飞秒激光参数对非绝热耦合分子态布居的影响

利用含时波包法研究强飞秒泵浦-探测激光场中激光脉宽、波长和场强对非绝热耦合NaI分子各态布居的影响.波包在势能面上做周期性运动,周期约为1 000 fs.延时为200 fs时,波包第一次到达交叉区域分裂成两部分.波包在交叉区域的分裂情况影响各态布居.脉宽增长,NaI分子的激发概率增大,而解离概率减小.泵浦波长为共振波长318 nm时,激发概率最大.泵浦波长增长,NaI分子的解离概率减小.泵浦场强增大,激发概率增大,但解离概率不变.探测激光波长和场强不影响NaI分子各态布居分布.调节激光场参数可实现对波包运动的控制从而控制态布居的选择性分布.研究结果为实验上实现分子的光控制过程提供参考.     

Pulse chirping effect on controlling the transverse cavity oscillations in nonlinear bubble regime

The propagation of an intense laser pulse in an under-dense plasma induces a plasma wake that is suitable for the acceleration of electrons to relativistic energies. For an ultra-intense laser pulse which has a longitudinal size shorter than the plasma wavelength, λp, instead of a periodic plasma wave, a cavity free from cold plasma electrons, called a bubble, is formed behind the laser pulse. An intense charge separation electric field inside the moving bubble can capture the electrons at the base of the bubble and accelerate them with a narrow energy spread. In the nonlinear bubble regime, due to localized depletion at the front of the pulse during its propagation through the plasma, the phase shift between carrier waves and pulse envelope plays an important role in plasma response. The carrier–envelope phase(CEP) breaks down the symmetric transverse ponderomotive force of the laser pulse that makes the bubble structure unstable. Our studies using a series of two-dimensional(2D) particle-in-cell(PIC) simulations show that the frequency-chirped laser pulses are more effective in controlling the pulse depletion rate and consequently the effect of the CEP in the bubble regime. The results indicate that the utilization of a positively chirped laser pulse leads to an increase in rate of erosion of the leading edge of the pulse that rapidly results in the formation of a steep intensity gradient at the front of the pulse. A more unstable bubble structure, the self-injections in different positions, and high dark current are the results of using a positively chirped laser pulse. For a negatively chirped laser pulse, the pulse depletion process is compensated during the propagation of the pulse in plasma in such a way that results in a more stable bubble shape and therefore, a localized electron bunch is produced during the acceleration process. As a result, by the proper choice of chirping, one can tune the number of self-injected electrons, the size of accelerated bunch and its energy spectrum to the values required for practical applications.     

A tunable XUV monochromatic light source based on the time preserving grating selection of high-order harmonic generation

We accomplish a laboratory facility for producing a femtosecond XUV coherent monochromatic radiation with a broad tunable spectral range of 20 eV-75 eV. It is based on spectral selected single-order harmonics from intense laser driven high harmonic generation in gas phase. The time preserving for the selected harmonic radiation is achieved by a Czerny-Turner type monochromator designed with a conical diffraction grating mount for minimizing the time broadening caused by grating diffraction and keeping a relatively high diffraction efficiency. Our measurement shows that the photon flux of the 23-order harmonic(H23) centered at 35.7 eV is 1×10~9 photons/s approximately with a resolving power E/?E ≈ 36.This source provides an ultrashort tunable monochromatic XUV beam for ultrafast studies of electronic and structural dynamics in a large variety of matters.     

On the regulator problem for linear degenerate control systems

In this paper, we study the finite-time regulator problem for linear, autonomous, degenerate systems, i.e., systems described by the differential equation with det(K)=0. Two investigations of the regulator problem are presented, which depend on the quadratic cost associated with the differential equation.This work was performed under the auspices of the National Research Council of Italy, Gruppo Nazionale per l'Analisi Funzionale e le Sue Applicazioni, Rome, Italy.     

高功率横流CO2激光器脉冲预电离过程研究

本文给出了对高功率横流CO_2激光器脉冲预电离过程的理论和实验研究.表明了预电离过程中光电离的重要作用.实验结果表明,脉冲预电离可增大高功率横流CO_2.激光器的pd值(p为放电气压、d为放电间隔),增大放电区注入功率密度.对于提高此类型激光器的放电稳定性和输出激光功率是一种技术简单而有效的手段.     

