ε双方程湍流模型,固相场采用基于拉格朗日坐标体系的DEM直接数值模拟方法,跟踪离散颗粒场的每一个颗粒,考虑颗粒与颗粒(壁面)之间的碰撞力、曳力、重力、Magnus升力、saffman升力。颗粒之间的碰撞采用Hertz-Mindlin无滑移模型计算。模拟对象为柱锥形喷动床,其直径为0.152 m,喷口直径为0.019 m,模拟颗粒数22万,探讨了喷动床中射流随时间的发展,不同气速下床内气固流动结构,以及颗粒速度与颗粒浓度的分布,并与实验数据进行了对比。 相似文献
903.
In this work we continue the study of a family of 1D piecewise smooth maps, defined by a linear function and a power function with negative exponent, proposed in engineering studies. The range in which a point on the right side is necessarily mapped to the left side, and chaotic sets can only be unbounded, has been already considered. In this work we are characterizing the remaining ranges, in which more iterations of the right branch are allowed and in which divergent trajectories occur. We prove that in some regions a bounded chaotic repellor always exists, which may be the only non-divergent set, or it may coexist with an attracting cycle. In another range, in which divergence cannot occur, we prove that unbounded chaotic sets always exist. The role of particular codimension-two points is evidenced, associated with fold bifurcations and border collision bifurcations (BCBs), related to cycles having the same symbolic sequences. We prove that they exist related to the border collision of any admissible cycle. We show that each BCB, each fold bifurcation and each homoclinic bifurcation is a limit set of infinite families of other BCBs. 相似文献
904.
905.
We discuss three different experiments for studying electron-excitation of atoms where lasers have been used in combination. These are stepwise electron–photon excitation, superelastic electron scattering from laser excited atoms and excitation of atoms using spin polarized electrons produced by lasers. We present distorted wave calculations and compare our results with the recently reported such experimental measurements. In particular, the results for the alignment and orientation of the excited n 2P states of K () and Rb () atoms and the spin parameters for the lowest excited 1P1 and 3P0,1,2 states of argon by polarized electrons are presented and discussed. 相似文献
906.
We have studied the protonated ether-(H2O)n (n = 1-3) complexes containing tetrahydrofuran, dimethyl, diethyl, dibutyl, and butylmethyl ethers using a flowing afterglow triple-quadrupole mass spectrometer. Collision-induced dissociation, CID, of all clusters with n = 1, 2 shows sequential water loss. The n = 3 cluster of dimethyl ether shows sequential water loss, while all other ether clusters display selective product formation. The CID spectra are interpreted based on known energetics, and theoretical studies of the dimethyl and diethyl ether systems. 相似文献
907.
利用分波法研究了低温及极低温下基态H和Br原子沿HBr(X1Σ+)分子相互作用势发生的弹性碰撞. 在1.0×10-11-1.0×10-3 a.u.的碰撞能区内通过数值求解原子-原子碰撞的薛定鄂方程, 计算了这一弹性碰撞的总截面和各分波截面, 讨论了各分波截面对总弹性截面的贡献. 结果表明在非常低的温度下这一弹性散射的总截面值很大、且几乎为一常数. 分析指出在极低能区内总弹性截面的形状主要由s分波截面的形状决定. 在总弹性截面上存在着2个较强的形状共振, 一个位于2.276×10-4 a.u., 另一个位于4.440×10-4 a.u. 计算表明前者主要来自于f和g分波的联合贡献, 后者主要来自于l = 5和l = 7分波的联合贡献. 虽然在f分波上还存在一个形状共振、且在直到l = 8的其它分波中也都存在强度不同的形状共振, 但它们都被淹没在较强的总弹性截面中. 同时计算还表明, 高于l = 10的分波对总弹性截面已无实质贡献. 相似文献
908.
909.
The interaction potential of a He-BH complex is investigated by the coupled-cluster single-double plus pertur-bative triples (CCSD (T)) method and an augmented correlation consistent polarized valence (aug-cc-pV)5Z basis set extended with a set of (3s3p2d1f1g) midbond functions. Using the five two-dimensional model potentials, the first three-dimensional interaction potential energy surface is constructed by interpolating along (r–r e ) by using a fourth-order polynomial. The cross sections for the rovibrational relaxation of BH in cold and ultracold collisions with 3 He atom are calculated based on the three-dimensional potential. The results show that the Δv =-1 transition is more efficient than the Δv =-2 transition, and that the process of relaxation takes place mainly between rotational energy levels with the same vibration state and the Δj =-1 transition is the most efficient. The zero temperature quenching rate coefficient is finite as predicted by Wigner’s law. The resonance is found to take place around 0.1–1 cm-1 translational energy, which gives rise to a step in the rate coefficients for temperatures around 0.1–1 K. The final rotational distributions in the state v = 0 resulting from the quenching of state (v = 1, j = 0) at three energies corresponding to the three different regimes are also given. 相似文献
910.