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21.
Facile Construction of 3D Reduced Graphene Oxide Wrapped Ni3S2 Nanoparticles on Ni Foam for High‐Performance Asymmetric Supercapacitor Electrodes 下载免费PDF全文
Jiqiu Qi Yuan Chang Yanwei Sui Yezeng He Qingkun Meng Fuxiang Wei Yulong Zhao Yunxue Jin 《Particle & Particle Systems Characterization》2017,34(12)
3D reduced graphene oxide (rGO)‐wrapped Ni3S2 nanoparticles on Ni foam with porous structure is successfully synthesized via a facile one‐step solvothermal method. This unique structure and the positive synergistic effect between Ni3S2 nanoparticles and graphene can greatly improve the electrochemical performance of the NF@rGO/Ni3S2 composite. Detailed electrochemical measurements show that the NF@rGO/Ni3S2 composite exhibits excellent supercapacitor performance with a high specific capacitance of 4048 mF cm?2 (816.8 F g?1) at a current density of 5 mA cm?2 (0.98 A g?1), as well as long cycling ability (93.8% capacitance retention after 6000 cycles at a current density of 25 mA cm?2). A novel aqueous asymmetric supercapacitor is designed using the NF@rGO/Ni3S2 composite as positive electrode and nitrogen‐doped graphene as negative electrode. The assembled device displays an energy density of 32.6 W h kg?1 at a power density of 399.8 W kg?1, and maintains 16.7 W h kg?1 at 8000.2 W kg?1. This outstanding performance promotes the as‐prepared NF@rGO/Ni3S2 composite to be ideal electrode materials for supercapacitors. 相似文献
22.
Network dynamics and its relationships to topology and coupling structure in excitable complex networks 下载免费PDF全文
All dynamic complex networks have two important aspects, pattern dynamics and network topology. Discovering different types of pattern dynamics and exploring how these dynamics depend or/network topologies are tasks of both great theoretical importance and broad practical significance. In this paper we study the oscillatory behaviors of excitable complex networks (ECNs) and find some interesting dynamic behaviors of ECNs in oscillatory probability, the multiplicity of oscillatory attractors, period distribution, and different types of oscillatory patterns (e.g., periodic, quasiperiodic, and chaotic). In these aspects, we further explore strikingly sharp differences among network dynamics induced by different topologies (random or scale-free topologies) and different interaction structures (symmetric or asymmetric couplings). The mechanisms behind these differences are explained physically. 相似文献
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MI Ai-Jun ZUO Wei LI Zeng-Hua Umberto Lombardo 《理论物理通讯》2009,51(6):1113-1116
The 3 P F2 superfluidity of neutron and proton is investigated in isospin-asymmetric nuclear matter within the Brueckner-Hartree-Fock approach and the BCS theory by adopting the Argonne V14 and the Argonne V18 nucleonnucleon interactions. We find that pairing gaps in the 3PF2 channel predicted by adopting the AV14 interaction are much larger than those by the AV18 interaction. As the isospin-asymmetry increases, the neutron 3 pF2 superfluidity is found to increase rapidly, whereas the proton one turns out to decrease and may even vanish at high enough asymmetries. As a consequence, the neutron 3pF2 superfluidity is much stronger than the proton one at high asymmetries and it predominates over the proton one in dense neutron-rich matter. 相似文献
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George Pitsevich Elena Shalamberidze Alex Malevich Valdas Sablinskas Vytautas Balevicius Lars G. M. Pettersson 《Molecular physics》2017,115(20):2605-2613
The frequencies and intensities of vibration–rotational transitions of water molecules in an argon matrix were calculated for temperatures of 6 and 30 K. The rigid asymmetric top approximation was used with available literature values of the effective rotational constants in the ground and excited vibrational states. The calculations were carried out by taking into account the existence of a non-equilibrium population distribution between the rotational levels of ortho- and para-water isomers. It was assumed that the temperature relaxation of the population of rotational levels is independent of the ortho- and para-isomers. Comparison of the results of the theoretical calculations with experimental literature data shows good agreement for the majority of the rotational structure lines for symmetric and antisymmetric stretching vibrations both in the frequency values and in the values of the relative intensities. 相似文献
27.
A planar chiral nanostructure with asymmetric transmission of linearly polarized wave and huge optical activity in near-infrared band 下载免费PDF全文
Just like an electronic diode that allows the electrical current to flow in one direction only, a kind of chiral metamaterial structure with a similar functionality for the electromagnetic wave is proposed. The designed nanostructure that consists of twisted metallic split-ring resonators on both sides of a dielectric substrate achieves asymmetric transmission for a forward and backward propagating linearly polarized wave by numerical simulation in near-infrared band. Difference in transmission efficiency of the optimized structure between the same polarized waves incident from opposite directions can reach a maximum at the communication wavelength (1.55 μm). Moreover, the simulation results of this structure also exhibit strong optical activity and circular dichroism. 相似文献
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ABSTRACTWe study the effect of the external electric field Fext on the low-temperature electron mobility μ in an asymmetrically doped AlxGa1-xAs based V-shaped double quantum well (VDQW) structure. We show that nonlinearity of µ occurs under double subband occupancy on account of intersubband effects. The field Fext alters the VDQW potential leading to transfer of subband wave functions between the wells, which affects the scattering potentials and hence μ. In the VDQW structure, due to the alloy channel layer, the alloy disorder (Al-) scattering happens to be significant along with the ionised impurity (Imp-) scattering. The non-linear behaviour of μ is because of μImp, while the overall magnitude of μ is mostly due to μAl. The increase of difference in the doping concentrations of the outer barriers increases the nonlinearity of μ. The oscillatory character of μ is amended by varying the width of the well and barrier and also the height of the VDQW. Our results can be used to study VDQW based nanoscale field effect transistor structures. 相似文献
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多通道磁共振成像方法采用多个接收线圈同时欠采样k空间以加快成像速度,并基于后处理算法重建图像,但在较高加速因子时,其图像重建质量仍然较差.本文提出了一种基于PCAU-Net的快速多通道磁共振成像方法,将单通道实数U型卷积神经网络拓展到多通道复数卷积神经网络,设计了一种结构不对称的U型网络结构,通过在解码部分减小网络规模以降低模型的复杂度.PCAU-Net网络在跳跃连接前增加了1×1卷积,以实现跨通道信息交互.输入和输出之间利用残差连接为误差的反向传播提供捷径.实验结果表明,使用规则和随机采样模板,在不同加速因子时,相比常规的GRAPPA重建算法和SPIRiT重建方法,本文提出的PCAU-Net方法可高质量重建出磁共振复数图像,并且相比于PCU-Net方法,PCAU-Net减少了模型参数、缩短了训练时间. 相似文献