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41.
Abstract In this study, it is demonstrated that the Coulomb interactions explains the essential of experimental thermodynamic and transport thermodynamic results. 相似文献
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The change of the size distribution of Au clusters induced by annealing was studied in situ by transmission electron microscopy. Starting from statistically distributed Au clusters on a thin amorphous carbon film, “islands” are formed within a few months storage at room temperature, which consist of Au clusters with sizes <4 nm embedded in a thin Au film. These islands cover originally areas with sizes around 25 × 70 nm2. If the temperature is increased in the transmission electron microscope two different processes can be clearly distinguished that lead to the coarsening of the cluster size distribution: cluster coalescence and (contactless) Ostwald ripening. The degree and rate of the coarsening are found to depend on the underlying surface (Au film or amorphous carbon) and the exposure to the high-flux high-energy electron beam, which can be estimated to lead to high-temperature excursions in a cluster on a 10−12 s time scale. The experimental findings are confirmed by Monte-Carlo simulations using the many-body Gupta potentials in order to calculate the Au/Au interaction. Moreover, the results of MC simulations suggest an electron-beam induced formation of a “quasi-two-dimensional gas” of small highly mobile Au species on the Au film, which promotes Ostwald ripening. 相似文献
44.
The existing literature contains many examples of mean-field particle systems converging to the distribution of a Markov process conditioned to not hit a given set. In many situations, these mean-field particle systems are failable, meaning that they are not well defined after a given random time. Our first aim is to introduce an original mean-field particle system, which is always well defined and whose large number particle limit is, in all generality, the distribution of a process conditioned to not hit a given set. Under natural conditions on the underlying process, we also prove that the convergence holds uniformly in time as the number of particles goes to infinity. As an illustration, we show that our assumptions are satisfied in the case of a piece-wise deterministic Markov process. 相似文献
45.
At the state of statistical stationarity, the response of a nonlinear system under multiplicative random excitations can be either trivial or non-trivial, depending on the spectral levels of the excitations and the values of certain system parameters. Assuming that the random excitations are Gaussian white noises, the two types of response may be investigated by way of their stationary densities, which are obtainable for first order dynamical systems and for higher order dynamical systems belonging to the class of generalized stationary potential. Alternatively, the Lyapunov exponents can be computed for perturbation from either the trivial or non-trivial solution, since a negative sign for the greatest Lyapunov exponent provides both the necessary and sufficient conditions for the stability of sample functions with probability one. It is shown in two specific examples, that the boundary at which the greatest Lyapunov exponent changes its sign coincides with the boundary for regularity (or being normalizable) for the probability density in both the trivial and non-trivial solutions. Thus, the stability conditions in the strong sense of probability one and the weak sense in distribution are identical in these cases. 相似文献
46.
A. V. Kozlov 《Fluid Dynamics》2004,39(1):162-167
Using the numerical method of direct statistical simulation (Monte-Carlo method), the effect of the intermolecular potential exponent on the dependence of the stress and the heat flux on the stress rate tensor components and the temperature gradient is analyzed for the nonequilibrium, spherically symmetric outflow of a monatomic gas into a vacuum. Analytical approximations of the constitutive relations are presented. The dependence of the macroscopic parameters on the distance from the source is found. 相似文献
47.
对腐蚀管道的模糊可靠度计算方法进行了深入研究,提出了确定性可靠度和模糊可靠度两个基本概念;提出了基于断裂失效判据、基于FAD失效评估图和基于剩余强度3种方法计算模糊可靠度的方法;提出了3种新的方法计算确定性可靠度,即改进的JC法、GA—JC法和改进的Monte-Carlo法.以胜利油田某试验区已加入缓蚀剂的注水管道为例,采用本文建立的计算模糊可靠度的3种计算方法和确定性可靠度的3种方法,分别计算注水管道可靠度随着时间的变化趋势.在模糊可靠度的3种计算方法中,基于剩余强度失效方法比较适中,是计算模糊可靠度较好的方法;在确定性可靠度的3种计算方法中,改进的Monte-Carlo法较好. 相似文献
48.
短脉冲强激光产生的电子束具有源尺寸小、脉宽窄、准单能谱等特点, 在放射照相诊断中具有独特作用. 本文通过分析电子在材料中散射并采用蒙特卡罗方法数值模拟, 研究了100 keV到几百MeV能量电子束对有厚度起伏或存在界面的靶的透视, 并与质子、X射线束透视结果比较, 给出了电子束放射照相的特性与参数优化: 基于电子在材料中非弹性散射或能量损失, 选用能量使其射程与靶厚度接近的电子束来诊断靶厚度不均匀性; 基于电子在材料中的弹性散射, 选用射程超过靶厚度的电子束来诊断靶界面. 相似文献
49.
We numerically study convection–diffusion equations arising in financial modeling. We focus on the convection-dominated cases, in which the diffusion coefficients are relatively small. Both finite-difference and Monte-Carlo methods which are widely used in the problems of this kind might be inefficient due to severe restrictions on the meshsize and the number of realizations needed to achieve high resolution.We propose an alternative approach based on particle methods which have extremely low numerical diffusion and thus do not have the aforementioned restrictions. Our approach is based on the operator splitting: The hyperbolic steps are made using the method of characteristics, while the parabolic steps are performed using either a special discretization of the integral representation of the solution (which leads to a deterministic particle method) or a stochastic random walk approach.We apply the designed particle methods to a variety of test problems and the numerical results indicate high accuracy, efficiency and robustness of both the deterministic and stochastic methods. In addition, our numerical experiments clearly demonstrate that the deterministic particle method outperforms its stochastic counterpart. 相似文献
50.