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11.
12.
A series of complexes formed between halogen-containing molecules and ammonia have been investigated by means of the atoms in molecules (AIM) approach to gain a deeper insight into halogen bonding. The existence of the halogen bond critical points (XBCP) and the values of the electron density (Pb) and Laplacian of electron density (V2pb) at the XBCP reveal the closed-shell interactions in these complexes. Integrated atomic properties such as charge, energy, polarization moment, volume of the halogen bond donor atoms, and the corresponding changes (△) upon complexation have been calculated. The present calculations have demonstrated that the halogen bond represents different AIM properties as compared to the well-documented hydrogen bond. Both the electron density and the Laplacian of electron density at the XBCP have been shown to correlate well with the interaction energy, which indicates that the topological parameters at the XBCP can be treated as a good measure of the halogen bond strength In addition, an excellent linear relationship between the interatomic distance d(X…N) and the logarithm of Pb has been established. 相似文献
13.
《Physics letters. A》2006,349(6):462-466
Many social, technological, biological and economical systems are best described by evolved network models. In this short Letter, we propose and study a new evolving network model. The model is based on the new concept of neighbourhood connectivity, which exists in many physical complex networks. The statistical properties and dynamics of the proposed model is analytically studied and compared with those of Barabási–Albert scale-free model. Numerical simulations indicate that this network model yields a transition between power-law and exponential scaling, while the Barabási–Albert scale-free model is only one of its special (limiting) cases. Particularly, this model can be used to enhance the evolving mechanism of complex networks in the real world, such as some social networks development. 相似文献
14.
In the present paper, we prove that the Bernstein-Kantorovič operators have the ability of preserving translation property
in both C and Lp norms.
Supported (in part) by the NSFC(10471130,10371024) of PRC and the Natural Science Foundation (Y604003) of Zhejiang Province. 相似文献
15.
《Electrochemistry communications》2007,9(8):1991-1997
The controllability of pore density and diameter is critical for emerging applications, e.g., non-lithographic photonic-crystal formation; however pore density and diameter could either increase or decrease self-orderedly with enhanced current density. In this letter, similar paradoxical phenomena were demonstrated; the etch rate as a function of field strength was evidenced and interpreted in light of current-burst-model. Based on a hybrid of SCR (space charge region) and breakdown effects, a semi-quantitative model was established in order to disentangle the paradox: such a model could also potentially serve as a design reference for various applications as far as breakdown comes into play. The paradox was finally found to be dominated by physics on patterned samples. 相似文献
16.
《Physica A》2006,365(1):190-196
The formula for probability density functions (PDFs) has been extended to include PDF for energy dissipation rates in addition to other PDFs such as for velocity fluctuations, velocity derivatives, fluid particle accelerations, energy transfer rates, etc., and it is shown that the formula actually explains various PDFs extracted from direct numerical simulations and experiments performed in a wind tunnel. It is also shown that the formula with appropriate zooming increment corresponding to experimental situation gives a new route to obtain the scaling exponents of velocity structure function, including intermittency exponent, out of PDFs of velocity fluctuations. 相似文献
17.
《Journal of magnetism and magnetic materials》2005,294(2):99-106
The article reviews and updates the understanding of the soft magnetic properties of nanocrystalline Fe-based alloys. In optimized compositions the random magneto-crystalline anisotropy of the structural phases is largely averaged out. The soft magnetic properties are then controlled by magneto-elastic and induced anisotropies which are uniform on a scale much larger than the exchange length. But unlike to the case of soft magnetic amorphous alloys, there is still a competition between the random and the more uniform anisotropy contributions. The experimental findings are complemented by theoretical results. 相似文献
18.
A simple and rapid method is developed to determine the high acidity and the basicity of solutions by chronopotentiometry with a platinum working electrode. The acidity range from 5.0 mol/l H+ to 1.0 mol/l OH− can be measured by the adjustment of deposition potential and time. The response mechanism to acidity and basicity has been explored. The transition potential plateau in chronopotentiograms is caused from the oxidation of hydrogen adsorbed on electrode surface. 相似文献
19.
《Physica A》2006,371(2):667-673
A new traffic flow model called density viscous continuum model is developed to describe traffic more reasonably. The two delay time scales are taken into consideration, differing from the model proposed by Xue and Dai [Phys. Rev. E 68 (2003) 066123]. Moreover the relative density is added to the motion equation from which the viscous term can be derived, so we obtain the macroscopic continuum model from microscopic car following model successfully. The condition for stable traffic flow is derived. Nonlinear analysis shows that the density fluctuation in traffic flow induces density waves. Near the onset of instability, a small disturbance could lead to solitons determined by the Korteweg-de-Vries (KdV) equation, and the soliton solution is derived. The results show that local cluster effects can be obtained from the new model and are consistent with the diverse nonlinear dynamical phenomena observed in the freeway traffic. 相似文献
20.