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991.
《化学:亚洲杂志》2017,12(10):1052-1056
The β‐cyclodextrin‐assisted aqueous‐exfoliation method was used to prepare transition‐metal dichalcogenide (TMD) nanosheets, in a cheap, highly efficient, scalable and environmentally friendly manner. As study cases, MoS2 and ReS2 nanoflakes were prepared according to this method. Particularly, the effective exfoliation of ReS2 crystals in an aqueous environment was observed for the first time. Moreover, exfoliated nanomaterials can be readily utilized in hydrogen evolution reactions (HERs) as noble‐metal‐free catalysts. This work provides new opportunities for highly efficient exfoliation of TMDs and other 2D nanomaterials into few‐layer nanosheets in aqueous media. Their production process showed high biocompatibility, broad applicability and excellent sustainability. 相似文献
992.
《化学:亚洲杂志》2017,12(8):882-889
Ag0.5La0.5TiO3 with an ABO3 perovskite structure was synthesized by a newly developed ion‐exchange method. Molten Ag2SO4 instead of traditional molten AgNO3 was used as Ag+ source in view of its high decomposition temperature (1052 °C), thereby guaranteeing the complete substitution of Ag+ for Na+ in Na0.5La0.5TiO3 with a stable ABO3 perovskite structure at a high ion‐exchange temperature (700 °C). Under full‐arc irradiation, the O2‐evolution activity of Ag0.5La0.5TiO3 was about 1.6 times that of Na0.5La0.5TiO3 due to the optimized electronic band structures and local lattice structures. On the one hand, the substitution of Ag+ for Na+ elevated the VBM and thus narrowed the band gap from 3.19 to 2.83 eV, thereby extending the light‐response range and, accordingly, enhancing the photoexcitation to generate more charge carriers. On the other hand, the substitution of Ag+ for Na+ induced a lattice distortion of the ABO3 perovskite structure, thereby promoting the separation and migration of charge carriers. Moreover, under visible‐light irradiation, Ag0.5La0.5TiO3 displayed notable O2 evolution whereas Na0.5La0.5TiO3 showed little O2 evolution, thus demonstrating that the substitution of Ag+ for Na+ enabled the use of visible light to evolve O2 photocatalytically. This work presents an effective route to explore novel Ag‐based photocatalysts. 相似文献
993.
994.
In this paper, the nonlinear iterative methods, which are different from the classical algorithms, to solve inverse problems are presented. Our methods by denoting some parameters and some properties of the algorithm in both noise and noiseless cases are studied. Finally, the convergence of the sequence generated by the algorithm without noise is discussed. 相似文献
995.
996.
997.
Paweł SZAFRANIEC 《数学物理学报(B辑英文版)》2017,37(4):1048-1060
In this paper we prove the existence and uniqueness of a weak solution for a dynamic electo-viscoelastic problem that describes a contact between a body and a foundation. We assume the body is made from thermoviscoelastic material and consider nonmonotone boundary conditions for the contact. We use recent results from the theory of hemivariational inequalities and the fixed point theory. 相似文献
998.
In this note, we explore the validity of Wente-type estimates for Neumann boundary problems involving Jacobians. We show in particular that such estimates do not in general hold under the same hypotheses on the data for Dirichlet boundary problems. 相似文献
999.
Mihajlo Cekić 《偏微分方程通讯》2017,42(11):1781-1836
In this paper, we consider the problem of identifying a connection ? on a vector bundle up to gauge equivalence from the Dirichlet-to-Neumann map of the connection Laplacian ?*? over conformally transversally anisotropic (CTA) manifolds. This was proved in [9] for line bundles in the case of the transversal manifold being simple—we generalize this result to the case where the transversal manifold only has an injective ray transform. Moreover, the construction of suitable Gaussian beam solutions on vector bundles is given for the case of the connection Laplacian and a potential, following the works of [11]. This in turn enables us to construct the Complex Geometrical Optics (CGO) solutions and prove our main uniqueness result. We also reduce the problem to a new non-abelian X-ray transform for the case of simple transversal manifolds and higher rank vector bundles. Finally, we prove the recovery of a flat connection in general from the DN map, up to gauge equivalence, using an argument relating the Cauchy data of the connection Laplacian and the holonomy. 相似文献
1000.
Monika Wolfmayr 《Numerical Methods for Partial Differential Equations》2017,33(2):403-424
In this work, new results on functional type a posteriori estimates for elliptic optimal control problems with control constraints are presented. More precisely, we derive new, sharp, guaranteed, and fully computable lower bounds for the cost functional in addition to the already existing upper bounds. Using both, the lower and the upper bounds, we arrive at two‐sided estimates for the cost functional. We prove that these bounds finally lead to sharp, guaranteed and fully computable upper estimates for the discretization error in the state and the control of the optimal control problem. First numerical tests are presented confirming the efficiency of the a posteriori estimates derived. © 2016 Wiley Periodicals, Inc. Numer Methods Partial Differential Eq 33: 403–424, 2017 相似文献