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961.
采用羟基铁离子柱撑Na-Mont制备出1.0Fe-PILC,通过超声浸渍法合成不同铜负载量的nCu-Fe-PILC,并测试了其在富氧条件下催化C_3H_6选择性催化还原NO的性能。通过N_2吸附脱附、XRD、UV-Vis、H_2-TPR、Py-FTIR等技术手段表征催化剂的微观结构和物化性质,进一步解释其催化反应机理。结果表明,Cu的引入提高了1.0Fe-PILC的中低温活性和抗水硫能力。其中9Cu-Fe-PILC在300℃时NO转化率可达69.8%以上,400℃后NO转化率保持在99%以上且水硫影响较小。XRD、N_2吸附脱附结果表明,催化剂的SCR活性与所负载的活性组分和催化剂的吸附能力有关。UV-Vis结果表明,9Cu-Fe-PILC具有较强的中低温活性,与其含有较多的游离态Cu~(2+)有关。H_2-TPR结果表明,与1.0Fe-PILC相比,经Cu修饰的nCu-Fe-PILC获得了中低温还原能力。Py-FTIR结果表明,nCu-Fe-PILC表面同时含有Lewis酸和Br?nsted酸,Lewis酸是影响催化剂SCR活性的主要因素。 相似文献
962.
963.
964.
Calculation of High Frequency Complex Permeability of Carbonyl Iron Flakes in a Nomagnetic Matrix 总被引:1,自引:0,他引:1 下载免费PDF全文
The carbonyl iron flakes are fabricated by high-energy ball milling. The effective permeability is measured and calculated for the composite consisting of flakes embedded in a nonmagnetic matrix. The magnetic flakes with a shape anisotropy and random spatial distribution of normal direction are considered to calculate the complex permeability of magnetic flake materials. Its analytical model is derived from the Landau-Lifshitz-Gilbert equation and Bruggeman 's effective medium theory. The calculated results agree well with the experiment. 相似文献
965.
We propose a non-stationary method to measure the energy relaxation time of Josephson tunnel junctions from microwave enhanced escape phenomena. Compared with the previous methods, our method possesses simple and accurate features. Moreover, having determined the energy relaxation time, we can further obtain the coupling strength between the microwave source and the junction by changing the microwave power. 相似文献
966.
Forcible-Measurement Attack on Quantum Secure Direct Communication Protocol with Cluster State 下载免费PDF全文
The security of the quantum secure direct communication (QSDC) protocol with cluster state is analysed. It is shown that the secret would be partially leaked out when an eavesdropper performs forcible measurements on the transmitted particles. With the help of the result in minimum error discrimination, an upper bound (i.e. 40%) of this leakage is obtained. Moreover, the particular measurements which makes the leakage reach this bound are given. 相似文献
967.
Conductive perovskite BaPb03 (BPO) films as a potential electrode material of PZT capacitors used in ferroelectric random access memory are prepared by rf magnetron sputtering. An x-ray diffractometer and standard four probe method are employed to investigate the dependence of growth conditions on crystal structure and conductivity of BPO films. It is found that BPO films with perovskite phase can be obtained at substrate temperatures above 425℃, and the sample with the lowest resistivity is obtained at 450℃ under pure argon atmosphere. Using this BPO film as electrode, ferroelectric properties of BPO/PZT/BPO and Pt/PZT/BPO sandwiched structures are evaluated. Their remanent polarization and coercive field are 36.6 ℃/cm^2 (81.3 k V/cm) and 36.9℃/cm^2 (89.1 kV/cm), respectively. The coercive field of the former structure is lower than that of the latter, but remanent polarizations are almost the same. In addition, the results imply that BPO electrode is helpful to improve the fatigue resistance of PZT. The reasons are discussed. 相似文献
968.
Self-Injection and Acceleration of Monoenergetic Electron Beams from Laser Wakefield Accelerators in a Highly Relativistic Regime 下载免费PDF全文
H.Yoshitama ;T.Kameshima ;谷渝秋 ;郭仪 ;焦春晔 ;刘红杰 ;彭翰生 ;唐传铭 ;王小东 ;温贤伦 ;温天舒 ;吴玉迟 ;张保汉 ;朱启华 ;黄晓军 ;安维民 ;黄文会 ;唐传祥 ;林郁正 ;王小东 ;陈黎明 ;H.Kotaki ;M.Kando ;K.Nakajima 《中国物理快报》2008,25(8):2938-2941
Self-injection and acceleration of monoenergetic electron beams from laser wakefield accelerators are first investigated in the highly relativistic regime, using 100 TW class, 27 fs laser pulses. Quasi-monoenergetic multi- bunched beams with energies as high as multi-hundredMeV are observed with simultaneous measurements of side-scattering emissions that indicate the formation of self-channelfing and self-injection of electrons into a plasma wake, referred to as a 'bubble'. The three-dimensional particle-in-cell simulations confirmed multiple self-injection of electron bunches into the bubble and their beam acceleration with gradient of 1.5 GeV/cm. 相似文献
969.
Cryptanalysis of Multiparty Quantum Secret Sharing of Quantum State Using Entangled States 下载免费PDF全文
Security of a quantum secret sharing of quantum state protocol proposed by Guo et al. [Chin. Phys. Lett. 25 (2008) 16] is reexamined. It is shown that an eavesdropper can obtain some of the transmitted secret information by monitoring the classical channel or the entire secret by intercepting the quantum states, and moreover, the eavesdropper can even maliciously replace the secret message with an arbitrary message without being detected. Finally, the deep reasons why an eavesdropper can attack this protocol are discussed and the modified protocol is presented to amend the security loopholes. 相似文献
970.
A hypothesis is brought forward that the materials with low propagation loss in both optical and microwave band may exhibit good performance in terahertz (THz) band because THz wave band interspaces those two wave bands. For the purpose-of exploring a kind of low-loss material for THz waveguide, Lu2.1Bi0.9Fe5O12(LuBiIG) garnet films are prepared by liquid phase epitaxy (LPE) method on a gadolinium gallium garnet (GGG) substrate from lead-free flux because of the good properties in both optical and microwave bands. In microwave band, the ferromagnetic resonance (FMR) linewidth of the film 2△H = 2.8-5.1Oe; in optical band, the optical absorption coefficient is 600cm^-1 at visible range and about 100-170cm^-1 when the wavelength is longer than 800nm. In THz range, our hypothesis is well confirmed by a THz-TDS measurement which shows that the absorbance of the film for THz wave is 0.05-0.3 cm 1 and the minimum value appears at 2.3 THz. This artificial ferromagnetic material holds a great promise for magnetic field tunable THz devices such as waveguide, modulator or switch. 相似文献