Angular distributions of CH3I fragment ions under the irradiation of a single pulse and trains of ultrashort laser pulses

The angular distribution of CH3I is investigated experimentally using a single Fourier transform-limited laser pulse and a pulse train, where a 90-fs 800-nm linearly polarized laser field with a moderate intensity of 2.8×1013 W/cm2 is used. The dynamic alignment is demonstrated in a single pulse experiment. Moreover, a pulse train is used to optimize the molecular alignment, and the alignment degree is almost identical to that with the single pulse. The results are analysed by using chirped femtosecond laser pulses, and it demonstrates that the structure of pulse train rather than its effective duration is crucial to the molecular alignment.     

Improving attosecond pulse reflection by large angle incidence for a periodic multilayer mirror in the extreme ultraviolet region

The improvement of attosecond pulse reflection by large angle incidence for a periodic multilayer mirror in the extreme ultraviolet region has been discussed. Numerical simulations of both spectral and temporal reflection characteristics of periodic multilayer mirrors under various incident angles have been analyzed and compared. It was found that the periodic multilayer mirror under a larger incidence angle can provide not only higher integrated reflectivity but also a broader reflection band with negligible dispersion, making it possible to obtain better a reflected pulse that has a higher pulse reflection efficiency and shorter pulse duration for attosecond pulse reflection. In addition, by increasing the incident angle, the promotion of attosecond pulse reflection capability has been proven for periodic multilayer mirrors with arbitrary layers.     

基于耦合Duffing振子的局部放电信号检测方法研究

以双向环形耦合Duffing振子系统为对象, 研究脉冲信号激励下耦合振子间动力学行为变化特征时, 发现其与单向环形耦合Duffing振子系统类似, 在一定的参数条件下, 脉冲信号能引起其中一个振子与其他振子运动轨迹间出现短暂失同步的现象即瞬态同步突变现象. 基于这种现象, 提出了一种微弱脉冲信号检测的新方法, 用于检测强噪声背景中的局部放电脉冲信号. 实验测试表明, 利用本文方法对不同放电电极的局部放电脉冲信号进行检测时, 在低信噪比条件下可取得良好的检测效果, 进而扩展了现有的Duffing振子对非周期信号的检测范围及应用领域. 关键词： 耦合Duffing 振子 微弱信号检测 瞬态同步突变 局部放电脉冲信号     

可调脉冲宽度的调Q掺铥双包层光纤激光器

在激光器输出平均功率一定的情况下,峰值功率主要取决于调制频率和脉冲宽度。这使得脉冲宽度的调节具有一定的实际应用价值。对调Q掺铥双包层光纤激光器进行研究,首先确定了激光器的最佳输出透过率,在65%最佳透过率时,得到2 m激光的输出功率3.9 W,斜率效率为31%。外接一个信号发生器,信号门宽从12 s变化到18 s,并测量了调制频率分别在30 kHz、40 kHz和50 kHz时输出脉冲宽度的变化情况,得到了555.6 W的最高峰值功率,实现了脉冲宽度从163.4 ns到207.9 ns的变化。实验情况证实了用外接信号发生器能有效控制激光器的输出脉冲宽度。     

Laser drilling of thick material using femtosecond pulse with a focus of dual-frequency beam

Laser drilling is one of the basic, most frequently performed, material removal processes. The drilling aspect ratio is theoretically limited by the size and the focal depth of the machining laser spot. The aspect ratio can be improved by using dual focus. In this paper we describe a focus of two different frequencies based on the longitudinal chromatic aberration arisen when polychromatic collimated light is incident on a positive lens element. In the experiments, a Ti:Sapphire laser of 800 nm wavelength and 150 fs pulse duration was used as a source. Two tightly focused laser spots few hundred micrometers apart from each other were formed by focusing a combined collimated laser beam which contains the fundamental optic frequency and the second harmonic optic frequency. The focus of dual-frequency beam was used to drill a 3 mm thick PMMA plate. The drilling aspect ratio of a dual-frequency beam was compared to that of a focus of single frequency beam. Experimental results reveal that dual-frequency beam increases the aspect ratio and improves the drilling quality in terms of profile of the produced features.